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Plasmonic dimer cavities can induce extreme electric-field hot spots that allow one to access ultrastrong coupling regimes using Raman-type spectroscopy on single vibrating molecules. Using a generalized master equation, we study resonant…

量子物理 · 物理学 2021-07-29 Stephen Hughes , Alessio Settineri , Salvatore Savasta , Franco Nori

Electromagnetic (EM) coupling between molecular exciton and plasmon has been studied using in Rayleigh scattering or extinction spectroscopy. However, evaluating EM coupling involving subradiant plasmon is challenging because this resonance…

光学 · 物理学 2026-05-15 Tamitake Itoh , Yuko S. Yamamoto

We report plasmon-enhanced Raman scattering in graphene coupled to a single plasmonic hotspot measured as a function of laser energy. The enhancement profiles of the G peak show strong enhancement (up to $10^5$) and narrow resonances (30…

This study investigated spectral changes in the absorption cross-sections of single strong coupling systems composed of single silver nanoparticle dimers and a few dye molecules during the quenching of surface-enhanced resonant Raman…

光学 · 物理学 2019-06-10 Tamitake Itoh , Yuko S. Yamamoto , Takayuki Okamoto

Surface enhanced Raman scattering mediated by surface plasmons polaritons with wave vector much larger than those of light is considered. The excitation of these polaritons and their efficient Raman scattering due to low group velocity and…

光学 · 物理学 2015-06-04 Tomas Lopez-Rios

We present a general model study of surface-enhanced resonant Raman scattering and fluorescence focusing on the interplay between electromagnetic effects and the molecular dynamics. Our model molecule is placed close to two Ag…

其他凝聚态物理 · 物理学 2007-05-23 Hongxing Xu , Xue-Hua Wang , Martin P. Persson , H. Q. Xu , Mikael Kall , Peter Johansson

Using resonant Raman scattering spectroscopy with 25 different laser lines, we describe the Raman scattering spectra of mono- and multi-layers 2H-molybdenum diselenide (MoSe$_2$) as well as the different resonances affecting the most…

介观与纳米尺度物理 · 物理学 2016-04-19 P. Soubelet , A. E. Bruchhausen , A. Fainstein , K. Nogajewski , C. Faugeras

We present a microscopic model describing the transition to strong coupling regime for an emitter resonantly coupled to a surface plasmon in a metal-dielectric structure. We demonstrate that the shape of scattering spectra is determined by…

介观与纳米尺度物理 · 物理学 2022-07-08 Tigran V. Shahbazyan

The spectral relationships between surface enhanced resonant Raman scattering (SERRS) and plasmon resonance observed in far field scattering cross are investigated using single silver nanoparticle dimers with focusing on the lowest energy…

光学 · 物理学 2023-04-07 Tamitake Itoh , Yuko S. Yamamoto

Methods to increase the light scattered from small particles can help improve the sensitivity of many sensing techniques. Here, we investigate the role multiple scattering plays in perturbing the scattered signal when a particle is added to…

光学 · 物理学 2021-08-03 Joel Berk , Matthew R. Foreman

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

We present a general model study of surface-enhanced resonant Raman scattering and fluorescence, focusing on the interplay between electromagnetic (EM) effects and the molecular dynamics as treated by a density matrix calculation. The model…

其他凝聚态物理 · 物理学 2007-05-23 Peter Johansson , Hongxing Xu , Mikael Käll , ;

We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…

光学 · 物理学 2015-03-25 Maxim Sukharev , Paul N. Day , Ruth Pachter

Raman spectra obtained by the inelastic scattering of light by crystalline solids contain contributions from first-order vibrational processes (e.g. the emission or absorption of one phonon, a quantum of vibration) as well as higher-order…

材料科学 · 物理学 2017-08-22 Yannick Gillet , Stefan Kontur , Matteo Giantomassi , Claudia Draxl , Xavier Gonze

Presented here are studies of the impact of excitation angle on surface enhanced Raman and luminescence spectroscopy of dye immobilised on a plasmon active nanocavity array support. Results show that both Raman and luminescence intensities…

光学 · 物理学 2015-05-20 Frances Lordan , James H Rice , Bincy Jose , Robert J Forster , Tia E Keyes

Effects of coupling between a molecular exciton and a surface plasmon (exciton-plasmon coupling) on the luminescence properties of the molecule and the surface plasmons are investigated using the nonequilibrium Green's function method.…

材料科学 · 物理学 2013-06-12 Kuniyuki Miwa , Mamoru Sakaue , Hideaki Kasai

Interaction between plasmonic nanostructures and molecules is modeled based on the concept of quantized optical cavity for surface enhanced Raman scattering process. We have found that the background emission from plasmonic nanostructures…

光学 · 物理学 2017-03-22 Yuqing Cheng , Jingyi Zhao , Te Wen , Guantao Li , Jianning Xu , Qihuang Gong , Guowei Lu

The amplification of evanescent waves by flat superlens requires a near-resonance coupling which has been linked to resonant surface plasmons. A subtle interplay has been proposed to exist between the excitation of well-defined resonant…

经典物理 · 物理学 2021-01-14 Ali Isa

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

介观与纳米尺度物理 · 物理学 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

Two-magnon Raman scattering provides important information about electronic correlations in the insulating parent compounds of high-$T_c$ materials. Recent experiments have shown a strong dependence of the Raman signal in $B_{1g}$ geometry…

强关联电子 · 物理学 2009-10-30 Dirk K. Morr , Andrey V. Chubukov
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