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Ultrafast responses of BCS superconductor Nb1-xTixN films in a nonadiabatic excitation regime were investigated by using terahertz (THz) pump-THz probe spectroscopy. After an instantaneous excitation with the monocycle THz pump pulse, a…

The recent observation of a transmitted Thz pulse oscillating at three times the frequency of the incident light paves the way to a new protocol to access resonant excitations in a superconductor. Here we show that this non-linear optical…

超导电性 · 物理学 2016-06-01 T. Cea , C. Castellani , L. Benfatto

We study the nonlinear optical response in a superconducting NbN thin film with strong terahertz (THz)wave. Besides the expected third harmonic generation, we observe a new transient oscillation which softensin frequency with temperature…

超导电性 · 物理学 2022-03-30 Z. X. Wang , J. R. Xue , H. K. Shi , X. Q. Jia , T. Lin , L. Y. Shi , T. Dong , F. Wang , N. L. Wang

Recent advances in time-domain terahertz (THz) spectroscopy have unveiled that resonantly-enhanced strong THz third-harmonic generation (THG) mediated by the collective Higgs amplitude mode occurs in s-wave superconductors, where…

超导电性 · 物理学 2017-07-26 Ryusuke Matsunaga , Naoto Tsuji , Kazumasa Makise , Hirotaka Terai , Hideo Aoki , Ryo Shimano

2H-NbSe2 is an archetypal system in which superconductivity and charge-density-wave (CDW) coexist and compete macroscopically with each other. In particular, this interplay also manifests in their dynamical fluctuations. As a result, the…

Recent developments in nonequilibrium and nonlinear terahertz (THz) spectroscopies have significantly advanced our understanding of collective excitations in superconductors. However, there is still debate surrounding the identification of…

超导电性 · 物理学 2024-12-19 Jiayu Yuan , Liyu Shi , Tiequan Xu , Yue Wang , Zizhao Gan , Hao Wang , Tianyi Wu , Dong Wu , Tao Dong , Nanlin Wang

Higgs mode in superconductors, i.e. the collective amplitude mode of the order parameter does not associate with charge nor spin fluctuations, therefore it does not couple to the electromagnetic field in the linear response regime. On the…

超导电性 · 物理学 2019-07-02 Sachiko Nakamura , Yudai Iida , Yuta Murotani , Ryusuke Matsunaga , Hirotaka Terai , Ryo Shimano

The dynamics of Higgs mode in superconductors, manifested as coherent oscillations of the superconducting order parameter amplitude, provides vital insights into the nature of the superconducting gap structure and symmetry. Here we utilize…

Recently developed terahertz (THz) two-dimensional coherent spectroscopy (2DCS) is a powerful technique to obtain materials information in a fashion qualitatively different from other spectroscopies. Here, we utilized THz 2DCS to…

Ultrafast optical control of quantum systems is an emerging field of physics. In particular, the possibility of light-driven superconductivity with ultrashort laser pulses has attracted much of attention. To identify non-equilibrium…

We reveal that due to the presence of disorder oscillations of the order parameter amplitude called the Higgs mode can be effectively excited by the external electromagnetic radiation in usual BCS superconductors. This mechanism works for…

超导电性 · 物理学 2019-06-26 Mikhail Silaev

Recent experiments with strong THz fields in unconventional cuprates superconductors have clearly evidenced an increase of the non-linear optical response below the superconducting critical temperature Tc. As in the case of conventional…

超导电性 · 物理学 2023-06-21 Mattia Udina , Jacopo Fiore , Tommaso Cea , Claudio Castellani , Goetz Seibold , Lara Benfatto

When a continuous symmetry of a physical system is spontaneously broken, two types of collective modes typically emerge: the amplitude and phase modes of the order-parameter fluctuation. For superconductors, the amplitude mode is recently…

超导电性 · 物理学 2020-03-19 Ryo Shimano , Naoto Tsuji

In superconductors the Anderson-Higgs mechanism allows for the existence of a collective amplitude (Higgs) mode which can couple to eV-light mainly in a non-linear Raman-like process. The experimental non-equilibrium results on isotropic…

超导电性 · 物理学 2021-11-05 M. Puviani , A. Baum , S. Ono , Y. Ando , R. Hackl , D. Manske

We show that a non-quasiparticle charge collective mode, in parallel and coincident with the d-wave pair conductivity, leads to a quantitative understanding of microwave surface impedance measurements on superconducting…

超导电性 · 物理学 2009-10-31 S. Sridhar , Z. Zhai

A puzzling phenomenon has been recently revealed in terahertz nonlinear optical response experiments: A third harmonic generation (THG) signal, identified only in the superconducting (SC) phase in a conventional BCS superconductor, is found…

强关联电子 · 物理学 2026-02-11 Xiang Li , Zheng-Yu Weng

By applying a microscopic gauge-invariant kinetic theory in $d$-wave superconductors, we analytically derive the energy spectra of the breathing Higgs mode and, in particular, rotating Higgs mode that is unique for the $d$-wave order…

超导电性 · 物理学 2020-07-27 F. Yang , M. W. Wu

We investigate the iron-based superconductor Ba$_{1-x}$K$_x$Fe$_2$As$_2$ using intense terahertz (THz) light. In the superconducting state a THz Kerr signal is observed and assigned to non-linear THz coupling to superconducting degrees of…

超导电性 · 物理学 2022-01-19 Romain Grasset , Kota Katsumi , Pierre Massat , Hai-Hu Wen , Xian-Hui Chen , Yann Gallais , Ryo Shimano

We report experimental evidences for the observation of the superconducting amplitude mode, so-called `Higgs' mode in the charge density wave superconductor 2H-NbSe2 using Raman scattering. By comparing 2H-NbSe2 and its iso-structural…

超导电性 · 物理学 2015-06-18 M. -A. Méasson , Y. Gallais , M. Cazayous , B. Clair , P. Rodière , L. Cario , A. Sacuto

Detection of the Higgs mode in superconductors using nonlinear terahertz spectroscopy is a key area of interest in condensed matter physics. We investigate the influence of disorder on the nonlinear terahertz response and the Higgs mode in…

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