相关论文: Nonlinear Phononic Control and Emergent Magnetism …
Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…
We employ time-resolved resonant x-ray diffraction to study the melting of charge order and the associated insulator-metal transition in the doped manganite Pr$_{0.5}$Ca$_{0.5}$MnO$_3$ after resonant excitation of a high-frequency…
Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…
Coherent manipulation of magnetism through the lattice provides unprecedented opportunities for controlling spintronic functionalities on the ultrafast timescale. Such nonthermal control conventionally involves nonlinear excitation of…
Femtosecond optical pulses at mid-infrared frequencies have opened up the nonlinear control of lattice vibrations in solids. So far, all applications have relied on second order phonon nonlinearities, which are dominant at field strengths…
We provide a theoretical demonstration of controllable non-relativistic spin splitting in both electronic and magnonic bands via targeted structural distortions tied to specific phonon modes. Using MnF$_2$ as a model system, we identify a…
Nonlinear phononics is the phenomenon in which a coherent dynamics in a material along a set of phonons is launched after its infrared-active phonons are selectively excited using external light pulses. The microscopic mechanism underlying…
Nonlinear phononics holds the promise for controlling properties of quantum materials on the ultrashort timescale. Using nonequilibrium dynamical mean-field theory, we solve a model for the description of organic solids, where correlated…
We present a microscopic theory for ultrafast control of solids with high-intensity terahertz frequency optical pulses. When resonant with selected infrared-active vibrations, these pulses transiently modify the crystal structure and lead…
Nonlinear phononics play important role in strong laser-solid interactions. We discuss nonlinear dynamical protocols which allow for efficient excitation and control of nonlinear phonons. We consider recent inspiring proposals: inducing…
Ultrafast optical control of ferroelectricity using intense terahertz fields has attracted significant interest. Here we show that the nonlinear interactions between two optical phonons in SnTe, a two-dimensional in-plane ferroelectric…
Epitaxial strain and chemical substitution have been the workhorses of functional materials design. These static techniques have shown immense success in controlling properties in complex oxides through the tuning of subtle structural…
Nonlinear interactions between phonon modes govern the behavior of vibrationally highly excited solids and molecules. Here, we demonstrate theoretically that optical cavities can be used to control the redistribution of energy from a highly…
To date, two types of coupling between electromagnetic radiation and a crystal lattice have been identified experimentally. One is direct, for infrared (IR)-active vibrations that carry an electric dipole. The second is indirect, it occurs…
Nonlinear phononics provides a route to control crystal structures through light-induced phonon excitation. In this study, we apply nonlinear phononics to an iron-based superconductor, LaFeAsO, with the aim of tuning its crystal structure…
The spin nematic phase, characterized by long-range order of spin quadrupole moments in the absence of dipolar magnetism, presents a significant challenge for conventional experimental detection. We propose a novel method to detect this…
Rare-earth titanates are Mott insulators whose magnetic ground state -- antiferromagnetic (AFM) or ferromagnetic (FM) -- can be tuned by the radius of the rare-earth element. Here, we combine phenomenology and first-principles calculations…
Light fields at THz and mid-infrared frequencies allow for the direct excitation of collective modes in condensed matter, which can be driven to large amplitudes. For example, excitation of the crystal lattice, has been shown to stimulate…
Breaking time-reversal symmetry in integrated photonics without magnetic fields remains a fundamental challenge. We demonstrate phonon-induced non-reciprocity through direct lifting of forward-backward mode degeneracy in microring…
Quantum control of phonons has being become a focus of attention for developing quantum technologies. Here, we propose a proposal to realize phonon blockade in a quadratically coupled optomechanical system, where a strong nonlinear…