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Chemical reactions can be surprisingly efficient at ultracold temperatures ( < 1mK) due to the wave nature of atoms and molecules. The study of reactions in the ultracold regime is a new research frontier enabled by cooling and trapping…

原子物理 · 物理学 2017-01-16 Lee R. Liu , Jessie T. Zhang , Yichao Yu , Nicholas R. Hutzler , Yu Liu , Till Rosenband , Kang-Kuen Ni

We demonstrate the formation of a single RbCs molecule during the merging of two optical tweezers, one containing a single Rb atom and the other a single Cs atom. Both atoms are initially predominantly in the motional ground states of their…

We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer,…

We investigate the formation of ultracold NaCs molecules by photoassociation of Na and Cs atoms.

化学物理 · 物理学 2010-08-09 Xuan Li

We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…

We demonstrate the formation of a single NaCs molecule in an optical tweezer by magnetoassociation through an s-wave Feshbach resonance at 864.11(5)G. Starting from single atoms cooled to their motional ground states, we achieve conversion…

Trapping and optically interfacing laser-cooled neutral atoms is an essential requirement for their use in advanced quantum technologies. Here we simultaneously realize both of these tasks with cesium atoms interacting with a multi-color…

量子物理 · 物理学 2010-06-03 E. Vetsch , D. Reitz , G. Sagué , R. Schmidt , S. T. Dawkins , A. Rauschenbeutel

We present the first simultaneous trapping of two different ultracold atomic species in a conservative trap. Lithium and cesium atoms are stored in an optical dipole trap formed by the focus of a CO$_2$ laser. Techniques for loading both…

原子物理 · 物理学 2009-11-07 A. Mosk , S. Kraft , M. Mudrich , K. Singer , W. Wohlleben , R. Grimm , M. Weidemuller

The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic)…

量子物理 · 物理学 2009-07-23 M. Vatasescu

We demonstrate simultaneous deceleration and trapping of a cold atomic and molecular mixture. This is the first step towards studies of cold atom-molecule collisions at low temperatures as well as application of sympathetic cooling. Both…

We simulate collisions between two atoms, which move in an optical lattice under the dipole-dipole interaction. The model describes simultaneously the two basic dynamical processes, namely the Sisyphus cooling of single atoms, and the…

原子物理 · 物理学 2009-11-07 J. Piilo , K. -A. Suominen , K. Berg-Sorensen

The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…

It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…

原子物理 · 物理学 2015-05-27 E. S. Shuman , J. F. Barry , D. DeMille

We present a theoretical analysis of optical pathways for formation of cold Ca($^1$S)Na$^+$($^1$S) molecular ions via an intermediate state. The formation schemes are based on ab initio potential energy curves and transition dipole moments…

原子物理 · 物理学 2016-08-03 Marko Gacesa , John A. Montgomery , H. Harvey Michels , Robin Côté

Measurements of interactions between cold molecules and ultracold atoms can allow for a detailed understanding of fundamental collision processes. These measurements can be done using various experimental geometries including where both…

原子物理 · 物理学 2020-03-25 N. J. Fitch , L. P. Parazzoli , H. J. Lewandowski

Coupling of atoms is the basis of chemistry, yielding the beauty and richness of molecules. We utilize semiconductor nanocrystals as artificial atoms to form nanocrystal molecules that are structurally and electronically coupled. CdSe/CdS…

Recently, laser cooling methods have been extended from atoms to molecules. The complex rotational and vibrational energy level structure of molecules makes laser cooling difficult, but these difficulties have been overcome and molecules…

原子物理 · 物理学 2019-02-18 M. R. Tarbutt

Fully internal and motional state controlled and individually manipulable polar molecules are desirable for many quantum science applications leveraging the rich state space and intrinsic interactions of molecules. While prior efforts at…

Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its…

光学 · 物理学 2015-06-04 M. Alharbi , A. Husakou , B. Debord , F. Gerome , F. Benabid

Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the…

原子物理 · 物理学 2015-06-18 A. M. Jayich , A. C. Vutha , M. T. Hummon , J. V. Porto , W. C. Campbell
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