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We extend the existing framework of macroscopic HHG to combine it with high-accuracy ab initio calculations for molecules as microscopic input. This approach is applied to HHG spectra exhibiting Mollow sidebands, for open shell molecules…

化学物理 · 物理学 2025-08-13 T Joyce , A. Jaron

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

Su-Schrieffer-Heeger (SSH) chains are the simplest model systems that display topological edge states. We calculate high-harmonic spectra of SSH chains that are coupled to an external laser field of a frequency much smaller than the band…

光学 · 物理学 2024-03-12 Hannah Jürß , Dieter Bauer

This paper focuses on investigating high-order harmonic generation (HHG) in graphene quantum dots (GQDs) under intense near-infrared laser fields. To model the GQD and its interaction with the laser field, we utilize a mean-field approach.…

介观与纳米尺度物理 · 物理学 2023-09-15 H. K. Avetissian , A. G. Ghazaryan , Kh. V. Sedrakian , G. F. Mkrtchian

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

原子物理 · 物理学 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

The extreme nonlinear optical process of high-harmonic generation (HHG) makes it possible to map the properties of a laser beam onto a radiating electron wavefunction, and in turn, onto the emitted x-ray light. Bright HHG beams typically…

High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…

光学 · 物理学 2021-03-26 M. S. Mrudul , Gopal Dixit

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

光学 · 物理学 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

We theoretically study high-harmonic generation (HHG) from solids driven by intense laser pulses using a one-dimensional model periodic crystal. By numerically solving the time-dependent Schr\"{o}dinger equation directly on a real-space…

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

原子物理 · 物理学 2016-04-27 M. A. Khokhlova , V. V. Strelkov

Collinear double-pulse seeding of the High-Gain Harmonic Generation (HGHG) process in a free-electron laser (FEL) is a promising approach to facilitate various coherent nonlinear spectroscopy schemes in the extreme ultraviolet (XUV)…

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

光学 · 物理学 2022-03-03 Davis M. Welakuh , Prineha Narang

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

强关联电子 · 物理学 2021-03-17 G. van der Laan , S. W. Lovesey

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup…

原子物理 · 物理学 2009-11-07 F. Ceccherini , D. Bauer

In strong field laser physics it is a common practice to use the high-order harmonic cutoff to estimate the laser intensity of the pulse that generates the harmonic radiation. Based on the semiclassical arguments it is possible to find a…

原子物理 · 物理学 2015-06-11 T. Shaaran , M. F. Ciappina , M. Lewenstein

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

原子物理 · 物理学 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

光学 · 物理学 2023-05-03 Lun Yue , Mette B. Gaarde

High harmonic generation (HHG) from condensed matter phase holds promise to promote future cutting-edge research in the emerging field of attosecond nanoscopy. The key for the progress of the field relies on the capability of the existing…

光学 · 物理学 2021-07-07 Hicham Agueny