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Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic…

We present comprehensive inelastic neutron spectroscopic maps of the magnetic field-induced disordered phase of the Kitaev quantum spin liquid candidate material $\alpha$-RuCl$_3$. For fields along both in-plane high-symmetry directions we…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

强关联电子 · 物理学 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

强关联电子 · 物理学 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

强关联电子 · 物理学 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

The honeycomb magnet $\alpha$-RuCl$_{3}$ has been a leading candidate for realizing the Kitaev quantum spin liquid (QSL), but its intrinsic spin dynamics have remained obscured by crystal twinning. Here we apply biaxial anisotropic strain…

The pure Kitaev honeycomb model harbors a quantum spin liquid in zero magnetic fields, while applying finite magnetic fields induces a topological spin liquid with non-Abelian anyonic excitations. This latter phase has been much sought…

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

强关联电子 · 物理学 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

$\alpha$-RuCl$_3$ has been studied extensively because of its proximity to the Kitaev quantum-spin-liquid (QSL) phase and the possibility of approaching it by tuning the competing interactions. Here we present the first polarized inelastic…

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

强关联电子 · 物理学 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

There has been a great interest in magnetic field induced quantum spin liquids in Kitaev magnets after the discovery of neutron scattering continuum and half quantized thermal Hall conductivity in the material $\alpha$-RuCl$_3$. In this…

强关联电子 · 物理学 2020-01-10 Li Ern Chern , Ryui Kaneko , Hyun-Yong Lee , Yong Baek Kim

An external magnetic field can induce a transition in $\alpha$-RuCl$_3$ from an ordered zigzag state to a disordered state that is possibly related to the Kitaev quantum spin liquid. Here we present new field dependent inelastic neutron…

The search for new elementary particles is one of the most basic pursuits in physics, spanning from subatomic physics to quantum materials. Magnons are the ubiquitous elementary quasiparticle to describe the excitations of fully-ordered…

Collective excitations in magnetic materials can be investigated by means of inelastic neutron scattering. We show that this experimental method gives access to the complete spectrum of magnetic fluctuations through the energy- and…

强关联电子 · 物理学 2007-05-23 B. Roessli , P. Böni

Frustration in magnetic materials arising from competing exchange interactions can prevent the system from adopting long-range magnetic order and can instead lead to a diverse range of novel quantum and topological states with exotic…

As one of the most promising Kitaev quantum-spin-liquid (QSL) candidates, $\alpha$-RuCl$_3$ has received a great amount of attention. However, its ground state exhibits a long-range zigzag magnetic order, which defies the QSL phase.…

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

强关联电子 · 物理学 2022-01-13 Heung-Sik Kim

The weakly coupled quasi-one-dimensional spin ladder compound (CH$_3$)$_2$CHNH$_3$CuCl$_3$ is studied by neutron scattering in magnetic fields exceeding the critical field of Bose-Einstein condensation of magnons. Commensurate long-range…

Collective motions in strongly interacting magnets involve many spins and are often described in terms of integer-spin excitations. However, in certain cases, the collective motion can behave as if these integer excitations break apart into…

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