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The properties of the electronic ground state of the polar and paramagnetic chromium--closed-shell-atom molecules have been investigated. State-of-the-art \textit{ab initio} techniques have been applied to compute the potential energy…

原子物理 · 物理学 2013-07-31 Michał Tomza

An increasing number of Yb-based compounds fulfill the conditions for the investigation of hyperfine electro-nuclear coupling effects related to 171-Yb and 173-Yb isotopes. Among them, the lack of magnetic order down to the milikelvin range…

强关联电子 · 物理学 2025-06-24 S. Gabani , I. Curlik , F. Akbar , M. Giovannini , J. G. Sereni

Molecular spin qubits with long spin coherence time as well as non-invasive operation methods on such qubits are in high demand. It was shown that both molecular electronic and nuclear spin levels can be used as qubits. In solid state…

材料科学 · 物理学 2020-10-28 Robert L. Smith , Aleksander L. Wysocki , Kyungwha Park

Measuring the hyperfine structure (HFS) of long-lived $^3P_2$ states of divalent atoms may offer the opportunity of extracting relatively unexplored nuclear magnetic octupole and electric hexadecapole moments. Here, using relativistic…

原子物理 · 物理学 2009-11-13 K. Beloy , A. Derevianko , W. R. Johnson

Fermionic alkaline-earth atoms have unique properties that make them attractive candidates for the realization of novel atomic clocks and degenerate quantum gases. At the same time, they are attracting considerable theoretical attention in…

量子气体 · 物理学 2010-04-20 A. V. Gorshkov , M. Hermele , V. Gurarie , C. Xu , P. S. Julienne , J. Ye , P. Zoller , E. Demler , M. D. Lukin , A. M. Rey

In this article we extend the theory of ultra-long-range giant dipole molecules, formed by an atom in a giant dipole state and a ground-state alkali atom, by angular-momentum couplings known from recent works on Rydberg molecules. In…

原子物理 · 物理学 2018-02-14 Thomas Stielow , Stefan Scheel , Markus Kurz

We show how to exploit the rich hyperfine structure of fermionic alkali atoms to produce a quasi-1D topological superfluid while avoiding excessive heating from off-resonant scattering. We model interacting fermions where four hyperfine…

量子气体 · 物理学 2014-01-31 Junjun Xu , Qiang Gu , Erich J. Mueller

The theory is developed for one and two atom interactions when the atom has a Rydberg electron attached to a hyperfine split core state. This situation is relevant for some of the rare earth and alkaline earth atoms that have been proposed…

原子物理 · 物理学 2018-02-21 F. Robicheaux , D. W. Booth , M. Saffman

The heavy fermion metal \beta-YbAlB4 exhibits a bulk room temperature conduction electron ESR signal which evolves into an Ising-anisotropic f-electron signal exhibiting hyperfine features at low temperatures. We develop a theory for this…

强关联电子 · 物理学 2014-03-20 Aline Ramires , Piers Coleman

The spectroscopic hyperfine constants for all the alkali atoms are reported. For atoms from lithium to cesium, only the long lived atomic isotopes are examined. For francium, the measured data for nuclear ground states of all available…

原子物理 · 物理学 2024-06-19 M. Allegrini , E. Arimondo , L. A. Orozco

A relativistic wave equation for bound states of two fermions with arbitrary masses which are exposed to a magnetic field is derived from quantum electrodynamics. The interaction kernels are based upon the generalized invariant M-matrices…

高能物理 - 唯象学 · 物理学 2007-05-23 Andrei G. Terekidi , Jurij W. Darewych , Marko Horbatsch

Ultracold molecules have experienced increasing attention in recent years. Compared to ultracold atoms, they possess several unique properties that make them perfect candidates for the implementation of new quantum-technological…

量子气体 · 物理学 2019-02-20 G. Cappellini , L. F. Livi , L. Franchi , D. Tusi , D. Benedicto Orenes , M. Inguscio , J. Catani , L. Fallani

We investigate theoretically radio-frequency spectroscopy of weakly bound molecules in an ultracold spin-orbit-coupled atomic Fermi gas. We consider two cases with either equal Rashba and Dresselhaus coupling or pure Rashba coupling. The…

量子气体 · 物理学 2013-02-04 Hui Hu , Han Pu , Jing Zhang , Shi-Guo Peng , Xia-Ji Liu

We describe the theoretical advances that influenced the experimental creation of vibrationally and translationally cold polar $^{40}$K$^{87}$Rb molecules \cite{nphys08,science08}. Cold molecules were created from very-weakly bound…

量子物理 · 物理学 2015-05-13 Svetlana Kotochigova , Eite Tiesinga , Paul S. Julienne

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

原子物理 · 物理学 2021-02-16 Michał Śmiałkowski , Michał Tomza

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

介观与纳米尺度物理 · 物理学 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

We present the python package DiPolMol-Py, which can be used to calculate the rotational and hyperfine structure of $^2\Sigma$ molecules. The calculations can be performed in the presence of dc magnetic fields, dc electric fields and far…

原子物理 · 物理学 2025-09-01 Bethan Humphreys , Alex J. Matthies , Hannah J. Williams

State-of-the-art {\em ab initio} techniques have been applied to compute the potential energy curves for the SrYb molecule in the Born-Oppenheimer approximation for the ground state and first fifteen excited singlet and triplet states…

We present a rigorous quantum scattering study of the effects of hyperfine and Zeeman interactions on cold Li - H$_{2}$ collisions in the presence of an external magnetic field using a recent ab initio potential energy surface. We find that…

化学物理 · 物理学 2024-03-06 Hubert Jóźwiak , Timur V. Tscherbul , Piotr Wcisło

The collective dipole mode is induced and measured in a spin-orbit (SO) coupled degenerate Fermi gas of $^{173}$Yb atoms. Using a differential optical Stark shift, we split the degeneracy of three hyperfine states in the ground manifold,…

量子气体 · 物理学 2018-11-27 Shanchao Zhang , Chengdong He , Elnur Hajiyev , Zejian Ren , Bo Song , Gyu-Boong Jo