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Optical frequency combs represent a revolutionary technology for high precision spectroscopy due to their narrow linewidths and precise frequency spacing. Generation of such combs in the mid-infrared (IR) spectral region (2-20 um) is of…

Mid-infrared frequency comb spectroscopy enables measurement of molecular at megahertz spectral resolution, sub-hertz frequency accuracy and microsecond acquisition speed. However, the widespread adoption of this technique has been hindered…

The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…

While mid-infrared optical frequency combs have been widely utilized in areas such as trace gas sensing, chemical kinetics, and combustion science, the relatively low power per comb tooth has limited acquisition times and sensitivities. We…

光学 · 物理学 2023-09-28 Adam T. Heiniger , Matthew J. Cich , David A. Long

Nanophotonic waveguides with sub-wavelength mode confinement and engineered dispersion profiles are an excellent platform for application-tailored nonlinear optical interactions at low pulse energies. Here, we present fully air clad…

Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we…

光学 · 物理学 2020-01-16 Noh Soo Han , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

We present a simple method for fully-stabilized mid-infrared optical frequency comb generation based on single-pass femtosecond optical parametric generation that is seeded by a continuous-wave laser. We have implemented the method in a…

光学 · 物理学 2024-06-12 Mikhail Roiz , Krishna Kumar , Juho Karhu , Markku Vainio

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

光学 · 物理学 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

We experimentally demonstrate a simple configuration for mid-infrared (MIR) frequency comb generation in quasi-phase-matched lithium niobate waveguides using the cascaded-$\chi^{(2)}$ nonlinearity. With nanojoule-scale pulses from an…

We demonstrate efficient generation of mid-infrared frequency combs based on continuous-wave-seeded femtosecond optical parametric generation in nonlinear waveguides. Conversion of the near-infrared pump to signal and idler light takes…

光学 · 物理学 2021-09-01 Mikhail Roiz , Jui-Yu Lai , Juho Karhu , Markku Vainio

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

光学 · 物理学 2017-04-05 Markku Vainio , Juho Karhu

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

Directly accessing the middle infrared, the molecular functional group spectral region, via supercontinuum generation processes based on turn-key fiber lasers offers the undeniable advantage of simplicity and robustness. Recently, the…

Infrared spectroscopy is a powerful tool for basic and applied science. The molecular spectral fingerprints in the 3 um to 20 um region provide a means to uniquely identify molecular structure for fundamental spectroscopy, atmospheric…

Mid-infrared (mid-IR) frequency combs have broad applications in molecular spectroscopy and chemical/biological sensing. Recently developed microresonator-based combs in this wavelength regime could enable portable and robust devices using…

The development of broadband microresonator frequency combs at visible wavelengths is pivotal for the advancement of compact and fieldable optical atomic clocks and spectroscopy systems. Yet, their realization necessitates resonators with…

Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…

光学 · 物理学 2014-05-28 P. Del Haye , A. Schliesser , O. Arcizet , T. Wilkins , R. Holzwarth , T. J. Kippenberg

We demonstrate dual-comb spectroscopy based on difference frequency generation of frequency-agile near-infrared frequency combs, produced with the help of electro-optic modulators. The combs have a remarkably flat intensity distribution and…

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