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H3LiIr2O6 is the first honeycomb-lattice system without any signs of long-range magnetic order down to the lowest temperatures, raising the hope for the realization of an ideal Kitaev quantum spin liquid. Its honeycomb layers are coupled by…

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Strongly enhanced quantum fluctuations often lead to a rich variety of quantum-disordered states. A representative case is liquid helium, in which zero-point vibrations of the helium atoms prevent its solidification at low temperatures. A…

Quantum spin liquids (QSLs) represent exotic states of matter where quantum spins interact strongly yet evade long-range magnetic order down to absolute zero. Characterized by non-local quantum entanglement and resultant fractionalized…

强关联电子 · 物理学 2025-12-05 Yuji Matsuda , Takasada Shibauchi , Hae-Young Kee

Kitaev magnets are materials with bond-dependent Ising interactions between localized spins on a honeycomb lattice. Such interactions could lead to a quantum spin-liquid (QSL) ground state at zero temperature. Recent theoretical studies…

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

强关联电子 · 物理学 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome

The quantum spin liquid (QSL) state has been searched intensively in Kitaev-like materials, such as the Iridium oxides $A_2$IrO$_3$ and $\alpha$-RuCl$_3$. The half-filled Kitaev-Hubbard model with bond dependent hopping terms is used to…

强关联电子 · 物理学 2022-10-06 Shaojun Dong , Hao Zhang , Chao Wang , Meng Zhang , Yong-Jian Han , Lixin He

A decade ago, Alexei Kitaev proposed an exactly solvable $S$ = 1/2 model on a two-dimensional honeycomb lattice, where the spins fractionalize into Majorana fermions and form a topological quantum spin liquid (QSL) in the ground state. It…

强关联电子 · 物理学 2022-01-21 Hidenori Takagi , Tomohiro Takayama , George Jackeli , Giniyat Khaliullin , Stephen E. Nagler

Kitaev iridates have been proposed as candidates for realizing an elusive quantum spin liquid (QSL) state, in which strong spin-orbit coupling and bond-directional exchange generate a highly frustrated and entangled ground state. However,…

Recently H$_3$LiIr$_2$O$_6$ has been reported as a spin-orbital entangled quantum spin liquid (QSL) [K. Kitagawa et al., Nature {\bf 554}, 341 (2018)], albeit its connection to Kitaev QSL has not been yet identified. To unveil the related…

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

强关联电子 · 物理学 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

Pursuing the exotic quantum spin liquid (QSL) state in the Kitaev material $\alpha$-RuCl$_3$ has intrigued great research interest recently. A fascinating question is on the possible existence of field-induced QSL phase in this compound.…

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

强关联电子 · 物理学 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

We present a theory of a hybrid quantum liquid state, $\textit{quantum spin-dipole liquid}$ (QSDL), in a hydrogen-bonded electron system, by combining a quantum proton ice and Anderson's resonating valence bond spin liquid theory, motivated…

强关联电子 · 物理学 2020-10-16 Masahiko G. Yamada , Yasuhiro Tada

The Kitaev model belongs to an unconventional class of two-dimensional spin systems characterized by anisotropic, bond-dependent interactions that give rise to Quantum Spin Liquid (QSL) states. These exotic phases, marked by the absence of…

强关联电子 · 物理学 2026-01-29 A. R. Moura , L. V. Santos

The ground state of the bilayer Kitaev model with the Heisenberg-type interlayer exchange interaction is investigated by means of the exact diagonalization. Calculating the ground-state energy, local quantity defined on each plaquette, and…

强关联电子 · 物理学 2019-05-24 Hiroyuki Tomishige , Joji Nasu , Akihisa Koga

Layered honeycomb magnets are of interest as potential realizations of the Kitaev quantum spin liquid (KQSL), a quantum state with long-range spin entanglement and an exactly solvable Hamiltonian. Conventional magnetically ordered states…

强关联电子 · 物理学 2020-01-28 Ruidan Zhong , Tong Gao , Nai Phuan Ong , Robert J. Cava

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however,…

We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…

强关联电子 · 物理学 2018-03-29 Kevin Slagle , Wonjune Choi , Li Ern Chern , Yong Baek Kim
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