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Most active colloid experiments are quasi-2D. Here a 3D density-matched solution of active particles propelled and aligned with an AC electric field uniquely facilitates measurement of short and long-range particle-wall interactions.…

软凝聚态物质 · 物理学 2025-05-02 Sandeep Ramteke , Jordan Dehmel , Touvia Miloh , Jarrod Schiffbauer , Alicia Boymelgreen

In the study of optical properties of large atomic system, a weak laser driving is often assumed to simplify the system dynamics by linearly coupled equations. Here, we investigate the light scattering properties of atomic ensembles beyond…

量子物理 · 物理学 2024-07-24 Chung-Hsien Wang , Nai-Yu Tsai , Yi-Cheng Wang , H. H. Jen

We show that optical properties of linear molecular aggregates undergo drastic changes when aggregates are deposited on a metal surface. The dipole-dipole interactions of monomers with their images can result in strong {re-structuring of…

材料科学 · 物理学 2008-11-19 A. V. Malyshev , V. A. Malyshev

Exciton transport in molecular aggregates with magic-angle orientation is expected to be strongly suppressed due to their negligible dipole-dipole interactions. However, recent reports show that light-matter interactions can significantly…

化学物理 · 物理学 2026-03-10 Siwei Wang , Liang-Yan Hsu , Hsing-Ta Chen

In a joint theoretical and experimental work the optical properties of azobenzene-functionalized self-assembled monolayers (SAMs) are studied at different molecular packing densities. Our results, based on density-functional and many-body…

材料科学 · 物理学 2016-12-19 Caterina Cocchi , Thomas Moldt , Cornelius Gahl , Martin Weinelt , Claudia Draxl

The interaction of laser radiation with single J aggregates of cyanine dyes is theoretically analyzed and numerically simulated. The quantum mechanical calculations of the equilibrium geometry and the energies and intensities of the lowest…

The pronounced light-matter interactions in photonic crystals make them interesting as opto-fludic "building blocks" for lab-on-a-chip applications. We show how conducting electrolytes cause dissipation and smearing of the…

光学 · 物理学 2007-05-23 Niels Asger Mortensen , Simon Ejsing , Sanshui Xiao

The dynamic charge susceptibility and the optical conductivity are calculated in the planar t-J model within the memory function method, working directly in terms of Hubbard operators. The density fluctuation spectrum consists of a damped…

强关联电子 · 物理学 2009-10-31 G. Jackeli , N. M. Plakida

The positive effects of various perturbations introduced in a bidimensional photonic-crystal patterned membrane on its integrated absorption are investigated numerically and theoretically. Two phenomena responsible for the enhanced…

New ways to treat electron correlation in electronic structure problems are discussed in the context of many-electron theory. The present work focuses primarily on static correlation. In related work, a method for including dynamical…

化学物理 · 物理学 2018-09-05 Jerry L. Whitten

We study the evolution of the optical conductivity in the t-J model with temperature and doping using the Extended Dynamical Cluster Approximation. The cluster approach results in an optical mass which is doping independent near half…

强关联电子 · 物理学 2009-11-11 Kristjan Haule , Gabriel Kotliar

We theoretically investigate optical absorption of molecules embedded nearby metallic antennas by using discrete dipole approximation method. It is found that the spectral peak of the absorption is shifted due to the radiation-induced…

介观与纳米尺度物理 · 物理学 2015-10-01 Yoshiki Osaka , Nobuhiko Yokoshi , Hajime Ishihara

We show that the third-order optical response of disordered linear J-aggregates can be calculated by considering only a limited number of transitions between (multi-) exciton states. We calculate the pump-probe absorption spectrum resulting…

无序系统与神经网络 · 物理学 2009-11-13 J. A. Klugkist , V. A. Malyshev , J. Knoester

We present a linear-response formalism for a system of correlated electrons out of equilibrium, as relevant for the probe optical absorption in pump-probe experiments. We consider the time dependent optical conductivity $\sigma(\omega,t)$…

强关联电子 · 物理学 2017-04-04 Zala Lenarčič , Denis Golež , Janez Bonča , Peter Prelovšek

Many soft-matter and biophysical systems are composed of monomers which reversibly assemble into rod-like aggregates. The aggregates can then order into liquid-crystal phases if the density is high enough, and liquid-crystal ordering…

软凝聚态物质 · 物理学 2010-07-27 Tatiana Kuriabova , M. D. Betterton , Matthew A. Glaser

We study numerically the phases and dynamics of a dense collection of self-propelled particles with soft repulsive interactions in two dimensions. The model is motivated by recent in vitro experiments on confluent monolayers of migratory…

软凝聚态物质 · 物理学 2015-05-28 Silke Henkes , Yaouen Fily , M. Cristina Marchetti

The theoretical studies of light absorption and scattering spectra of the plexcitonic two-layer triangular nanoprisms and three-layer nanospheres are reported. The optical properties of such metal-organic core--shell and core--double-shell…

光学 · 物理学 2022-02-09 Alexey D. Kondorskiy , Sergey S. Moritaka , Vladimir S. Lebedev

Using computer simulations, we identify the mechanisms causing aggregation and structural arrest of colloidal suspensions interacting with a short-ranged attraction at moderate and high densities. Two different non-ergodicity transitions…

凝聚态物理 · 物理学 2009-11-07 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

Solid-state spin defects are attractive candidates for developing quantum sensors and simulators. The spin and charge degrees of freedom in large defect ensembles are a promising platform to explore complex many-body dynamics and the…