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A low temperature Monte Carlo dynamics of a Keating like oscillator model is used to study the relationship between the nature of glasses from the viewpoint of rigidity, and the strong-fragile behaviour of glass-forming liquids. The model…

统计力学 · 物理学 2008-03-14 Matthieu Micoulaut

Amorphous solids exhibit quasi-universal low-temperature anomalies whose origin has been ascribed to localized tunneling defects. Using an advanced Monte Carlo procedure, we create {\it in silico} glasses spanning from hyperquenched to…

无序系统与神经网络 · 物理学 2020-06-17 Dmytro Khomenko , Camille Scalliet , Ludovic Berthier , David R. Reichman , Francesco Zamponi

We analyse the collective dynamics of self-propelled particles in the large density regime where passive particles undergo a kinetic arrest to an amorphous glassy state. We capture the competition between self-propulsion and crowding…

统计力学 · 物理学 2014-06-11 Ludovic Berthier

In supercooled liquids, vitrification generally suppresses crystallization. Yet some glasses can still crystallize despite the arrest of diffusive motion. This ill-understood process may limit the stability of glasses, but its microscopic…

The physics of the glass transition and amorphous materials continues to attract the attention of a wide research community after decades of effort. Supercooled liquids and glasses have been studied numerically since the advent of molecular…

统计力学 · 物理学 2023-02-09 Ludovic Berthier , David R. Reichman

Using positional data from video-microscopy of a two-dimensional colloidal system and from simulations of hard discs we determine the wave-vector-dependent normal mode spring constants in the supercooled fluid and glassy state,…

软凝聚态物质 · 物理学 2012-10-26 Christian L. Klix , Florian Ebert , Fabian Weysser , Matthias Fuchs , Georg Maret , Peter Keim

Much of the progress achieved in understanding plasticity and failure in amorphous solids had been achieved using experiments and simulations in which the materials were loaded using strain control. There is paucity of results under stress…

统计力学 · 物理学 2015-06-19 Vladimir Dailidonis , Valery Ilyin , Pankaj Mishra , Itamar Procaccia

Glasses have a wide range of technological applications. The recent discovery of ultrastable glasses that are obtained by depositing the vapor of a glass-forming liquid onto the surface of a cold substrate has sparked renewed interest in…

统计力学 · 物理学 2014-09-04 Amir Haji-Akbari , Pablo G. Debenedetti

We explore glassy dynamics of dense assemblies of soft particles that are self-propelled by active forces. These forces have a fixed amplitude and a propulsion direction that varies on a timescale tau_p, the persistence timescale. Numerical…

软凝聚态物质 · 物理学 2021-05-26 Rituparno Mandal , Peter Sollich

This paper is the fifth in a series exploring the physical consequences of the solidity of glass-forming liquids. Paper IV proposed a model where the density field is described by a time-dependent Ginzburg-Landau equation of the…

软凝聚态物质 · 物理学 2009-11-13 Jeppe C. Dyre

We use computer simulations to probe the thermodynamic and dynamic properties of a glass-former that undergoes an ideal glass-transition because of the presence of randomly pinned particles. We find that even deep in the equilibrium glass…

无序系统与神经网络 · 物理学 2018-12-03 Misaki Ozawa , Atsushi Ikeda , Kunimasa Miyazaki , Walter Kob

Recent literature indicates that attractive interactions between particles of a dense liquid play a secondary role in determining its bulk mechanical properties. Here we show that, in contrast with their apparent unimportance to the bulk…

软凝聚态物质 · 物理学 2021-02-11 Karina González-López , Mahajan Shivam , Yuanjian Zheng , Massimo Pica Ciamarra , Edan Lerner

The universal anomalous vibrational and thermal properties of amorphous solids are believed to be related to the local variations of the elasticity. Recently it has been shown that the vibrational properties are sensitive to the glass's…

软凝聚态物质 · 物理学 2019-09-30 Alireza Shakerpoor , Elijah Flenner , Grzegorz Szamel

The statics-dynamics correspondence in spin glasses relate non-equilibrium results on large samples (the experimental realm) with equilibrium quantities computed on small systems (the typical arena for theoretical computations). Here we…

无序系统与神经网络 · 物理学 2015-05-27 Luis Antonio Fernandez , Victor Martin-Mayor

Physical vapor deposition can prepare organic glasses with high kinetic stability. When heated, these glassy solids slowly transform into the supercooled liquid in a process known as rejuvenation. In this study, we anneal vapor-deposited…

We investigate how structural relaxation in mixtures with strong dynamical asymmetry is affected by the microscopic dynamics. Brownian and Newtonian dynamics simulations of dense mixtures of fast and slow hard spheres reveal a striking…

软凝聚态物质 · 物理学 2017-10-02 Suvendu Mandal , Thomas Franosch , Thomas Voigtmann

A growing body of experimental work indicates that physical vapor deposition provides an effective route for preparation of stable glasses, whose properties correspond in some cases to those expected for glasses that have been aged for…

软凝聚态物质 · 物理学 2015-06-16 Ivan Lyubimov , Mark D. Ediger , Juan J. de Pablo

It was recently discovered that SWAP, a Monte Carlo algorithm that involves the exchange of pairs of particles of differing diameters, can dramatically accelerate the equilibration of simulated supercooled liquids in regimes where the…

统计力学 · 物理学 2019-04-02 Ludovic Berthier , Giulio Biroli , Jean-Philippe Bouchaud , Gilles Tarjus

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

软凝聚态物质 · 物理学 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

Finite-dimensional signatures of spinodal criticality are notoriously difficult to come by. The dynamical transition of glass-forming liquids, first described by mode-coupling theory, is a spinodal instability preempted by thermally…

统计力学 · 物理学 2020-09-09 Ludovic Berthier , Patrick Charbonneau , Joyjit Kundu