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The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

介观与纳米尺度物理 · 物理学 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

The nitrogen-vacancy (NV) center can serve as a magnetic sensor for electron paramagnetic resonance (EPR) measurements. Benefiting from its atomic size, the diamond chip can integrate a tremendous amount of NV centers to improve the…

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

量子物理 · 物理学 2024-11-12 Yuhang Ren , Susumu Takahashi

An ultimate goal of electron paramagnetic resonance (EPR) spectroscopy is to analyze molecular dynamics in place where it occurs, such as in a living cell. The nanodiamond (ND) hosting nitrogen-vacancy (NV) centers will be a promising EPR…

A nitrogen-vacancy (NV) center in diamond is a promising sensor for nanoscale magnetic sensing. Here we report electron spin resonance (ESR) spectroscopy using a single NV center in diamond. First, using a 230 GHz ESR spectrometer, we…

介观与纳米尺度物理 · 物理学 2016-10-05 Chathuranga Abeywardana , Viktor Stepanov , Franklin H. Cho , Susumu Takahashi

Electron paramagnetic resonance spectroscopy (EPR) is among the most important analytical tools in physics, chemistry, and biology. The emergence of nitrogen-vacancy (NV) centers in diamond, serving as an atomic-sized magnetometer, has…

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

介观与纳米尺度物理 · 物理学 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

The protocols for the control and readout of Nitrogen Vacancy (NV) centres electron spins in diamond offer an advanced platform for quantum computation, metrology and sensing. These protocols are based on the optical readout of photons…

介观与纳米尺度物理 · 物理学 2019-06-26 E. Bourgeois , A. Jarmola , M. Gulka , J. Hruby , D. Budker , M. Nesladek

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

Sensing of a few unpaired electron spins, such as metal ions and radicals, is a useful but difficult task in nanoscale physics, biology, and chemistry. Single nitrogen-vacancy (NV) centers in diamond offer high sensitivity and spatial…

介观与纳米尺度物理 · 物理学 2018-08-13 F. Gorrini , R. Giri , C. E. Avalos , S. Tambalo , S. Mannucci , L. Basso , N. Bazzanella , C. Dorigoni , M. Cazzanelli , P. Marzola , A. Miotello , A. Bifone

We present an alternative to conventional Electron Paramagnetic Resonance (EPR) spectroscopy equipment. Avoiding the use of bulky magnets and magnetron equipment, we use the photoluminescence of an ensemble of Nitrogen-Vacancy centers at…

应用物理 · 物理学 2023-03-08 C. Mignon , A. R. Ortiz Moreno , H. Shirzad , S. K. Padamati , V. Damle , Y. Ong , R. Schirhagl , M. Chipaux

Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the…

介观与纳米尺度物理 · 物理学 2015-06-11 H. J. Mamin , M. H. Sherwood , D. Rugar

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

A key limitation of electron paramagnetic resonance (EPR), an established and powerful tool for studying atomic-scale biomolecular structure and dynamics is its poor sensitivity, samples containing in excess of 10^12 labeled biomolecules…

We perform sensitive nuclear magnetic resonance (NMR) with spin ensembles which are polarized by nitrogen vacancy centers (NV centers) in diamond at room-temperature. With a near shot-noise-limited photoluminescence detection and a highly…

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing.…

量子物理 · 物理学 2021-03-31 C. Pellet-Mary , P. Huillery , M. Perdriat , A. Tallaire , G. Hétet

Dynamic nuclear polarization via contact with electronic spins has emerged as an attractive route to enhance the sensitivity of nuclear magnetic resonance (NMR) beyond the traditional limits imposed by magnetic field strength and…

Over the years, an enormous effort has been made to establish nitrogen vacancy (NV) centers in diamond as easily accessible and precise magnetic field sensors. However, most of their sensing protocols rely on the application of bias…

We present a technique that uses an ensemble of nitrogen-vacancy (NV) centers in diamond to image magnetic fields with high spatio-temporal resolution and sensitivity. A focused laser beam is raster-scanned using an acousto-optic deflector…

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