相关论文: Lattice-Mediated Magnetic Order Melting in TbMnO3
We performed ultrafast time-resolved near-infrared pump, resonant soft X-ray diffraction probe measurements to investigate the coupling between the photoexcited electronic system and the spin cycloid magnetic order in multiferroic TbMnO3 at…
We investigate the demagnetization dynamics of the cycloidal and sinusoidal phases of multiferroic TbMnO$_3$ by means of time-resolved resonant soft x-ray diffraction following excitation by an optical pump. Using orthogonal linear x-ray…
Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…
Photo-excitation in complex oxides1 transfers charge across semicovalent bonds, drastically perturbing spin and orbital orders2. Light may then be used in compounds like magnetoresistive manganites to control magnetism on nanometre…
In Mott insulators the evolution of antiferromagnetic order to superconducting or charge-density-wave-like states upon chemical doping underpins the control of quantum phases. Photo-doping can induce similar transitions on the ultrafast…
We demonstrate a new approach for directly measuring the ultrafast energy transfer between elec- trons and magnons, enabling us to track spin dynamics in an antiferromagnet (AFM). In multiferroic HoMnO3, optical photoexcitation creates hot…
In the mixed-valence manganites, a near-infrared laser typically melts the orbital and spin order simultaneously, corresponding to the photoinduced $d^{1}d^{0}$ $\xrightarrow{}$ $d^{0}d^{1}$ excitations in the Mott-Hubbard bands of…
Optical control of magnetism, of interest for high-speed data processing and storage, has only been demonstrated with near-infrared excitation to date. However, in absorbing materials, such high photon energies can lead to significant…
To elucidate different photoinduced melting dynamics of charge orders observed in quasi-two-dimensional organic conductors $ \theta $-(BEDT-TTF)$_2$RbZn(SCN)$_4$ and $ \alpha $-(BEDT-TTF)$_2$I$_3$…
Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…
We have carried out a first-principles theoretical study of the magnetically induced polarization in orthorhombic TbMnO3, a prototypical material in which a cycloidal spin structure generates an electric polarization via the spin-orbit…
Single-crystal synchrotron x-ray diffraction measurements in strong magnetic fields have been performed for magnetoelectric compounds GdMnO3 and TbMnO3. It has been found that the P || a ferroelectric phase induced by the application of a…
We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…
The effects associated with exciton Bose condensate formation in strongly correlated spin crossover systems are considered within the effective Hamiltonian obtained from the two-orbital Hubbard-Kanamori model. The collective excitations…
The magnetic properties of the layered oxypnictide LaMnAsO have been revisited using neutron scattering and magnetization measurements. The present measurements identify the N\'{e}el temperature $T_N$ = 360(1) K. Below $T_N$ the critical…
The ultrafast manipulation of magnetic order due to optical excitation is governed by the intricate flow of energy and momentum between the electron, lattice and spin subsystems. While various models are commonly employed to describe these…
Ordered electronic phases are intimately related to emerging phenomena such as high Tc superconductivity and colossal magnetoresistance. The coupling of electronic charge with other degrees of freedom such as lattice and spin are of central…
We propose an experimental setup of ultracold fermions in an optical lattice to determine the pairing gap in a superfluid state and the spin ordering in a Mott-insulating state. The idea is to apply a periodic modulation of the lattice…
We have uncovered a giant gyrotropic magneto-optical response for doped ferromagnetic manganite La2/3Ca1/3MnO3 around the near room-temperature paramagnetic-to-ferromagnetic transition. At odds with current wisdom, where this response is…
Research efforts on the low temperature magnetic order and electronic properties of U$_3$O$_8$ have been inconclusive so far. Reinterpreting neutron scattering results, we use group representation theory to show that the ground state…