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High-order harmonics generated by bicircular laser field have helicities which alternate between $+1$ and $-1$. In order to generate circularly polarized high-harmonic pulses, which are important for applications, it is necessary to achieve…

原子物理 · 物理学 2018-09-26 Dejan B. Milošević

High-order harmonic generation by a bicircular field, which consists of two coplanar counter-rotating circularly polarized fields of frequency $r\omega$ and $s\omega$ ($r$ and $s$ are integers), is investigated for a polyatomic molecule.…

原子物理 · 物理学 2016-10-05 Senad Odžak , Elvedin Hasović , Dejan B. Milošević

We employ a rotating frame of reference to elucidate high-harmonic generation of circularly polarized light by bicircular driving fields. In particular, we show how the experimentally observed circular components of the high-harmonic…

原子物理 · 物理学 2016-04-21 Daniel M. Reich , Lars Bojer Madsen

High-harmonic generation in two-colour ($\omega-2\omega$) counter-rotating circularly polarised laser fields opens the path to generate isolated attosecond pulses and attosecond pulse trains with controlled ellipticity. The generated…

We predict high-order harmonics in which the polarization within the spectral bandwidth of each harmonic varies continuously and significantly. For example, the interaction of counter-rotating circularly-polarized bichromatic drivers having…

光学 · 物理学 2014-10-24 Avner Fleischer , Ofer Kfir , Pavel Sidorenko , Oren Cohen

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…

原子物理 · 物理学 2014-02-06 Francois Mauger , A. D. Bandrauk , Adam Kamor , Turgay Uzer , Cristel Chandre

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

原子物理 · 物理学 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

We investigate the polarization properties of high harmonics generated with the bichromatic counterrotating circularly polarized (BCCP) laser fields by numerically solving time-dependent Schr\"odinger equation (TDSE). It is found that, the…

原子物理 · 物理学 2016-12-21 Xiaofan Zhang , Liang Li , Xiaosong Zhu , Xi Liu , Qingbin Zhang , Pengfei Lan , Peixiang Lu

The generation of high-order harmonics in a medium of chiral molecules driven by intense bi-elliptical laser fields can lead to strong chiroptical response in a broad range of harmonic numbers and ellipticities [D. Ayuso et al, J. Phys. B…

光学 · 物理学 2018-07-04 David Ayuso , Piero Decleva , Serguei Patchkovskii , Olga Smirnova

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

原子物理 · 物理学 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

Generation of circularly-polarized high-harmonics with the same helicity to all orders is indispensable for chiral-sensitive spectroscopy with attosecond temporal resolution. Solid-state samples have added a valuable asset in controlling…

光学 · 物理学 2023-06-06 Navdeep Rana , M. S. Mrudul , Gopal Dixit

We introduce two-color counterrotating circularly polarized laser fields as a new way to spectrally control high harmonic generation (HHG) from relativistic plasma mirrors. Through particle-in-cell simulations, we show that only a selected…

等离子体物理 · 物理学 2018-04-13 Zi-Yu Chen

The present work introduces a robust way to generate attosecond pulses with tunable ellipticity via high-order harmonic generation by co-rotating $\omega - 2\omega$ bicircular laser fields. The total electric field of the laser fields…

光学 · 物理学 2023-05-02 Rambabu Rajpoot , Amol R. Holkundkar , Navdeep Rana , Gopal Dixit

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

原子物理 · 物理学 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We study high-order harmonic generation (HHG) from aligned molecules in strong elliptically polarized laser fields numerically and analytically. Our simulations show that the spectra and polarization of HHG depend strongly on the molecular…

原子物理 · 物理学 2021-05-19 F. J. Sun , C. Chen , W. Y. Li , X. Liu , W. Li , Y. J. Chen

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

原子物理 · 物理学 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational…

光学 · 物理学 2022-01-25 Yigeng Peng , Tong Wu , Guanglu Yuan , Lihan Chi , Chao Yu , Ruifeng Lu

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

The first scheme for quasi-phase-matching high harmonic generation of circularly polarized radiation is proposed: optical rotation quasi-phase-matching (ORQPM). In ORQPM propagation of the driving radiation in a system exhibiting circular…

光学 · 物理学 2013-03-19 Lewis Z. Liu , Kevin O'Keeffe , Simon M. Hooker
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