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We investigate the use of Bismuth Ferrite (BFO) nanoparticles for tumor tissue labelling in combination with infrared multi-photon excitation at 1250 nm. We report the efficient and simultaneous generation of second and third harmonic by…

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

Nanoantenna is one of the most important optical components for light harvesting. In this study, we show experimental evidence of interactions between coupled nanowires by comparing the fluorescence properties of quantum dots on both…

We analyze third-harmonic generation from high-index dielectric nanoparticles and discuss the basic features and multipolar nature of the parametrically generated electromagnetic fields near the Mie-type optical resonances. By combining…

We investigate Second Harmonic Generation from individual silicon nanowires and study the influence of resonant optical modes on the far-field nonlinear emission. We find that the polarization of the Second Harmonic has a size-dependent…

介观与纳米尺度物理 · 物理学 2016-03-18 Peter R. Wiecha , Arnaud Arbouet , Christian Girard , Thierry Baron , Vincent Paillard

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

Second-order optical nonlinear effects (second-harmonic and sum-frequency generation) are demonstrated in the telecommunication band by periodic poling of thin films of lithium niobate wafer-bonded on silicon substrates and rib-loaded with…

We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…

介观与纳米尺度物理 · 物理学 2015-05-30 A. Slablab , L. Le Xuan , M. Zielinski , Y. de Wilde , V. Jacques , D. Chauvat , J. -F. Roch

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

Spectral properties of fluorescent radiation from a two-level quantum system with broken inversion spatial symmetry, which can be described by a model of an one-electron two-level atom whose electric dipole moment operator has permanent…

量子物理 · 物理学 2024-12-17 Nikolai N. Bogolyubov, , Andrey V. Soldatov

We demonstrate third harmonic generation in plasmonic antennas made of highly doped germanium and designed to be resonant in the mid infrared. Owing to the near-field enhancement, the result is an ultrafast, sub-diffraction, coherent light…

The integration of ferroelectrics that exhibit high dielectric, piezoelectric, and thermal susceptibilities with the mainstream semiconductor industry will enable novel device types for widespread applications, and yet there are few…

材料科学 · 物理学 2023-01-11 Changming Ke , Yihao Hu , Shi Liu

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

光学 · 物理学 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…

We present the generation of high order harmonics in crystalline silicon subjected to intense near-infrared 30fs laser pulse. The harmonic spectrum extends from the near infrared to the extreme ultraviolet spectral region. Depending on the…

原子物理 · 物理学 2020-08-10 Boyan Obreshkov , Tzveta Apostolova

Bismuth nanostructures are appealing for sustainable color generation and sunlight harvesting, thanks to their non-toxicity and their tunable visible-to-near infrared interband plasmon resonances. However, owing to their broad and…

Nonlinear wavefront control is a crucial requirement in realizing nonlinear optical applications with metasurfaces. Numerous aspects of nonlinear frequency conversion and wavefront control have been demonstrated for plasmonic metasurfaces.…

We present experimental results on the observation of a bulk second-order nonlinear susceptibility derived from both free-space and integrated measurements in silicon nitride. Phase-matching is achieved through dispersion engineering of the…

High-index spherical nanoparticles with low material losses support sharp high-Q electric and magnetic resonances and exhibit a number of interesting optical phenomena. Developments in fabrication techniques have enabled the further study…

光学 · 物理学 2020-12-30 D. A. Pidgayko , Z. F. Sadrieva , K. S. Ladutenko , A. A. Bogdanov
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