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With the consideration of photon recycling effect, the efficiency limit of methylammonium lead iodide (CH3NH3PbI3) perovskite solar cells is predicted by a detailed balance model. To obtain convincing predictions, both AM 1.5 spectrum of…

材料科学 · 物理学 2015-07-01 Wei E. I. Sha , Xingang Ren , Luzhou Chen , Wallace C. H. Choy

Perovskite semiconductors have demonstrated outstanding external luminescence quantum yields, enabling high power conversion efficiencies (PCE). However, the precise conditions to advance to an efficiency regime above monocrystalline…

Deposition of perovskite thin films by antisolvent engineering is one of the most common methods employed in perovskite photovoltaics research. Herein, we report on a general method that allows the fabrication of highly efficient perovskite…

Perovskite solar cells (PSCs) have experienced a remarkable rise in power conversion efficiency (PCE) over the past 15 years, positioning them as a promising alternative or complement to silicon for large-scale photovoltaic deployment.…

Perovskite solar cells have reached power conversion efficiencies that rival those of established silicon photovoltaics. Nanotextures in perovskite solar cells scatter the incident light, thereby improving optical absorption. In addition,…

For opto-electronic and photo-voltaic applications of perovskites, it is essential to know the optical properties and intrinsic losses of the used materials. A systematic microscopic analysis is presented for the example of methylammonium…

材料科学 · 物理学 2018-10-29 Lars C. Bannow , Jörg Hader , Jerome V. Moloney , Stephan W. Koch

Selecting suitable charge transport layers and suppressing non-radiative recombination at interfaces to the absorber layer are vital to maximize the efficiency of halide perovskite solar cells. In this work, high-quality perovskite thin…

Fundamental electronic processes such as charge-carrier transport and recombination play a critical role in determining the efficiency of hybrid perovskite solar cells. The presence of mobile ions complicates the development of a clear…

材料科学 · 物理学 2020-12-17 Sebastian Reichert , Katelyn Goetz , Christopher Wöpke , Yana Vaynzof , Carsten Deibel

Perovskite solar cells (PSCs) without a hole transport layer (HTL) offer a cost-effective and stable alternative to conventional architectures, utilizing only an absorber layer and an electron transport layer (ETL). This study presents a…

机器学习 · 计算机科学 2025-05-27 Ihtesham Ibn Malek , Hafiz Imtiaz , Samia Subrina

III-V materials show a wide range of gaps making them ideal for the design of high efficiency solar cells. This chapter reviews relevant growth methods and material properties of these materials and discusses methods of combining…

材料科学 · 物理学 2013-01-08 James P. Connolly , Denis Mencaraglia

Light Management (LM) is essential for metal-halide perovskite solar cells in their race for record performance. In this review, criteria on materials, processes and photonic engineering are established such as to enhance mainly the short…

This paper presents a multiscale approach to evaluate perovskite solar cell performance which determines material properties at the atomistic scale with first-principles calculations, and applies them in macro-scale device models. This work…

Fully-textured perovskite/silicon tandem solar cells have emerged as promising candidates for next-generation photovoltaics. The optical functions of full texturing, however, are not yet fully understood. A key challenge is the requirement…

光学 · 物理学 2025-11-05 Michel Gaglioni Rocha , Emiliano Rezende Martins

Next-generation low-cost semiconductors such as halide perovskites exhibit optoelectronic properties dominated by nanoscale variations in their structure, composition and photophysics. While microscopy provides a proxy for ultimate device…

Perovskite/Si tandem solar cells have the potential to considerably out-perform conventional solar cells. Under standard test conditions, perovskite/Si tandem solar cells already outperform the Si single junction. Under realistic…

材料科学 · 物理学 2017-08-23 Moritz H. Futscher , Bruno Ehrler

It is currently possible to fabricate crystalline silicon solar cells with the absorber thickness ranging from a few hundreds of micrometers (conventional wafer-based cells) to devices as thin as $1\,\mu\mathrm{m}$. In this work, we use a…

光学 · 物理学 2015-05-18 Piotr Kowalczewski , Lucio Claudio Andreani

Drift-diffusion model is an indispensable modeling tool to understand the carrier dynamics (transport, recombination, and collection) and simulate practical-efficiency of solar cells (SCs) through taking into account various carrier…

介观与纳米尺度物理 · 物理学 2017-04-20 Xingang Ren , Zishuai Wang , Wei E. I. Sha , Wallace C. H. Choy

The quest for optimal perovskite for tandem cell configurations is challenging as it involves several factors ranging from device level performance under field conditions to degradation rates and cost. Here, we first highlight the…

材料科学 · 物理学 2025-09-03 Karthik Raitani , Pradeep R. Nair

We study the radiative decay, or fluorescence, of excitons in organic solar cells as a function of its geometrical parameters. Contrary to their non-radiative counterpart, fluorescence losses strongly depend on the environment. By properly…

应用物理 · 物理学 2017-10-04 Blaise Godefroid , Gregory Kozyreff

The ability to extract material parameters of perovskite from quantitative experimental analysis is essential for rational design of photovoltaic and optoelectronic applications. However, the difficulty of this analysis increases…