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XUV and X-ray Free Electron Lasers (FELs) produce short wavelength pulses with high intensity, ultrashort duration, well-defined polarization and transverse coherence, and have been utilised for many experiments previously possible at long…

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the…

原子物理 · 物理学 2016-05-30 Paul Hockett , Matthias Wollenhaupt , Thomas Baumert

We demonstrate a left-right asymmetry control of the photo\-electron angular distribution in multi\-photon ionization of Li atoms by a bichromatic laser field. By delaying the fundamental (780 nm) and its second harmonic relative to each…

原子物理 · 物理学 2024-05-20 Silva Mezinska , Alexander Dorn , Thomas Pfeifer , Klaus Bartschat

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

化学物理 · 物理学 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

We consider the classical dynamics of a two-electron system subjected to an intense bichromatic linearly polarized laser pulse. By varying the parameters of the field, such as the phase lag and the relative amplitude between the two colors…

混沌动力学 · 物理学 2011-04-04 Adam Kamor , Francois Mauger , Cristel Chandre , Turgay Uzer

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

原子物理 · 物理学 2009-10-30 D. Bauer

We consider the ionization of neon induced by a femtosecond laser pulse composed of overlapping, linearly polarized bichromatic extreme ultraviolet and infrared fields. In particular, we study the effects of the infrared light on a…

原子物理 · 物理学 2017-01-25 Nicolas Douguet , Alexei N. Grum-Grzhimailo , Klaus Bartschat

We consider the role of quantum mechanics in a specific coherent control scenario, designing a "coherent control interferometer" as the essential tool that links coherent control to quantum fundamentals. Building upon this allows us to…

量子物理 · 物理学 2014-11-27 Torsten Scholak , Paul Brumer

The phonon-induced dephasing dynamics in optically excited semiconductor quantum dots is studied within the frameworks of the independent Boson model and optimal control. We show that appropriate tailoring of laser pulses allows a complete…

介观与纳米尺度物理 · 物理学 2009-11-10 Ulrich Hohenester , Georg Stadler

We propose an extension of coherent control using laser-synthesized free-electron matter waves. In contrast to coherent control schemes exploiting optical coherences to steer the dynamics of matter waves, we analyze the opposite and…

量子物理 · 物理学 2021-04-21 R. Esteban Goetz , Klaus Bartschat

Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

原子物理 · 物理学 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…

原子物理 · 物理学 2009-11-10 C. Figueira de Morisson Faria , X. Liu , A. Sanpera , M. Lewenstein

We describe numerically the ionization process induced by linearly and circularly polarized XUV attosecond laser pulses on an aligned atomic target, specifically, the excited state…

原子物理 · 物理学 2021-05-26 Juan J. Omiste , Lars Bojer Madsen

Single photon laser enabled Auger decay (spLEAD) has been redicted theoretically [Phys. Rev. Lett. 111, 083004 (2013)] and here we report its first experimental observation in neon. Using coherent, bichromatic free-electron laser pulses, we…

Coherent optical control schemes exploit the coherence of laser pulses to change the phases of interfering dynamical pathways in order to manipulate dynamical processes. These active control methods are closely related to dynamical…

其他凝聚态物理 · 物理学 2015-05-18 Luis G. C. Rego , L. F. Santos , V. S. Batista

We study phonon-assisted dephasing in optically excited semiconductor quantum dots within the frameworks of the independent Boson model and optimal control. Using a realistic description for the quantum dot states and the phonon coupling,…

介观与纳米尺度物理 · 物理学 2009-11-13 Ulrich Hohenester

We describe optimized coherent control methods for two-photon transitions in atoms of a ladder-type three-state energy configuration. Our approach is based on the spatial coherent control scheme which utilizes counter-propagating ultrashort…

原子物理 · 物理学 2015-10-28 Woojun Lee , Hyosub Kim , Kyungtae Kim , Jaewook Ahn
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