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Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

Current optical detection schemes for single molecules require light absorption, either to produce fluorescence or direct absorption signals. This severely limits the range of molecules that can be detected, because most molecules are…

化学物理 · 物理学 2012-07-06 Peter Zijlstra , Pedro M. R. Paulo , Michel Orrit

Controlling absorption and emission of organic molecules is crucial for efficient light-emitting diodes, organic solar cells and single-molecule spectroscopy. Here, a new molecular absorption is activated inside a gold plasmonic nanocavity,…

We use frequency entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive index sensing of a…

量子物理 · 物理学 2014-03-27 Dmitry A. Kalashnikov , Zhenying Pan , Arseniy I. Kuznetsov , Leonid A. Krivitsky

We extend Lamb's reduced density matrix laser theory to analyze the inhomogeneous molecular couplings and the mode-correlation in a plasmonic nano-laser consisting of a gold sphere and many dye molecules interacting with a driving optical…

光学 · 物理学 2017-04-27 Yuan Zhang , Klaus Mølmer

This article describes the optical properties of nanostructures composed of silver particles embedded into a gold matrix. In previous studies these materials were shown to exhibit temperature dependent transitions to a highly conductive and…

Surface Plasmon Resonance sensors are a well-established class of sensors which includes a very large variety of materials and detection schemes. However, the development of portable devices is still challenging as due to the intrinsic…

Non-Hermitian singularities known as exceptional-points (EPs) have been shown to exhibit increased sensitivities but the observation of EPs has so far been limited to wavelength scaled systems subject to diffraction limit. We propose a…

光学 · 物理学 2019-04-03 J. -H. Park , A. Ndao , W. Cai , L. -Y. Hsu , A. Kodigala , T. Lepetit , Y. -H. Lo , B. Kanté

We demonstrate experimentally and support by a theoretical analysis an effect of asymmetric spectrum broadening, which results from doping of silver nanoparticles into a heavy-glass matrix, 90(0.5WO3-0.3SbPO4-0.2PbO)-10AgCl. The strong…

光学 · 物理学 2015-05-27 N. Zhavoronkov , R. Driben , B. A. Bregadiolli , M. Nalin , B. A. Malomed

The optical responses of structured array of noble-metal nanoparticle dimers immersed in a glass matrix are investigated theoretically, motivated by the recent experimental observation of the splitting of the surface plasmon bands in silver…

光学 · 物理学 2007-05-23 J. J. Xiao , J. P. Huang , K. W. Yu

The ability to confine light down to atomic scales is critical for the development of applications in optoelectronics and optical sensing as well as for the exploration of nanoscale quantum phenomena. Plasmons in metallic nanostructures can…

Plasmonic nanoparticles from unconventional materials can improve or even bring some novel functionalities into the disciplines inherently related to plasmonics such as photochemistry or (spectro)electrochemistry. They can, for example,…

We present theoretical and experimental studies of the optical response of L-shaped silver nanoparticles. The scattering spectrum exhibits several plasmon resonances that depend sensitively on the polarization of the incident…

光学 · 物理学 2007-11-14 Maxim Sukharev , Jiha Sung , Kenneth G. Spears , Tamar Seideman

The response of gold nanoparticle dimers is studied theoretically near and beyond the limit where the particles are touching. As the particles approach each other, a dominant dipole feature is observed that is pushed into the infrared due…

其他凝聚态物理 · 物理学 2009-11-13 I. Romero , J. Aizpurua , G. W. Bryant , F. J. Garcia de Abajo

Light-matter interaction at the atomic scale rules fundamental phenomena such as photoemission and lasing, while enabling basic everyday technologies, including photovoltaics and optical communications. In this context, plasmons --the…

The selective optical detection of individual metallic nanoparticles (NPs) with high spatial and temporal resolution is a challenging endeavour, yet is key to the understanding of their optical response and their exploitation in…

介观与纳米尺度物理 · 物理学 2012-06-05 Francesco Masia , Wolfgang Langbein , Paola Borri

Nanoporous gold can be exploited as plasmonic material for enhanced spectroscopy both in the visible and in the near infrared spectral regions. In particular, with respect to bulk metal it presents interesting optical properties in the…

应用物理 · 物理学 2019-10-02 Eugenio Calandrini , Giorgia Giovannini , Denis Garoli

Deep understanding of plasmonic nanoparticles (PNPs)-light interaction over semiconductors surface shows great promises in enhancing their optoelectronic devices efficiency beyond the conventional limit. However, PNP-light interaction…

应用物理 · 物理学 2018-10-01 Kanika Arora , Vishal Kumar , Mukesh Kumar

Despite tremendous potential of highly sensitive electronic detection of bio-molecules by nanoscale biosensors for genomics and proteomic applications, many aspects of experimentally observed sensor response (S) are unexplained within…

软凝聚态物质 · 物理学 2015-05-13 Pradeep R. Nair , Muhammad A. Alam

Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

光学 · 物理学 2023-06-28 Weixiang Ye
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