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The effects of interactions between He- and clusters of fullerenes in helium nanodroplets are described. Electron transfer from $He^{-}$ to $(C_{60})_n$ and $(C_{70})_n$ clusters results in the formation of the corresponding fullerene…

原子与分子团簇 · 物理学 2016-05-03 A. Mauracher , M. Daxner , S. E. Huber , J. Postler , M. Renzler , S. Denifl , P. Scheier , A. M. Ellis

We have studied complexes of gold atoms and imidazole (C$_3$N$_2$H$_4$, abbreviated Im) produced in helium nanodroplets. Following the ionization of the doped droplets we detect a broad range of different Au$_m$Im$_n^+$ complexes, however…

Dissociation and fission of small neutral, singly and doubly charged strontium clusters are studied by means of ab initio density functional theory methods and high-resolution time-of-flight mass spectrometry. Magic numbers for small…

原子与分子团簇 · 物理学 2009-09-29 A. Lyalin , A. V. Solov'yov , C. Brechignac , W. Greiner

We review the theory behind abundance of experimentally observed nanoclusters produced in beams, aiming to understand their magic number behavior. It is shown how use of statistical physics, with certain assumptions, reduces the calculation…

统计力学 · 物理学 2014-04-02 Kiamars Vafayi , Keivan Esfarjani

The distribution of the sizes of clusters is not continuous, but rather has local maxima. The numbers of atoms of those maxima distribution is called magic numbers. Two methods of determining magic numbers are firstly introduced, followed…

材料科学 · 物理学 2014-11-05 Siwei Luo

We present the results of over 90 tight-binding molecular-dynamics simulations of collisions between three- and five-atom silicon clusters, at a system temperature of 2000K. Much the most likely products are found to be two 'magic'…

原子与分子团簇 · 物理学 2007-05-23 A. R. Porter , R. W. Godby

We use a novel technique to solvate silver cations in small clusters of noble gases. The technique involves formation of large, superfluid helium nanodroplets that are subsequently electron ionized, mass-selected by deflection in an…

原子与分子团簇 · 物理学 2022-11-11 Masoomeh Mahmoodi-Darian , Paul Martini , Lukas Tiefenthaler , Jaroslav Kočišek , Paul Scheier , Olof Echt

We study superfluid helium droplets multiply charged with ions. When stable, the charges are found to reside in equilibrium close to the droplet surface, thus representing a physical realization of Thomson's model. We find the minimum…

介观与纳米尺度物理 · 物理学 2024-10-23 Ernesto Garcia-Alfonso , Francesco Ancilotto , Manuel Barranco , Fausto Cargnoni , Nadine Halberstadt , Marti Pi

Electron ionization of helium droplets doped with cesium or potassium results in doubly and, for cesium, triply charged cluster ions. The smallest observable doubly charged clusters are $Cs_{9}^{2+}$ and $K_{11}^{2+}$; they are a factor two…

原子与分子团簇 · 物理学 2016-09-07 Michael Renzler , Martina Harnisch , Matthias Daxner , Lorenz Kranabetter , Martin Kuhn , Paul Scheier , Olof Echt

Electron-induced chemistry in imidazole (IMI) clusters embedded in helium nanodroplets (with an average size of 2$\times$10$^5$ He atoms) has been investigated with high-resoluton time-of-flight mass spectrometry. The formation of both,…

原子与分子团簇 · 物理学 2018-05-03 M. Kuhn , S. Raggl , P. Martini , N. Gitzl , M. Mahmoodi Darian , M. Goulart , J. Postler , L. Feketeová , P. Scheier

Variational MonteCarlo and Diffusion MonteCarlo calculations have been carried out for cations like Li$^+$, Na$^+$ and K$^+$ as dopants of small helium clusters over a range of cluster sizes up to about 12 solvent atoms. The interaction has…

化学物理 · 物理学 2007-05-23 E. Coccia , E. Bodo , F. Marinetti , F. A. Gianturco , E. Yildrim , M. Yurtsever , E. Yurtsever

We present a new approach to understanding star-to-star helium abundance variations within globular clusters. We begin with detailed radiation hydrodynamics simulations of cluster formation within giant molecular clouds, and investigate the…

星系天体物理 · 物理学 2020-03-18 Alison Sills

Anions are formed by electron attachment to helium nanodroplets doped with N$_2$. The most prominent ion series is due to odd-numbered N$_m$$^{-}$ with 3 $\le$ m < 140. Neither N$^{-}$ nor N$_2$$^{-}$ are observed. An appearance energy of…

原子与分子团簇 · 物理学 2018-05-03 Nikolaus Weinberger , Johannes Postler , Paul Scheier , Olof Echt

We show that element diffusion can produce large fluctuations in the initial helium abundance of the star-forming clouds. Diffusion time-scale, which in stars is much larger than the Hubble time, can fall below 10^8 years in the neutral gas…

天体物理学 · 物理学 2009-11-11 Leonid Chuzhoy

We propose that the abundance anomalies of proton-capture elements in globular clusters, such as the C-N, Na-O, Mg-Al and Na-F anti-correlations, were produced by super-massive stars with M ~ 10,000 Msun. Such stars could form in the…

太阳与恒星天体物理 · 物理学 2015-06-16 Pavel A. Denissenkov , F. D. A. Hartwick

We use high-resolution three-dimensional adaptive mesh refinement simulations to investigate the interaction of high-redshift galaxy outflows with low-mass virialized clouds of primordial composition. While atomic cooling allows star…

宇宙学与河外天体物理 · 物理学 2021-11-24 William J Gray , Evan Scannapieco

We report on the production and study of stable, highly charged droplets of superfluid helium. Using a novel experimental setup we produce neutral beams of liquid helium nanodroplets containing millions of atoms or more that can be ionized…

The abundances of elements in stars are a critical clue to their origins. Observed star-to-star variations in logarithmic abundance within an open cluster are typically only $\sim 0.01-0.05$ over many elements, significantly smaller than…

星系天体物理 · 物理学 2015-06-22 Yi Feng , Mark R. Krumholz

The reactions of carbon atoms with dihydrogen have been investigated in liquid helium droplets at $T$ = 0.37 K. A calorimetric technique was applied to monitor the energy released in the reaction. The barrierless reaction between a single…

星系天体物理 · 物理学 2016-03-01 S. A. Krasnokutski , M. Kuhn , M. Renzler , C. Jäger , Th. Henning , P. Scheier

Helium abundances and atmospheric parameters have been determined from high resolution spectra for a new sample of 46 bright hot subdwarf B (sdB) stars. The helium abundances have been measured with high accuracy. We confirm the correlation…

太阳与恒星天体物理 · 物理学 2011-12-14 S. Geier , U. Heber , H. Edelmann , L. Morales-Rueda , D. Kilkenny , D. O'Donoghue , T. R. Marsh , C. Copperwheat
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