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Infrared spectra of the CO2-N2 dimer are observed in the carbon dioxide nu3 asymmetric stretch region (~2350 cm-1) using a tunable infrared optical parametric oscillator to probe a pulsed slit jet supersonic expansion. Previous results for…

原子与分子团簇 · 物理学 2020-07-15 A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

Rovibrational energy level calculations using a high-level intermolecular potential surface are reported for H2O-CO and D2O-CO. They predict the ground K = 1 levels to lie about 20 (12) cm-1 above K = 0 for H2O-CO (D2O-CO) in good agreement…

原子与分子团簇 · 物理学 2019-07-24 A. Barclay , A. van der Avoird , A. R. W. McKellar , N. Moazzen-Ahmadi

Extensive infrared spectra of the weakly-bound CO$_2$-CO dimer are observed in the carbon dioxide $\nu_3$ asymmetric stretch region (~2350 cm-1) using a tunable infrared OPO laser source to probe a pulsed slit jet supersonic expansion. Both…

原子与分子团簇 · 物理学 2021-05-28 A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

The infrared spectrum of the weakly-bound CO2-Xe complex is studied in the region of the carbon dioxide nu3 fundamental vibration (~2350 cm-1), using a tunable OPO laser source to probe a pulsed supersonic slit jet expansion. The Xe isotope…

原子与分子团簇 · 物理学 2021-06-30 A. J. Barclay , A. R. W. McKellar , Colin M. Western , N. Moazzen-Ahmadi

Spectra of water-CO2 dimers are studied using a tunable mid-infrared source to probe a pulsed slit jet supersonic expansion. H2O-CO2 and D2O-CO2 are observed in the CO2 nu3 fundamental region (~2350 cm-1), D2O-CO2 is also observed in the…

原子与分子团簇 · 物理学 2023-07-19 T. Gartner , C. Lauzin , A. R. W. McKellar , N. Moazzen-Ahmadi

The weak infrared spectrum of CO2-Ar corresponding to the (0111) <-- (0110) hot band of CO2 is detected in the region of the carbon dioxide nu3 fundamental vibration (~2340 cm-1), using a tunable OPO laser source to probe a pulsed…

原子与分子团簇 · 物理学 2020-10-28 T. A. Gartner , A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

The infrared spectrum of the weakly-bound CO2-Ne complex is studied in the region of the carbon dioxide nu3 fundamental vibration (~2350 cm-1), using a tunable OPO laser source to probe a pulsed supersonic slit jet expansion. For the…

原子与分子团簇 · 物理学 2021-11-02 A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

Weakly-bound CO2-Rg2 trimers are studied by high resolution (0.002 cm-1) infrared spectroscopy in the region of the CO2 nu3 fundamental band (~2350 cm-1), using a tunable OPO to probe a pulsed supersonic slit jet expansion with an effective…

化学物理 · 物理学 2024-06-19 A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

The infrared spectrum of the weakly-bound C2H4-CO2 complex is investigated in the region of the nu3 fundamental band of CO2 (~2350 cm-1), using a tunable OPO laser source to probe a pulsed supersonic slit jet expansion. The spacing of the…

原子与分子团簇 · 物理学 2020-07-01 A. R. W. McKellar , N. Moazzen-Ahmadi

The fundamental band for the OC-C2H2 dimer and two combination bands involving the intermolecular bending modes nu9 and nu8 in the carbon monoxide CO stretch region are re-examined. Spectra are obtained using a pulsed supersonic slit jet…

原子与分子团簇 · 物理学 2018-11-14 A. J. Barclay , A. Mohandesi , K. H. Michaelian , A. R. W. McKellar , N. Moazzen-Ahmadia

Using the Short-Wavelength-Spectrometer on the Infrared Space Observatory (ISO), we obtained near- and mid-infrared spectra toward the brightest H_2 emission peak of the Orion OMC-1 outflow. A wealth of emission and absorption features were…

天体物理学 · 物理学 2007-05-23 Dirk Rosenthal , Frank Bertoldi , Siegfried Drapatz

Vibrational-excitation cross sections of ground electronic state of carbon dioxide molecule by electron-impact through the CO2-(2\Pi) shape resonance is considered in the separation of the normal modes approximation. Resonance curves and…

化学物理 · 物理学 2016-11-01 V. Laporta , J. Tennyson , R. Celiberto

Cross sections for the rotational (de)excitation of CO by ground state para- and ortho-H_2 are obtained using quantum scattering calculations for collision energies between 1 and 520 cm^{-1}. A new CO-H_2 potential energy surface is…

天体物理学 · 物理学 2008-11-26 M. Wernli , P. Valiron , A. Faure , L. Wiesenfeld , P. Jankowski , K. Szalewicz

High resolution spectra of (CO$_2$)$_2$-Rg trimers (Rg = Ne, Ar, Kr, and Xe) in the region of the CO2 nu3 fundamental (~2350 cm$^{-1}$) are reported, using a tunable OPO laser source to probe a pulsed supersonic slit jet expansion. These…

原子与分子团簇 · 物理学 2022-07-27 A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

Using time-resolved infrared-vacuum-ultraviolet double-resonance spectroscopy, experimental room temperature measurements of state-to-state rate coefficients for rotational energy transfer within the X $^1\Sigma^+(v=2)$ vibrational state of…

量子物理 · 物理学 2026-03-10 Hamza Labiad , Alexandre Faure , Ian R. Sims

We present a unified variational treatment of the magnetic dipole matrix elements, Einstein coefficients and line strength for general open-shell diatomic molecules in the general purpose diatomic code Duo. Building on previous work in…

大气与海洋物理 · 物理学 2025-04-08 Wilfrid Somogyi , Sergey N. Yurchenko , Gap-Sue Kim

The spectra of pure, mixed and layered CO and CO2 ices have been studied systematically under laboratory conditions using infrared spectroscopy. This work provides improved resolution spectra (0.5 cm-1) of the CO2 bending and asymmetric…

天体物理学 · 物理学 2009-11-11 F. A. van Broekhuizen , I. M. N. Groot , H. J. Fraser , E. F. van Dishoeck , S. Schlemmer

We extend studies of micro-solvation of carbon monoxide by a combination of high-resolution IR spectroscopy and ab initio calculations. Spectra of the (H2O)4-CO and (D2O)4-CO pentamers are observed in the C-O stretch fundamental region…

原子与分子团簇 · 物理学 2021-02-24 A. J. Barclay , A. Pietropolli Charmet , A. R. W. McKellar , N. Moazzen-Ahmadi

Structural calculations and high-resolution infrared spectra are reported for trimers and tetramers containing CO$_2$ together with CO and/or N$_2$. Among the 9 clusters studied here, only (CO$_2$)$_2$-CO was previously observed by…

原子与分子团簇 · 物理学 2022-04-06 A. J. Barclay , A. R. W. McKellar , A. Pietropolli Charmet , N. Moazzen-Ahmadi

We investigate the bright CO fundamental emission in the central regions of five protostars in their primary mass assembly phase using new observations from JWST's Near-Infrared Spectrograph (NIRSpec) and Mid-Infrared Instrument (MIRI). CO…

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