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Exciton-polaritons in semiconductors are quasi-particles which have recently shown the capability to undergo phase transition into a coherent hybrid state of light and matter. The observation of such quasi-particles in organic microcavities…

Exciton-plasmon polaritons (EPPs) are attractive both for the exploration of fundamental phenomena and applications in nanophotonics. Previous studies of EPPs mainly relied on far-field characterization. Here, using near-field optical…

We investigate the strong coupling between the excitons and quasi-bound states in the continuum (BIC) resonance in a bulk WS$_2$ metasurface. Here we employ the bulk WS$_2$ to construct an ultrathin nanodisk metasurface, supporting the…

Room temperature strong coupling of WS_2 monolayer exciton transitions to metallic Fabry-Perot and plasmonic optical cavities is demonstrated. A Rabi splitting of 101 meV is observed for the Fabry-Perot cavity, more than double those…

材料科学 · 物理学 2016-08-24 S. Wang , S. Li , T. Chervy , A. Shalabney , S. Azzini , E. Orgiu , J. A. Hutchison , C. Genet , P. Samori , T. W. Ebbesen

We study a doped transition metal dichalcogenide (TMDC) monolayer in an optical microcavity. Using the microscopic theory, we simulate spectra of quasiparticles emerging due to the interaction of material excitations and a high-finesse…

材料科学 · 物理学 2024-07-23 Y. V. Zhumagulov , S. Chiavazzo , D. R. Gulevich , V. Perebeinos , I. A. Shelykh , O. Kyriienko

Polariton-based devices require materials where light-matter coupling under ambient conditions exceeds losses, but our current selection of such materials is limited. Here we measured the dispersion of polaritons formed by the $A$ and $B$…

材料科学 · 物理学 2021-06-16 Patryk Kusch , Niclas S. Mueller , Martin T. Hartmann , Stephanie Reich

Exciton polaritons based on atomically thin semiconductors are essential building blocks of quantum optoelectronic devices. Their properties are governed by an ultrafast and oscillatory energy transfer between their excitonic and photonic…

We demonstrate strong light-matter interaction at ambient conditions between a ladder-type conjugated polymer and the individual modes of a vertical microcavity with tunable resonance frequencies. Zero-dimensional wavelength-scale…

介观与纳米尺度物理 · 物理学 2019-01-28 Darius Urbonas , Thilo Stöferle , Fabio Scafirimuto , Ullrich Scherf , Rainer F. Mahrt

The work is devoted to the investigation of the surface plasmon polaritons in the metal - dielectric heterostructures containing materials with magnetoelectric properties. The analysis of various possible configurations shows that the…

Strong exciton-plasmon interaction between the layered two-dimensional (2D) semiconductors and gap plasmons shows a great potential to implement cavity quantum-electrodynamics in ambient condition. However, achieving a robust…

We study theoretically optical response of WS2 monolayer located near periodic metal nanostructured arrays in two and three dimensions. The emphasis of simulations is on the strong coupling regime of excitons supported by WS2 and surface…

介观与纳米尺度物理 · 物理学 2018-04-04 Maxim Sukharev , Ruth Pachter

Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of…

Polaritons can provide strong optical field enhancement allowing to boost light-matter interaction. Here, we experimentally observe enhancement of mid-infrared second-harmonic generation (SHG) using grating-coupled surface phonon polaritons…

Moire lattices attract significant attention in double-layer graphene and TMD layer heterostructures as well as in photonic crystals due to the interesting exotic physics that emerges within these structures. However, direct measurement of…

Two-dimensional transition metal di-chalcogenide semiconductors provide unique possibilities to investigate strongly confined excitonic physics and a plasmonic platform integrable to such materials constitutes a hybrid system that can be of…

介观与纳米尺度物理 · 物理学 2022-05-26 Bidisha Roy , Maex Blauth , Siddharth Dhomkar , Michael Kaniber , Vinod M. Menon , Jonathan. J. Finley

Strong-coupling of monolayer metal dichalcogenide semiconductors with light offers encouraging prospects for realistic exciton devices at room temperature. However, the nature of this coupling depends extremely sensitively on the optical…

The possibility of creating heterostructure of two-dimensional (2D) materials has emerged as a viable route towards realizing novel optoelectronic devices. However, the low light absorption due to their small absorption cross section,…

介观与纳米尺度物理 · 物理学 2023-03-14 Shubhrasish Mukherjee , Didhiti Bhattacharya , Samit Kumar Ray , Atindra Nath Pal

The goal of nanophotonics is to control and manipulate light at length scales below the diffraction limit. Typically nanostructured metals are used for this purpose, light being confined by exploiting the surface plasmon-polaritons such…

介观与纳米尺度物理 · 物理学 2017-05-24 Martin J. Gentile , William L. Barnes

We consider the scenario of excitons in a semiconductor bilayer that are strongly coupled to cavity photons, leading to the formation of dipolar exciton polaritons (dipolaritons). Using a realistic pseudopotential for the dipolar…

介观与纳米尺度物理 · 物理学 2026-02-27 Yasufumi Nakano , Olivier Bleu , Brendan C. Mulkerin , Jesper Levinsen , Meera M. Parish

Light-matter interactions at the nanoscale constitute a fundamental ingredient for engineering applications in nanophotonics and quantum optics. To this regard electromagnetic Mie resonances excited in high-refractive index dielectric…