相关论文: Utilizing Microcavities to Suppress Third-order Ca…
The nonlinear optical response of a system of molecules often contains contributions whereby the products of lower-order processes in two separate molecules give signals that appear on top of a genuine direct higher-order process with a…
Since the discovery of the laser, optical parametric nonlinearities have been at the core of efficient light conversion sources. Typically, thick transparent crystals or quasi-phase matched waveguides, are utilized in conjunction with…
Optical microcavities are often used to realize enhanced nonlinear optical interactions for highly efficient second-harmonic generation. With increased pump power, the efficiency of nonlinear frequency conversion can be increased further,…
Third-harmonic generation can be realized via both $\chi^{(3)}$ and cascaded $\chi^{(2)}$ nonlinear processes in a triply-resonant microcavity. It is still unknown how these processes interfere with each other and the optimization of the…
We analyze an optical parametric oscillator (OPO) in which cascaded down-conversion occurs inside a cavity resonant for all modes but the initial pump. Due to the resonant cascade design, the OPO present two \chi^2 level oscillation…
In broadband quantum optical systems, nonlinear interactions among a large number of frequency components induce complex dynamics that may defy heuristic analysis. In this work we introduce a perturbative framework for factoring out…
High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…
Optical nonreciprocity is important in photonic information processing to route the optical signal or prevent the reverse flow of noise. By adopting the strong nonlinearity associated with a few atoms in a strongly coupled cavity QED system…
We observe a nonlinear optical process in a gas of cold atoms that simultaneously displays the largest reported fifth-order nonlinear susceptibility \chi^(5) = 1.9x10^{-12} (m/V)^4 and high transparency. The nonlinearity results from the…
Silicon nitride (Si$_3$N$_4$) is an ever-maturing integrated platform for nonlinear optics. Yet, due to the absence of second-order ($\chi^{(2)}$) nonlinearity, Si$_3$N$_4$ is mostly considered for third-order ($\chi^{(3)}$) nonlinear…
We experimentally investigate on-chip control and analysis of spatially multimode nonlinear interactions in silicon nitride waveguide circuits. Using widely different dispersion of transverse supermodes in a strongly-coupled dual-core…
We propose a cavity QED scheme to enable cross-phase modulation between two arbitrarily weak classical fields in the optical domain, using organic molecular photoswitches as a disordered intracavity nonlinear medium. We show that a…
We propose and theoretically investigate a model to realize cascaded optical nonlinearity with few atoms and photons in one-dimension (1D). The optical nonlinearity in our system is mediated by resonant interactions of photons with…
The cascaded biphoton state generated from a cold atomic ensemble presents one of the strongly correlated resources that can preserve and relay quantum information. Under the four-wave mixing condition, the emitted signal and idler photons…
Second-order optical nonlinearities can be greatly enhanced by orders of magnitude in resonantly excited nanostructures, theoretically predicted and experimentally investigated in a variety of semiconductor systems. These resonant…
We calculate the third order susceptibility $\chi^{(3)}$ of a pair of 2 level atoms which interact via the exchange of photons. QED corrections to second order in coupling to vacuum field modes yield collective two photon absorption…
Microscopic cascading of second-order nonlinearities between two molecules has been proposed to yield an enhanced third-order molecular nonlinear-optical response. In this contribution, we investigate the two-molecule cascaded second…
Nonlinear optics processes lie at the heart of photonics and quantum optics for their indispensable role in light sources and information processing. During the past decades, the three- and four-wave mixing ($\chi^{(2)}$ and $\chi^{(3)}$)…
We demonstrate the emergence of nonreciprocal superradiant phase transitions and novel multicriticality in a cavity quantum electrodynamics (QED) system, where a two-level atom interacts with two counter-propagating modes of a…
We present a theoretical model and respective numerical simulation of cascaded four-wave mixing of femtosecond pulses in bulk chi(3) media, evidencing the importance of two-dimensional interaction geometries in the efficient generation of…