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Excitons, Coulomb-bound electron and hole pairs, are elementary photo-excitations in semiconductors, that can couple directly to light through radiative relaxation. In contrast to these bright excitons, dark excitons X$\rm{_D}$ with…

材料科学 · 物理学 2018-02-14 Kyoung-Duck Park , Tao Jiang , Genevieve Clark , Xiaodong Xu , Markus B. Raschke

Two-dimensional halide perovskite nanoplatelets (NPLs) have exceptional light-emitting properties, including wide spectral tunability, ultrafast radiative decays, high quantum yields (QY), and oriented emission. To realize efficient…

Controlling light-matter interactions in solid-state systems has motivated intense research to produce bosonic quasi-particles known as exciton-polaritons, which requires strong coupling between excitons and cavity photons. Ultra-low…

The realization and control of polaritons is of paramount importance in the prospect of novel photonic devices. Here, we investigate the emergence of plasmon-exciton polaritons in hybrid structures consisting of a two-dimensional (2D)…

介观与纳米尺度物理 · 物理学 2018-01-10 P. A. D. Gonçalves , L. P. Bertelsen , Sanshui Xiao , N. Asger Mortensen

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

介观与纳米尺度物理 · 物理学 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

Room-temperature strong coupling of a single quantum emitter and a single resonant plasmonic mode is a key resource for quantum information processing and quantum sensing at ambient conditions. To beat dephasing, ultrafast energy transfer…

Polaritons, formed as a result of strong hybridization of matter with light, are promising for important applications including organic solar cells, optical logic gates, and qubits. Owing to large binding energies of Frenkel excitons…

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Strong light-matter interactions in both the single-emitter and collective strong coupling regimes attract significant attention due to emerging quantum and nonlinear optics applications, as well as opportunities for modifying…

介观与纳米尺度物理 · 物理学 2019-09-11 Tuomas P. Rossi , Timur Shegai , Paul Erhart , Tomasz J. Antosiewicz

Strong coupling between light and matter in an optical cavity provides a pathway to giant polariton nonlinearity, where effective polariton-polariton interactions are mediated by materials' nonlinear responses. The pursuit of such enhanced…

光学 · 物理学 2024-11-26 Zhi Wang , Li He , Bumho Kim , Bo Zhen

Exciton polaritons are hybrid particles of excitons (bound electron-hole pairs) and cavity photons, which are renowned for displaying Bose Einstein condensation and other coherent phenomena at elevated temperatures. However, their formation…

介观与纳米尺度物理 · 物理学 2024-08-29 Kenneth Choo , Olivier Bleu , Jesper Levinsen , Meera M. Parish

In an effort to elucidate the spin (rather than charge) degrees of freedom in colloidal semiconductor nanocrystal quantum dots, we report on a series of static and time-resolved photoluminescence measurements of colloidal CdSe quantum dots…

材料科学 · 物理学 2007-05-23 Madalina Furis , Jennifer Hollingsworth , Victor I. Klimov , Scott A. Crooker

Although both epitaxial quantum dots (QDs) and colloidal nanocrystals (NCs) are quantum-confined semiconductor nanostructures, so far they have demonstrated dramatically-different exciton fine structure splittings (FSSs) at the cryogenic…

介观与纳米尺度物理 · 物理学 2017-07-19 Chunyang Yin , Liyang Chen , Yan Lv , Fengrui Hu , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and…

光学 · 物理学 2018-07-04 Alex Krasnok , Sergey Lepeshov , Andrea Alú

Atomically thin semiconductors exhibit tunable exciton resonances that can be harnessed for dynamic manipulation of visible light in ultra-compact metadevices. However, the rapid nonradiative decay and dephasing of excitons at room…

光学 · 物理学 2025-02-18 Tom Hoekstra , Jorik van de Groep

We investigate theoretically the effects of interaction between an optical dipole (semiconductor quantum dot or molecule) and metal nanoparticles. The calculated absorption spectra of hybrid structures demonstrate strong effects of…

介观与纳米尺度物理 · 物理学 2009-11-13 Jie-Yun Yan , Wei Zhang , Suqing Duan , Xian-Geng Zhao , Alexander O. Govorov

We demonstrate control over light-matter coupling at room temperature combining a field effect transistor (FET) with a tuneable optical microcavity. Our microcavity FET comprises a monolayer tungsten disulfide WS$_2$ semiconductor which was…

介观与纳米尺度物理 · 物理学 2019-05-29 Henry A. Fernandez , Freddie Withers , Saverio Russo , William L. Barnes

We describe photonic crystal microcavities with very strong light-matter interaction to realize room-temperature, equilibrium, exciton-polariton Bose-Einstein condensation (BEC). This is achieved through a careful balance between strong…

量子气体 · 物理学 2015-03-17 Jian-Hua Jiang , Sajeev John