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We study the magnetic excitation spectra of L-edge resonant inelastic x-ray scattering (RIXS) from the spin singlet ground state in one-dimensional undoped cuprates. Analyzing the transition amplitudes of the magnetic excitations in the…

强关联电子 · 物理学 2013-05-30 Jun-ichi Igarashi , Tatsuya Nagao

We report the high resolution resonant inelastic EUV scattering study of quantum Heisenberg antiferromagnet KCoF3. By tuning the EUV photon energy to cobalt M23 edge, a complete set of low energy 3d spin-orbital excitations is revealed.…

We study a spin-orbital model for 4$d^{1}$ or 5$d^{1}$ Mott insulators in ordered double perovskites with strong spin-orbit coupling. This model is conveniently written in terms of pseudospin and pseudo-orbital operators representing…

强关联电子 · 物理学 2017-09-12 Willian Natori , Maria Daghofer , Rodrigo Pereira

Two-dimensional coherent terahertz spectroscopy (2DCS) emerges as a valuable tool to probe the nature, couplings, and lifetimes of excitations in quantum materials. It thus promises to identify unique signatures of spin liquid states in…

强关联电子 · 物理学 2024-10-22 Yihua Qiang , Victor L. Quito , Thaís V. Trevisan , Peter P. Orth

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

强关联电子 · 物理学 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

Kitaev quantum spin liquid is a topological magnetic quantum state characterized by Majorana fermions of fractionalized spin excitations, which are identical to their own antiparticles. Here, we demonstrate emergence of Majorana fermions…

Although orbital degrees of freedom are a factor of fundamental importance in strongly correlated transition metal compounds, orbital correlations and dynamics remain very difficult to access, in particular by neutron scattering. Via a…

强关联电子 · 物理学 2015-03-20 Pasquale Marra , Krzysztof Wohlfeld , Jeroen van den Brink

Several powerful techniques exist to detect topologically protected surface states of weakly-interacting electronic systems. In contrast, surface modes of strongly interacting systems which do not carry electric charge are much harder to…

强关联电子 · 物理学 2016-08-24 Brent Perreault , Johannes Knolle , Natalia B. Perkins , F. J. Burnell

We theoretically demonstrate that a resonant inelastic x-ray scattering (RIXS) with a sizable momentum transfer can be utilized to study valence band dispersion for broad band materials. We take RIXS at the Si K edge of 3C-SiC as a typical…

材料科学 · 物理学 2009-09-21 Yunori Nisikawa , Muneharu Ibuki , Manabu Usuda

We present a new set up for resonant inelastic hard X-ray scattering at the Bernina beamline of SwissFEL with energy, momentum, and temporal resolution. The compact R=0.5 m Johann-type spectrometer can be equipped with up to 3 crystal…

The excitations in honeycomb $\alpha$-Li$_2$IrO$_3$ have been investigated with high-resolution resonant inelastic x-ray scattering (RIXS) at the O K edge. The low-energy response is dominated by a fully resolved ladder of excitations,…

Emergent symmetry breakings in condensed matter systems are often intimately linked to collective excitations. For example, the intertwined spin-charge stripe order in cuprate superconductors is associated with spin and charge excitations.…

We explore the general phenomenology of resonant inelastic scattering (RIXS) using CuB2O4, a network of CuO4 plaquettes electronically isolated by B+3 ions. Spectra show a small number of well-separated features, and we exploit the simple…

Inelastic neutron scattering (INS) has traditionally been one of the primary methods for investigating quantum magnets, particularly in identifying a continuum of excitations as a hallmark of spin fractionalization in quantum spin liquids…

强关联电子 · 物理学 2025-12-11 Emily Z. Zhang , Ciarán Hickey , Yong Baek Kim

Resonant inelastic X-ray scattering (RIXS) detects various types of high- and low-energy elementary excitations in correlated solids, and this tool will play an increasingly important role in investigations of time-dependent phenomena in…

强关联电子 · 物理学 2021-12-21 Philipp Werner , Steven Johnston , Martin Eckstein

The fractionalization of elementary excitations in quantum spin systems is a central theme in current condensed matter physics. The Kitaev honeycomb spin model provides a prominent example of exotic fractionalized quasiparticles, composed…

强关联电子 · 物理学 2016-09-21 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Choi , K. -Y. Choi

We calculate the K-edge indirect bimagnon resonant inelastic X-ray scattering (RIXS) intensity spectra of the bicollinear antiferromagnetic order known to occur in the $\alpha$-FeTe chalcogenide system. Utilizing linear spin wave theory for…

材料科学 · 物理学 2017-11-28 Zengye Huang , Sean Mongan , Trinanjan Datta , Dao-Xin Yao

Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray…

We present the first circularly polarized Floquet engineering time-resolved Resonant Inelastic X-ray Scattering (tr-RIXS) experiment in H$_3$LiIr$_2$O$_6$, an iridium-based Kitaev system. Our calculations and experimental results are…

We report an Fe $L$-edge resonant inelastic x-ray scattering (RIXS) study of the unusual superconductor $\beta$-FeSe. The high energy resolution of this RIXS experiment ($\approx\,$55$\,$meV FWHM) made it possible to resolve low-energy…

超导电性 · 物理学 2019-01-16 M. C. Rahn , K. Kummer , N. B. Brookes , A. A. Haghighirad , K. Gilmore , A. T. Boothroyd