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We present a theoretical model for the experimentally found but counter-intuitive exceptionally long lifetime of surface nanobubbles. We can explain why, under normal experimental conditions, surface nanobubbles are stable for many hours or…

流体动力学 · 物理学 2015-06-11 Joost H. Weijs , Detlef Lohse

The stability and growth or dissolution of a single surface nanobubble on a chemically patterned surface are studied by Molecular Dynamics (MD) simulations of binary mixtures consisting of Lennard-Jones (LJ) particles. Our simulations…

流体动力学 · 物理学 2017-07-14 Shantanu Maheshwari , Martin van der Hoef , Xuehua Zhang , Detlef Lohse

Recent experiments have convincingly demonstrated the existence of surface nanobubbles on submerged hydrophobic surfaces. However, classical theory dictates that small gaseous bubbles quickly dissolve because their large Laplace pressure…

流体动力学 · 物理学 2009-11-13 Michael P. Brenner , Detlef Lohse

While growth and dissolution of surface nanobubbles has been widely studied in recent years, their stability under pressure changes or a temperature increase has not received the same level of scrutiny. Here, we present theoretical…

软凝聚态物质 · 物理学 2020-07-10 Yawei Liu , Stefano Bernardi , Asaph Widmer-Cooper

Experiments have not only revealed the remarkably long lifetime of nanobubbles, but also demonstrated the diffusive instability of bubbles above micrometers, thus a full-scale physical understanding on the stability of bubbles is in urgent…

软凝聚态物质 · 物理学 2021-12-28 Binghai Wen , Yongcai Pan , Lijuan Zhang , Shuo Wang , Limin Zhou , Chunlei Wang , Jun Hu

Surface nanobubbles are stable gaseous phases in liquids that form on solid substrates. While their existence has been confirmed, there are many open questions related to their formation and dissolution processes along with their structures…

流体动力学 · 物理学 2022-04-20 Zhizhao Che , Panagiotis E. Theodorakis

Surface nanobubbles (NBs) are stable gaseous phases in liquids that form at the interface with solid substrates. They have been particularly intriguing for their high stability that contradicts theoretical expectations and their potential…

软凝聚态物质 · 物理学 2019-09-09 Panagiotis E. Theodorakis , Zhizhao Che

Surface nanobubbles are nanoscopic spherical-cap shaped gaseous domains on immersed substrates which are stable, even for days. After the stability of a {\it single} surface nanobubble has been theoretically explained, i.e. contact line…

流体动力学 · 物理学 2020-02-06 Xiaojue Zhu , Roberto Verzicco , Xuehua Zhang , Detlef Lohse

Shock wave induced cavitation experiments and atomic force microscopy measurements of flat polyamide and hydrophobized silicon surfaces immersed in water are performed. It is shown that surface nanobubbles, present on these surfaces, do not…

流体动力学 · 物理学 2009-11-13 Bram M. Borkent , Stephan M. Dammer , Holger Schoenherr , G. Julius Vancso , Detlef Lohse

It has been recently shown that nanobubbles exhibit a remarkable and unexpected stability. The lifetime of nanobubbles, formed either within liquids or on hydrophobic surfaces, can exceed by more than 10 orders of magnitude the theoretical…

软凝聚态物质 · 物理学 2019-05-14 Caroline Desgranges , Jerome Delhommelle

Surface nanobubbles are complex micro- and nanoscale fluid systems. While thermodynamics is believed to dominate nanobubble dynamics, the precise mechanism by which nanobubble evolution is driven by thermodynamics remains unclear. It is…

软凝聚态物质 · 物理学 2025-02-06 Lili Lan , Yongcai Pan , Liang Zhao , Binghai Wen

A model for gas nanobubbles is proposed in which their remarkable stability is explained as due to the presence of a qualitatively different form of water covering the nanobubble surface layer which leads to a reduction of the diffusion…

介观与纳米尺度物理 · 物理学 2014-10-15 Siddhartha Sen , Kumar S. Gupta

We study surface nanobubbles using molecular dynamics simulation of ternary (gas, liquid, solid) systems of Lennard-Jones fluids. They form for sufficiently low gas solubility in the liquid, i.e., for large relative gas concentration. For…

流体动力学 · 物理学 2012-11-19 J. H. Weijs , J. H. Snoeijer , D. Lohse

The observed stability of nanobubbles contradicts the well-known result in classical nucleation theory, that the critical radius is both microscopic and thermodynamically unstable. Here nanoscopic stability is shown to be the combined…

化学物理 · 物理学 2015-03-17 Phil Attard

When a film of a liquid suspension of nanoparticles or a polymer solution is deposited on a surface, it may dewet from the surface and as the solvent evaporates the solute particles/polymer can be deposited on the surface in regular line…

软凝聚态物质 · 物理学 2013-03-25 Lubor Frastia , Andrew J. Archer , Uwe Thiele

Previous experiments have shown that spherical colloidal particles relax to equilibrium slowly after they adsorb to a liquid-liquid interface, despite the large interfacial energy gradient driving the adsorption. The slow relaxation has…

软凝聚态物质 · 物理学 2016-11-08 Anna Wang , Ryan McGorty , David M. Kaz , Vinothan N. Manoharan

The formation and evolution of immersed surface micro- and nanobubbles are essential in various practical applications, such as the usage of superhydrophobic rematerials, drug delivery, and mineral flotation. In this work, we investigate…

Pinning of liquid droplets on solid substrates is ubiquitous and plays an essential role in many applications, especially in various areas, such as microfluidics and biology. Although pinning can often reduce the efficiency of various…

流体动力学 · 物理学 2023-11-28 Panagiotis E. Theodorakis , Alidad Amirfazli , Bin Hu , Zhizhao Che

The primary attribute of interest of surface nanobubbles is their unusual stability and a number of theories trying to explain this have been put forward. Interestingly, the dissolution of nanobubbles is a topic that did not receive a lot…

Using molecular dynamics, we study the nucleation and stability of bulk nanobubble clusters. We study the formation, growth, and final size of bulk nanobubbles. We find that, as long as the bubble-bubble interspacing is small enough, bulk…

流体动力学 · 物理学 2012-11-19 Joost H. Weijs , James R. T. Seddon , D. Lohse
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