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The transport of fluids at the nanoscale is fundamental to manifold biological and industrial processes, ranging from neurotransmission to ultrafiltration. Yet, it is only recently that well-controlled channels with cross-sections as small…

介观与纳米尺度物理 · 物理学 2022-10-05 Nikita Kavokine , Paul Robin , Lydéric Bocquet

Lithium-ion transport is significantly retarded in ionic liquids (ILs). In this work, we performed extensive molecular dynamics (MD) simulations to mimic the kinetics of lithium ions in ILs using [\emph{N}-methyl-\emph{N}-propylpyrrolidium…

计算物理 · 物理学 2023-09-19 YeongKyu Lee , JunBeom Cho , Junseong Kim , Won Bo Lee , YongSeok Jho

Ionic Coulomb blockade in nanopores is a phenomenon that shares some similarities but also differences with its electronic counterpart. Here, we investigate extensively this phenomenon using all-atom molecular dynamics of ionic transport…

介观与纳米尺度物理 · 物理学 2017-12-27 Hiroya Tanaka , Hideo Iizuka , Yuriy V. Pershin , Massimiliano Di Ventra

We present a theoretical study of the influence of the molecular geometry of the cation on the response of ionic liquid (IL) to confinement and mechanical strain. The so-called {\it tailed} model includes a large spherical anion and…

软凝聚态物质 · 物理学 2019-03-27 Miljan Dašić , Igor Stanković , Konstantinos Gkagkas

Ionic microgel particles are intriguing systems in which the properties of thermo-responsive polymeric colloids are enriched by the presence of charged groups. In order to rationalize their properties and predict the behaviour of microgel…

软凝聚态物质 · 物理学 2021-01-28 G. Del Monte , F. Camerin , A. Ninarello , N. Gnan , L. Rovigatti , E. Zaccarelli

Ionic gating is a very popular tool to investigate and control the electric charge transport and electronic ground state in a wide variety of different materials. This is due to its capability to induce large modulations of the surface…

超导电性 · 物理学 2021-05-27 Erik Piatti

Three-terminal electrochemical ionic synapses (EIoS) have recently attracted interest for in-memory computing applications. These devices utilize electrochemical ion intercalation to modulate the ion concentration in the channel material.…

介观与纳米尺度物理 · 物理学 2025-08-01 Michael L. Li , Dingyu Shen , Jesus A. del Alamo , Martin Z. Bazant

Many plastic crystals, molecular solids with long-range, center-of-mass crystalline order but dynamic disorder of the molecular orientations, are known to exhibit exceptionally high ionic conductivity. This makes them promising candidates…

无序系统与神经网络 · 物理学 2019-06-28 D. Reuter , P. Lunkenheimer , A. Loidl

Room Temperature Ionic Liquids (RTILs) have attracted much of the attention of the scientific community in the past decade due the their novel and highly customizable properties. Nonetheless their high viscosities pose serious limitations…

化学物理 · 物理学 2012-08-09 Oliviero Andreussi , Nicola Marzari

We investigate correlation physics in high-density, two-dimensional electron liquids that reside in narrow SrTiO3 quantum wells. The quantum wells are remotely doped via an interfacial polar discontinuity and the three-dimensional (3D)…

强关联电子 · 物理学 2013-11-26 Pouya Moetakef , Clayton A. Jackson , Jinwoo Hwang , Leon Balents , S. James Allen , Susanne Stemmer

Recent experiments measuring the electrical conductivity of DNA molecules highlight the need for a theoretical model of ion transport along a charged surface. Here we present a simple theory based on the idea of unbinding of ion pairs. The…

软凝聚态物质 · 物理学 2009-10-23 Brian Skinner , M. S. Loth , B. I. Shklovskii

Humid hydrophobic ionic liquids, widely used as electrolytes, have narrowed electrochemical windows, because their water, absorbed on the electrode surface, gets involved in electrolysis. In this work, we performed molecular dynamics…

应用物理 · 物理学 2020-12-02 Ming Chen , Jiedu Wu , Ting Ye , Jinyu Ye , Sheng Bi , Jiawei Yan , Bingwei Mao , Guang Feng

We investigate the mobility of nanometer-size solutes in water in a uniform external electric field. General arguments are presented to show that a closed surface cutting a volume from a polar liquid will carry an effective non-zero surface…

软凝聚态物质 · 物理学 2016-08-24 Mohammadhasan Dinpajooh , Dmitry V. Matyushov

The self-assembly mechanism of one-end-open carbon nanotubes (CNTs) suspended in an aqueous solution was studied by molecular dynamics simulations. It was shown that two one-end-open CNTs with different diameters can coaxially self-assemble…

介观与纳米尺度物理 · 物理学 2017-07-31 Hang Xiao , Xiaoyang Shi , Xi Chen

We present porous electrode theory for capacitive deionization (CDI) with electrodes containing nanoparticles that consist of a redox-active intercalation material. A geometry of a desalination cell is considered which consists of two…

化学物理 · 物理学 2019-12-24 K. Singh , H. J. M. Bouwmeester , L. C. P. M de Smet , M. Z. Bazant , P. M. Biesheuvel

Networks of ligand-free semiconductor nanocrystals (NCs) offer a valuable combination of high carrier mobility and optoelectronic properties tunable via quantum confinement. In principle, maximizing carrier mobility entails crossing the…

Nanoporous carbon-based supercapacitors store electricity through adsorption of ions from the electrolyte at the surface of the electrodes. Room temperature ionic liquids, which show the largest ion concentrations among organic liquid…

Ionic liquid ion sources are a promising technology that can be used for many applications from space propulsion to focused ion beam microetching. Ionic liquid ion sources produce ion beams by extracting single ions and metastable solvated…

化学物理 · 物理学 2021-11-17 Madeleine Schroeder

Due to the coexistence of many emergent phenomena, including 2D superconductivity and a large Rashba spin-orbit coupling, 5d transition metal oxides based two-dimensional electron systems (2DESs) have been prospected as one of the potential…

材料科学 · 物理学 2022-10-24 H. Yan , S. W. Zeng , K. Rubi , G. J. Omar , Z. T. Zhang , M. Goiran , W. Escoffier , A. Ariando

We study charge transport in an ionic solution in a confined nanoscale geometry in the presence of an externally applied electric field and immobile background charges. For a range of parameters, the ion current shows non-monotonic behavior…

统计力学 · 物理学 2015-05-13 Punyabrata Pradhan , Yariv Kafri , Dov Levine