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We introduce two-color counterrotating circularly polarized laser fields as a new way to spectrally control high harmonic generation (HHG) from relativistic plasma mirrors. Through particle-in-cell simulations, we show that only a selected…

等离子体物理 · 物理学 2018-04-13 Zi-Yu Chen

Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…

原子物理 · 物理学 2008-04-04 Toru Morishita , Anh-Thu Le , Zhangjin Chen , C. D. Lin

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

原子物理 · 物理学 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

光学 · 物理学 2017-07-12 F. Risoud , C. Lévêque , M. Labeye , J. Caillat , A. Maquet , P. Salières , R. Taïeb , T. Shaaran

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…

原子物理 · 物理学 2014-02-06 Francois Mauger , A. D. Bandrauk , Adam Kamor , Turgay Uzer , Cristel Chandre

High-order harmonic generation is a powerful and sensitive tool for probing atomic and molecular structures, combining in the same measurement an unprecedented attosecond temporal resolution with a high spatial resolution, of the order of…

化学物理 · 物理学 2015-06-23 M. Negro , M. Devetta , D. Faccialà , S. De Silvestri , C. Vozzi , S. Stagira

Phase-of-the-phase (PoP) spectroscopy is extended to two-color laser fields having a circularly counter-rotating polarization. In particular, the higher harmonics of the (two-color) phase information are analyzed in order to extract the…

原子物理 · 物理学 2020-04-22 V. A. Tulsky , B. Krebs , J. Tiggesbäumker , D. Bauer

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

原子物理 · 物理学 2009-11-07 F. Ceccherini , D. Bauer

We develop theoretically and confirm both numerically and experimentally a comprehensive analytical model which describes the propensity rules in the emission of circularly polarized high harmonics by systems driven by two-color…

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

原子物理 · 物理学 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

Spectra of circularly polarized harmonics is calculated by numerically solving the Time-Dependent Schr\"{o}dinger Equation for a 2D model of Ne atom using circularly polarized fundamental with counter-rotating second harmonic laser fields.…

原子物理 · 物理学 2015-10-28 Lukas Medišauskas , Jack Wragg , Hugo van der Haart , Misha Yu. Ivanov

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

High harmonic generation by relativistically intense laser pulses from overdense plasma layers is surveyed. High harmonics are generated in form of (sub-)attosecond pulses when the plasma surface rebounds towards the observer with…

等离子体物理 · 物理学 2011-11-18 Daniel an der Brügge , Alexander Pukhov

We exploit a slightly noncollinear second-harmonic cross-correlation scheme to map the 3D space-time intensity distribution of an unknown complex-shaped ultrashort optical pulse. We show the capability of the technique to reconstruct both…

The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in…

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

原子物理 · 物理学 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti
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