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The theory of energy transfer dynamics of a pair of donor and acceptor molecules located in the plasmonic hot spots is developed by means of the master equation approach and the electromagnetic Green's tensor technique. A nonlocal effect…

光学 · 物理学 2017-12-29 Jun Ren , Tian Chen , Bo Wang , Xiangdong Zhang

We develop a mathematically rigorous theory for the quantum transfer processes in degenerate donor-acceptor dimers in contact with a thermal environment. We calculate explicitly the transfer rates and the acceptor population efficiency. The…

量子物理 · 物理学 2020-07-15 Marco Merkli , Gennady P. Berman , Avadh Saxena

The rapidly advancing capabilities in nanophotonic design are enabling complex functionalities limited mainly by physical bounds. The efficiency of transmission is a major consideration, but its ultimate limit remains unknown for most…

光学 · 物理学 2024-06-05 Shiyu Li , Chia Wei Hsu

We derive an efficiency bound for continuous quantum heat engines absorbing heat from squeezed thermal reservoirs. Our approach relies on a full-counting statistics description of nonequilibrium transport and it is not limited to the…

统计力学 · 物理学 2018-02-05 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

We investigate the role of quantum coherence in modulating the energy transfer rate between two independent energy donors and a single acceptor participating in an excitonic energy transfer process. The energy transfer rate depends…

化学物理 · 物理学 2015-07-13 Sreenath K. Manikandan , Anil Shaji

We study quantum transport through two-terminal nanoscale devices in contact with two particle reservoirs at different temperatures and chemical potentials. We discuss the general expressions controlling the electric charge current, heat…

介观与纳米尺度物理 · 物理学 2017-08-04 G. Bevilacqua , G. Grosso , G. Menichetti , G. Pastori Parravicini

Nanophotonics achieves accurate control over the luminescence properties of a single quantum emitter by tailoring the light-matter interaction at the nanoscale and modifying the local density of optical states (LDOS). This paradigm could…

We analytically derive the upper bound on the overall efficiency of single-photon generation based on cavity quantum electrodynamics (QED), where cavity internal loss is treated explicitly. The internal loss leads to a tradeoff relation…

量子物理 · 物理学 2019-06-05 Hayato Goto , Shota Mizukami , Yuuki Tokunaga , Takao Aoki

Machines are only Carnot efficient if they are reversible, but then their power output is vanishingly small. Here we ask, what is the maximum efficiency of an irreversible device with finite power output? We use a nonlinear scattering…

介观与纳米尺度物理 · 物理学 2014-04-23 Robert S. Whitney

Photon impingement is capable of liberating electrons in electronic devices and driving the electron flux from the lower chemical potential to higher chemical potential. Previous studies hinted that the thermodynamic efficiency of a…

量子物理 · 物理学 2016-05-11 Shan-He Su , Chang-Pu Sun , Sheng-Wen Li , Jin-Can Chen

Modern nanophotonic and meta-optical devices utilize a tremendous number of structural degrees of freedom to enhance light--matter interactions. A fundamental question is how large such enhancements can be. We develop an analytical…

光学 · 物理学 2020-11-13 Zeyu Kuang , Lang Zhang , Owen D. Miller

There is a remarkable characteristic of photosynthesis in nature, that is, the energy transfer efficiency is close to 100%. Recently, due to the rapid progress made in the experimental techniques, quantum coherent effects have been…

化学物理 · 物理学 2020-02-25 Ming-Jie Tao , Na-Na Zhang , Peng-Yu Wen , Fu-Guo Deng , Qing Ai , Gui-Lu Long

The wave-like nature of electrons leads to the existence of upper bounds on the thermoelectric response of nanostructured devices [R. S. Whitney, Phys. Rev. Lett. 112, 130601 (2014); Phys. Rev. B 91, 115425 (2015)]. This fundamental result,…

介观与纳米尺度物理 · 物理学 2022-08-24 Giuseppe Bevilacqua , Alessandro Cresti , Giuseppe Grosso , Guido Menichetti , Giuseppe Pastori Parravicini

A generic and intuitive model for coherent energy transport in multiple minima systems coupled to a quantum mechanical bath is shown. Using a simple spin-boson system, we illustrate how a generic donor-acceptor system can be brought into…

生物物理 · 物理学 2014-06-24 Tristan Farrow , Vlatko Vedral

We study a quantum thermal engine model for which the heat transfer law is determined by Einstein's theory of radiation. The working substance of the quantum engine is assumed to be a two-level quantum systems of which the constituent…

统计力学 · 物理学 2012-11-30 H. Yan , Hao Guo

The realization of robust coherent energy transfer with a long range from a donor to an acceptor has many important applications in the field of quantum optics. However, it is hard to be realized using conventional schemes. Here, we…

光学 · 物理学 2020-10-27 Yujing Wang , Jun Ren , Weixuan Zhang , Lu He , Xiangdong Zhang

We investigate the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems, mimicking a light-harvesting antenna connected to a reaction center as it is found in natural…

We consider the nonlinear scattering theory for three-terminal thermoelectric devices, used for power generation or refrigeration. Such systems are quantum phase-coherent versions of a thermocouple, and the theory applies to systems in…

介观与纳米尺度物理 · 物理学 2017-05-25 Robert S. Whitney

We present a first-principles calculation on the rate and efficiency of F\"orster resonance energy transfer (FRET) from a donor to an acceptor when they are located in the hotspots of nanoparticle clusters. Nonlocal effect has been…

光学 · 物理学 2017-12-29 Jun Ren , Tong Wu , Bing Yang , Xiangdong Zhang

A genuine feature of projective quantum measurements is that they inevitably alter the mean energy of the observed system if the measured quantity does not commute with the Hamiltonian. Compared to the classical case, Jacobs proved that…

统计力学 · 物理学 2015-06-10 Kay Brandner , Michael Bauer , Michael T. Schmid , Udo Seifert
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