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We study the dynamics of paramagnetic molecular superrotors in an external magnetic field. Optical centrifuge is used to create dense ensembles of oxygen molecules in ultra-high rotational states. It is shown for the first time, that the…

量子物理 · 物理学 2015-06-10 A. A. Milner , A. Korobenko , J. Floß , I. Sh. Averbukh , V. Milner

We consider optical properties of a gas of molecules that are brought to fast unidirectional spinning by a pulsed laser field. It is shown that a circularly polarized probe light passing through the medium inverts its polarization…

光学 · 物理学 2015-06-17 Uri Steinitz , Yehiam Prior , Ilya Sh. Averbukh

An all-optical method of ultrafast spin rotation is put forward to precisely manipulate the polarization of relativistic charged particle beams of leptons or ions. In particular, laser-driven dense ultrashort beams are manipulated via…

We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…

化学物理 · 物理学 2024-06-19 P. Amani , A. A. Milner , V. Milner

We investigate theoretically the ability of an optical centrifuge - a laser pulse whose linear polarization is rotating at an accelerated rate, to control molecular rotation in the regime when the rigid-rotor approximation breaks down due…

量子物理 · 物理学 2025-12-11 J. M. García-Garrido , V. Milner , C. P. Koch , R. González-Férez

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

介观与纳米尺度物理 · 物理学 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

We demonstrate demagnetization cooling of a gas of ultracold $^{52}$Cr atoms. Demagnetization is driven by inelastic dipolar collisions which couple the motional degrees of freedom to the spin degree. By that kinetic energy is converted…

其他凝聚态物理 · 物理学 2015-06-25 M. Fattori , T. Koch , S. Goetz , A. Griesmaier , S. Hensler , J. Stuhler , T. Pfau

The non-thermal optical control of magnetic order offers a promising route to ultrafast, energy-efficient information technologies. Although optical manipulation of magnetism in metals has been extensively studied, experimentally…

We outline the design and characterization of a laser pulse shaper, which creates an ``ultraslow optical centrifuge'' - a linearly polarized field whose polarization vector rotates with arbitrarily low angular acceleration. By directly…

化学物理 · 物理学 2026-03-12 Kevin Wang , Ian MacPhail-Bartley , Cameron E. Peters , Valery Milner

In past decades, ultrafast spin dynamics in magnetic systems have been associated with heat deposition from high energy laser pulses, limiting the selective access to spin order. Here we use a long wavelength terahertz pump optical probe…

材料科学 · 物理学 2021-06-04 Hovan Lee , Cedric Weber , Manfred Fähnle , Mostafa Shalaby

We excite diatomic oxygen and nitrogen to high rotational states with an optical centrifuge and study their dynamics in external magnetic field. Ion imaging is employed to directly visualize, and follow in time, the rotation plane of…

化学物理 · 物理学 2015-04-08 Aleksey Korobenko , Valery Milner

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

材料科学 · 物理学 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

The control of ultrafast molecular rotational motion has benefited from the development of innovative techniques in strong-field laser physics. Here, we theoretically demonstrate a novel type of coherent control by inducing rotation of an…

化学物理 · 物理学 2018-08-27 Alec Owens , Andrey Yachmenev , Jochen Küpper

Laser control of molecular rotation is an area of active research. A number of recent studies has aimed at expanding the reach of rotational control to extreme, previously inaccessible rotational states, as well as controlling the…

量子物理 · 物理学 2015-01-13 V. Milner , J. W. Hepburn

Since its invention in 1999, optical centrifuge has become a powerful tool for controlling molecular rotation and studying molecular dynamics and molecular properties at extreme levels of rotational excitation. The technique has been…

仪器与探测器 · 物理学 2020-05-20 Ian MacPhail-Bartley , Walter W. Wasserman , Alexander A. Milner , V. Milner

Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…

We show that the electron spin polarization generated by an electrical current may have its direction controlled and magnitude amplified by periodic optical excitation. The electrical and optical spin control methods were combined and…

介观与纳米尺度物理 · 物理学 2014-07-17 Felix G. G. Hernandez , Gennady M. Gusev , Askhat K. Bakarov

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific…

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

光学 · 物理学 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

We report the experimental observation of the rotation of the polarization plane of light propagating in a gas of fast-spinning molecules (molecular super-rotors). In the observed effect, related to Fermi's prediction of "polarization drag"…

原子物理 · 物理学 2021-08-18 Alexander A. Milner , Uri Steinitz , Ilya Sh. Averbukh , Valery Milner
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