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相关论文: Ba8CoNb6O24: a spin-1/2 triangular-lattice Heisenb…

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We successfully synthesized and characterized the triangular lattice anitferromagnet Ba$_8$MnNb$_6$O$_{24}$, which comprises equilateral spin-5/2 Mn$^{2+}$ triangular layers separated by six non-magnetic Nb$^{5+}$ layers. The detailed…

材料科学 · 物理学 2019-06-03 R. Rawl , L. Ge , Z. Lu , Z. Evenson , C. R. Dela Cruz , Q. Huang , M. Lee , E. S. Choi , M. Mourigal , H. D. Zhou , J. Ma

The double perovskite ${\rm La}_2{\rm NiTiO}_6$ is identified as a three-dimensional $S=1$ quantum magnet. By means of Density Functional Theory we demonstrate that this material is a high-spin $d$-electron system deep in the Heisenberg…

强关联电子 · 物理学 2015-03-03 Michael Karolak , Martin Edelmann , Giorgio Sangiovanni

We report the results of magnetization and specific heat measurements on Ba$_3$CoSb$_2$O$_9$, in which the magnetic Co$^{2+}$ ion has a fictitious spin-1/2, and show evidence that a spin-1/2 Heisenberg antiferromagnet on a regular…

强关联电子 · 物理学 2015-05-30 Yutaka Shirata , Hidekazu Tanaka , Akira Matsuo , Koichi Kindo

Frustrated quantum magnets pose well-defined questions concerning quantum fluctuation effects and the nature of the many-body wavefunction, which challenge theory, numerics, experiment and materials synthesis. The S = 1/2 triangular-lattice…

强关联电子 · 物理学 2017-09-28 Y. Cui , J. Dai , P. Zhou , P. S. Wang , T. R. Li , W. H. Song , L. Ma , Z. Zhang , S. Y. Li , G. M. Luke , B. Normand , T. Xiang , W. Yu

We develop anisotropic pseudo-spin antiferromagnetic Heisenberg models for monoclinically distorted double perovskites. We focus on these A$_2$BB'O$_6$ materials that have magnetic moments on the 4d or 5d transition metal B' ions, which…

强关联电子 · 物理学 2011-12-12 Tyler Dodds , Ting-Pong Choy , Yong Baek Kim

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

We have studied the magnetic properties of Ba_2FeNbO_6 and Ba_2MnNbO_6. it is seen that Ba_2FeNbO_6 is an antiferromagnet with a weak ferromagnetic behaviour at 5K while Ba_2MnNbO_6 shows two magnetic transitions one at 45 K and the other…

We report the crystal structure of Ba$_2$La$_2$CoTe$_2$O$_{12}$ determined by Rietveld analysis using X-ray powder diffraction data. It was found from magnetic measurements that Ba$_2$La$_2$CoTe$_2$O$_{12}$ can be described as a spin-1\2…

We report the magnetic susceptibility and the low-temperature specific heat of a double perovskite compound, Sr2CuTeO6, which is expected as the spin-1/2 square-lattice Heisenberg antiferromagnet with nearest-neighbor J1 and…

强关联电子 · 物理学 2015-06-23 Tomoyuki Koga , Nobuyuki Kurita , Hidekazu Tanaka

The ordered hexagonal perovskite Ba2CuTeO6 hosts weakly coupled S=1/2 spin ladders produced by an orbital ordering of Cu2+. The magnetic susceptibility chi(T) of Ba2CuTeO6 is well described by that expected for isolated spin ladders with…

The magnetic structure of the double perovskite compound Sr$_2$CuTeO$_6$ was determined from neutron powder diffraction data. This material is magnetically described as an $S\,{=}\,1/2$ quasi-two-dimensional square-lattice Heisenberg model…

强关联电子 · 物理学 2016-03-09 Tomoyuki Koga , Nobuyuki Kurita , Maxim Avdeev , Sergey Danilkin , Taku J. Sato , Hidekazu Tanaka

We establish the double perovskite Ba$_2$CeIrO$_6$ as a nearly ideal model system for j=1/2 moments, with resonant inelastic x-ray scattering indicating a deviation of less than 1% from the ideally cubic j=1/2 state. The local j=1/2 moments…

We report the structural, magnetic and thermodynamic properties of the double perovskite compound La2CuIrO6 from X-ray, neutron diffraction, neutron depolarization, dc magnetization, ac susceptibility, specific heat, muon-spin-relaxation…

We report the synthesis and initial characterization of Ba6Y2Rh2Ti2O17-{\delta}, a previously unreported material with a hexagonal symmetry structure. Face-sharing RhO6 octahedra form triangular planes of Rh2O9 dimers that are widely…

强关联电子 · 物理学 2021-04-07 Loi T. Nguyen , Daniel B. Straus , Q. Zhang , R. J. Cava

We report on the cubic double perovskite Ba2MgReO6 containing Re6+ ions with the 5d1 electron configuration. Resistivity, magnetization, and heat capacity measurements using single crystals show that the compound is a Mott insulator with a…

强关联电子 · 物理学 2019-06-11 Daigorou Hirai , Zenji Hiroi

Magnetic properties of an antiferromagnetic double perovskite oxide Ba2CaReO6, where Re6+ (5d1) ions with large spin-orbit coupling are arranged on the face-centered-cubic lattice, are investigated using pulsed high magnetic field up to 66…

Hexagonal perovskite 15R-BaMnO2.99 with a ratio of cubic to hexagonal layers of 1/5 in the unit cell is an antiferromagnetic insulator that orders at a N\'eel temperature TN = 220 K. Here we report structural, magnetic, dielectric and…

强关联电子 · 物理学 2010-11-11 O. B. Korneta , T. F. Qi , M. Ge , S. Parkin , L. E. DeLong , P. Schlottmann , G. Cao

We report on the quasi-two-dimensional magnetism of the natural mineral diaboleite Pb2Cu(OH)4Cl2 with a tetragonal crystal structure, which is closely related to that of the frustrated spin-1/2 magnet PbVO3. Magnetic susceptibility of…

材料科学 · 物理学 2013-02-15 Alexander A. Tsirlin , Oleg Janson , Stefan Lebernegg , Helge Rosner

The synthesis and physical properties of the double perovskite (DP) compound Ba2CdReO6 with the 5d1 electronic configuration are reported. Three successive phases originating from a spin-orbit-entangled Jeff = 3/2 state, confirmed by the…

强关联电子 · 物理学 2021-04-06 Daigorou Hirai , Zenji Hiroi

Magnetic properties of the spin-3/2 Heisenberg system Cr2BP3O12 are investigated by magnetic susceptibility chi(T) measurements, electron spin resonance, neutron diffraction, and density functional theory (DFT) calculations, as well as…

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