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We report on the ESR, magnetization and magnetic susceptibility measurements performed over a large temperature range, from 1.5 to 750 K, on high-quality stoichiometric LiNiO2. We find that this compound displays two distinct temperature…

Using Monte Carlo techniques, we show that the two--dimensional anisotropic Heisenberg model reproducing nicely inelastic neutron scattering measurements on La_5 Ca_9 Cu_24 O_41 (Matsuda et al. [Phys. Rev. B 68, 060406(R) (2003)]) seems to…

统计力学 · 物理学 2009-11-10 R. Leidl , W. Selke

Neutron diffraction and bulk measurements are used to determine the nature of the low-temperature ordered state in LiCu$_2$O$_2$, a $S=1/2$ spin-chain compound with competing interactions. The magnetic structure is found to be helimagnetic,…

强关联电子 · 物理学 2007-05-23 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

Altermagnetism is a topic that has lately been gaining attention and the RuO$_2$ compound is among one of the most studied altermagnetic candidates. However, the survey of available literature on RuO$_2$ properties suggests that there is no…

材料科学 · 物理学 2024-05-03 Andriy Smolyanyuk , Igor I. Mazin , Laura Garcia-Gassull , Roser Valentí

The electronic states and magnetic properties for the copper oxides containing edge-sharing Cu-O chains such as Li$_2$CuO$_2$, La$_6$Ca$_8$Cu$_{24}$O$_{41}$ and CuGeO$_3$ are systematically studied. The optical conductivity $\sigma(\omega)$…

The preparative method, characterization and magnetic susceptibility \chi measurements versus temperature T of the heavy fermion transition metal oxide LiV_{2}O_{4} are reported in detail. The intrinsic \chi(T) shows a nearly T-independent…

强关联电子 · 物理学 2010-11-12 S. Kondo , D. C. Johnston , L. L. Miller

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

The possibilities of oxygen moment formation and canting in the quasi-1D cuprate Li2CuO2 are investigated using single crystal neutron diffraction at 2 K. The observed magnetic intensities could not be explained without the inclusion of a…

强关联电子 · 物理学 2009-11-10 E. M. L. Chung , G. J. McIntyre , D. McK. Paul , G. Balakrishnan , M. R. Lees

We report susceptibility, specific heat, and neutron diffraction measurements on NaCu$_2$O$_2$, a spin-1/2 chain compound isostructural to LiCu$_2$O$_2$, which has been extensively investigated. Below 13 K, we find a long-range ordered,…

强关联电子 · 物理学 2013-05-29 L. Capogna , M. Mayr , P. Horsch , M. Raichle , R. K. Kremer , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

Recent developments in the synthesis of new magnetic materials lead to the discovery of new quantum paramagnets. Many of these materials, such as the perovskites Ba$_{4}$LnMn$_{4}$O$_{12}$ (Ln = Sc or Nb), Ba$_{3}$Mn$_{2}$O$_{8}$, and…

材料科学 · 物理学 2022-02-08 Lauro B. Braz , Fernando A. Garcia

We provide experimental evidence for the absence of a magnetic moment in bulk RuO$_2$, a candidate altermagnetic material, by using a combination of M\"ossbauer spectroscopy, nuclear forward scattering, inelastic X-ray and neutron…

Neutron diffraction and 7Li-NMR have been applied to determine the multiferroic system LiCu2O2, which has four chains (ribbon chains) of edge-sharing CuO4 square planes in a unit cell. We have confirmed that there are successive magnetic…

Comprised of ferromagnetic edge-sharing CuO$_2$ chains that order in antialigned fashion at T$_N$=9 K, Li$_2$CuO$_2$ is found from local spin density calculations to display several surprising characteristics: (1) the ordered moment/f.u. of…

材料科学 · 物理学 2009-10-31 Ruben Weht , W. E. Pickett

NMR, muSR, magnetization and specific heat measurements in Li(2)VOSiO(4) powders and single crystals are reported. Specific heat and magnetization measurements evidence that Li(2)VOSiO(4) is a frustrated two-dimensional S=1/2 Heisenberg…

强关联电子 · 物理学 2009-11-07 R. Melzi , S. Aldrovandi , F. Tedoldi , P. Carretta , P. Millet , F. Mila

The magnetic phase diagram of CuFeO2 as a function of applied magnetic field and temperature is thoroughly explored and expanded, both for magnetic fields applied parallel and perpendicular to the material's c-axis. Pulsed field…

材料科学 · 物理学 2015-05-18 Tom T. A. Lummen , Cornelius Strohm , Harison Rakoto , Paul H. M. van Loosdrecht

We investigate magnetic, thermal, and dielectric properties of SrCuTe2O6, which is isostructural to PbCuTe2O6, a recently found, Cu-based 3D frustrated magnet with a corner sharing triangular spin network having dominant first and second…

The frustrated one-dimensional (1D) quantum magnet LiCuSbO$_4$ is one rare realization of the $J_1-J_2$ spin chain model with an easily accessible saturation field, formerly estimated to 12~T. Exotic multipolar nematic phases were…

We present an inelastic neutron scattering investigation of Li2CuO2 detecting the long sought quasi-1D magnetic excitations with a large dispersion along the CuO2-chains studied up to 25 meV. The total dispersion is governed by a…

Exchanged interactions in recently observed helical structure in LiCu2O2 is probed by inelastic neutron scattering. The main conlusions of Refs. [1,2] are confirmed: nn interactions in single chains are ferromagnetic and frustrated by nnn…

强关联电子 · 物理学 2009-11-10 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

By means of density functional theory, we investigate the magnetic ground state of edge-sharing CuO_2 spin-chains, as found in the (La,Ca,Sr)_14Cu_24O_41system, for instance. Our data rely on spin-polarized electronic structure calculations…

强关联电子 · 物理学 2009-11-13 U. Schwingenschloegl , C. Schuster