相关论文: Magnetic interactions and spin dynamics in the bon…
We present results of $^{23}$Na and $^{19}$F nuclear magnetic resonance (NMR) measurements on NaCaCo$_2$F$_7$, a frustrated pyrochlore magnet with a Curie-Weiss temperature, $T_{cw}$ ~-140 K, and intrinsic bond disorder. Below 3.6 K both…
We report the crystal growth, crystal structure and basic magnetic properties of a new cobalt-based pyrochlore, NaSrCo$_2$F$_7$. Na and Sr are completely disordered on the non-magnetic large atom A sites, while magnetic S=3/2 Co$^{2+}$…
In this study, I have investigated the magnetic and critical properties of manganese pyrochlore fluoride NaSrMn$_{2}$F$_{7}$, which exhibits a glass transition at T$_\text{f}$$=$2.5 (K) due to charge disorder. A DFT+$U$+SOC framework is…
Cobalt pyrochlore fluoride NaCaCo$_2$F$_7$ is a disordered frustrated magnet composed of Co$^{2+}$ ions with an effective spin-$\frac{1}{2}$ magnetic moment and exhibits spin freezing below $T_f \sim$2.4 K. We perform ultrasound velocity…
Weak bond disorder disrupts the expected spin-liquid ground-state of the ideal $S$ = 1/2 Heisenberg pyrochlore antiferromagnet. Here we introduce a single crystal study of the structural and magnetic properties of the bond-disordered…
Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…
We report the magnetic characterization of the frustrated transition metal pyrochlore NaCaCo$_2$F$_7$. This material has high spin Co$^{2+}$ in CoF$_6$ octahedra in a pyrochlore lattice, and disordered non-magnetic Na and Ca on the…
The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold…
The spin dynamics in the geometrically frustrated pyrochlore antiferromagnet $\rm Gd_2Sn_2O_7$ is studied by means of the electron spin resonance. In the ordered phase ($T_N = 1$ K), we have detected three gapped resonance modes. Their…
We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…
The spin-1 anisotropic antiferromagnet NiCl_2-4SC(NH2)_2 exhibits a field-induced quantum phase transition that is formally analogous to Bose-Einstein condensation. Here we present results of systematic high-field electron spin resonance…
The crystal structures and magnetic properties of three previously unreported A2B2F7 pyrochlore materials, NaSrMn2F7, NaCaFe2F7, and NaSrFe2F7 are presented. In these compounds, either S=2 Fe2+ or S=5/2 Mn2+ is on the B site, while…
NaCaNi$_2$F$_7$ is an insulating, frustrated A$_2$B$_2$F$_7$ pyrochlore with magnetic S = 1 Ni$^{2+}$ on the pyrochlore B site. Non-magnetic Na and Ca are disordered on the A-site. Magnetic susceptibility measurements made on an oriented…
We report the observation of spin glass state in the double perovskite oxide Sr$_{2}$FeCoO$_{6}$ prepared through sol-gel technique. Initial structural studies using x rays reveal that the compound crystallizes in tetragonal $I 4/m$…
We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…
A single crystal of the Co2+ based pyrochlore NaCaCo2F7 was studied by inelastic neutron scattering. This frustrated magnet with quenched exchange disorder remains in a strongly correlated paramagnetic state down to one 60th of the…
We report a random singlet ground state in the $S=\frac{1}{2}$ Heisenberg pyrochlore antiferromagnet NaCdCu$_2$F$_7$. Cationic Na$^+$/Cd$^{2+}$ disorder on the pyrochlore $A$ site generates a broad distribution of…
We report an experimental study of the static magnetization $M(H,T)$ and high-field electron spin resonance (ESR) of polycrystalline \MgGd, a representative member of the newly discovered class of the so-called tripod-kagome…
The $T$-dependence (2- 400 K) of the electron paramagnetic resonance (EPR), magnetic susceptibility, $\chi (T)$, and specific heat, $C_{v}(T)$, of the $normal$ antiferromagnetic (AFM) spinel ZnCr$_{2}$O$_{4}$ and the spin-glass (SG)…
We report the experimental and the analytical results of electron spin resonance (ESR) and magnetization in high magnetic fields up to about 68 T of the quasi two-dimensional triangular lattice antiferromagnet NiGa$_2$S$_4$. From the…