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We study the shift of rotational levels of a diatomic polar molecule due to its van der Waals (vdW) interaction with a gently curved dielectric surface at temperature $T$, and submicron separations. The molecule is assumed to be in its…

量子物理 · 物理学 2016-08-18 Giuseppe Bimonte , Thorsten Emig , Robert L. Jaffe , Mehran Kardar

We show theoretically that ultracold hydrogen atoms have very favorable properties for sympathetic cooling of molecules to microkelvin temperatures. We calculate the potential energy surfaces for spin-polarized interactions of H atoms with…

原子物理 · 物理学 2013-11-20 Maykel L. Gonzalez-Martinez , Jeremy M. Hutson

A novel two-stage helium buffer gas cooled beam source is introduced. The properties of the molecular beams produced from this source are investigated theoretically using the CaF as a test molecule. The gas-phase molecules are first…

原子物理 · 物理学 2020-04-14 Vijay Singh

The association processes between engineered TiO2 nanoparticles and Suwannee River humic acids are investigated by isothermal titration calorimetry and by measuring the exchanged heat during binding process allowing the determination of…

材料科学 · 物理学 2021-09-21 Frédéric Loosli , Letícia Vitorazi , Jean-François Berret , Serge Stoll

We investigate the possibility of producing ultracold NH3 molecules by sympathetic cooling in a bath of ultracold atoms. We consider the interactions of NH3 with alkali-metal and alkaline-earth atoms, and with Xe, using ab initio…

化学物理 · 物理学 2010-03-09 Piotr S. Żuchowski , Jeremy M. Hutson

In the cooling concept by adiabatic melting, solid $^{4}$He is converted to liquid and mixed with $^{3}$He to produce cooling power directly in the liquid phase. This method overcomes the thermal boundary resistance that conventionally…

其他凝聚态物理 · 物理学 2019-02-13 T. S. Riekki , A. P. Sebedash , J. T. Tuoriniemi

We study the energetics of chemical reactions between ultracold ground-state alkaline-earth-metal diatomic molecules. We show that the atom-exchange reactions forming homonuclear dimers are energetically allowed for all heteronuclear…

原子物理 · 物理学 2023-12-01 Hela Ladjimi , Michał Tomza

We study the interaction of atomic and molecular hydrogen with a surface of tholin, a man-made polymer considered to be an analogue of aerosol particles present in Titan's atmosphere, using thermal programmed desorption at low temperatures…

地球与行星天体物理 · 物理学 2010-10-08 Ling Li , Hui Zhao , Gianfranco Vidali , Yechiel Frank , Ingo Lohmar , Hagai B. Perets , Ofer Biham

The study of the formation of molecular hydrogen on low temperature surfaces is of interest both because it allows to explore elementary steps in the heterogeneous catalysis of a simple molecule and because of the applications in…

化学物理 · 物理学 2008-11-21 G. Vidali , V. Pirronello , L. Li , J. Roser , G. Manico , R. Mehl , A. Lederhendler , H. B. Perets , J. R. Brucato , O. Biham

The long-range electrostatic interactions between molecules depend strongly on their relative orientation, which manifests as a rotational state dependence. Interactions between molecules in the same rotational quantum state are well-known…

原子物理 · 物理学 2024-05-16 Etienne F. Walraven , Tijs Karman

An evaluation of slow neutrons deceleration through their interaction with nanoclusters in liquid helium is performed. It is shown that process is strongly suppresed if the clusters are bound by the van der Waals interaction.

原子与分子团簇 · 物理学 2008-12-06 Yu. N. Pokotilovski

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…

量子物理 · 物理学 2009-10-07 M. Zeppenfeld , M. Motsch , P. W. H. Pinkse , G. Rempe

The paper presents a simplified formula to determine an electron temperature, Te(He I), for planetary nebulae (PNe) using the He I 7281/6678 line flux ratio. In our previous studies of Te(He I) (Zhang et al. 2005), we used the He I line…

天体物理学 · 物理学 2007-05-23 Y. Zhang , R. H. Rubin , X. -W. Liu

Elemental tellurium (Te) is a compelling van der Waals material due to its interesting chiral crystal structure and predicted topological properties. Here, we report the fabrication and comprehensive quantum transport study of devices based…

Diffusion mediated interaction in metal-substrate assembly during high temperature annealing leads to possible formation of new composite materials. Here, sputtered grown Ti films on Si3N4/Si substrate has been reported to produce titanium…

材料科学 · 物理学 2020-11-19 Sachin Yadav , Sangeeta Sahoo

We produce beams of neutral titanium (Ti) atoms in their metastable $3d^{3}(^4F){4}s$ $a^5F_5$ state by laser ablation into He, N$_2$, and Ar buffer gases. The high temperatures realized in the ablation process populate the $a^5F_5$ level…

原子物理 · 物理学 2024-10-11 Jack Schrott , Scott Eustice , Dan Stamper-Kurn

The present study aims to detect helium-3 in nickel-based metal nano-composites doped with zirconia, which exhibited anomalous heat generation when exposed to hydrogen gas at approximately 450{\deg}C. Two complementary analytical techniques…

We explore the potential energy surfaces for NH molecules interacting with alkali-metal and alkaline-earth atoms using highly correlated ab-initio electronic structure calculations. The surfaces for interaction with alkali-metal atoms have…

化学物理 · 物理学 2015-05-13 Pavel Soldán , Piotr S. Żuchowski , Jeremy M. Hutson

Using electrospray ion beam deposition, we collide the complex molecule Reichardt's Dye (C41H30NO+) at low, hyperthermal translational energy (2-50 eV) with a Cu(100) surface and image the outcome at single-molecule level by scanning…

Direct laser cooling of molecules has made significant progress in recent years. However, the selective cooling and manipulation of molecules based on their isotopic composition, which is ubiquitous in atomic laser cooling, has not yet been…