相关论文: Giant pressure dependence and dimensionality switc…

Metal organic magnets have enormous potential to host a variety of electronic and magnetic phases that originate from a strong interplay between the spin, orbital and lattice degrees of freedom. We control this interplay in the quantum…

We present the results of high-field magnetization and muon-spin relaxation measurements on the coordination polymer CuF_2(H_2O)_2(pyrazine) in pressures up to 22.5 kbar. We observe a transition from a quasi-two-dimensional to a…

Cu(pz)2(ClO4)2 (with pz denoting pyrazine, C4H4N2) is among the best realizations of a two-dimensional spin-1/2 square-lattice antiferromagnet. Below T_N = 4.21 K, its weak interlayer couplings induce a 3D magnetic order, strongly…

Quantum magnets in two dimensions display strong quantum interaction effects even when magnetically ordered. Using the metal-organic framework material CuF$_2$(D$_2$O)$_2$(pyz), we investigate the field-dependent spin dynamics of the $S =…

Near zero temperature, quantum magnetism can non-trivially arise from short-range interactions, but the occurrence of magnetic order depends crucially on the interplay of interactions, lattice geometry, dimensionality and doping. Even…

Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…

We report the magnetization ($\chi$, $M$), specific heat ($C_{\text{P}}$), and neutron powder diffraction results on a quasi-two-dimensional $S$ = 2 square lattice antiferromagnet Ba$_2$FeSi$_2$O$_7$ consisting of FeO$_4$ tetragons with a…

The field dependence of interlayer magnetoresistance of the pressurized (to the normal state) layered organic metal $\alpha $-(BEDT-TTF)$_{2}$KHg(SCN)$_{4}$ is investigated. The high quasi-two-dimensional anisotropy, when the interlayer…

The magnetic properties of [Mn(pyrazinecarboxylate)2]n (Mn-pyrazine), empirical formula C10H6MnN4O4, are investigated through susceptibility, heat capacity and neutron scattering measurements. The structure of Mn-pyrazine consists of Mn-Mn…

Although the isotope effect in superconducting materials is well-documented, changes in the magnetic properties of antiferromagnets due to isotopic substitution are seldom discussed and remain poorly understood. This is perhaps surprising…

We study the S=1/2 Heisenberg antiferromagnet on a square lattice with nearest-neighbor and plaquette four-spin exchanges (introduced by A.W. Sandvik, Phys. Rev. Lett. {\bf 98}, 227202 (2007).) This model undergoes a quantum phase…

Quasi-one-dimensional quantum antiferromagnets formed by a d-dimensional hypercubic lattice of weakly coupled spin-1/2 antiferromagnetic Heisenberg chains are studied by combining exact results in one-dimension and renormalization group…

Using a mixed-ligand synthetic scheme, we create a family of quasi-two-dimensional antiferromagnets, namely, [Cu(HF$_2$)(pyz)$_2$]ClO$_4$ [pyz = pyrazine], [Cu$L_2$(pyz)$_2$](ClO$_4$)$_2$ [$L$ = pyO = pyridine-N-oxide and 4-phpyO =…

We have considered the $S=1/2$ antiferromagnetic Heisenberg model in two dimensions, with an additional Ising \nnn interaction. Antiferromagnetic \nnn interactions will lead to frustration, and the system responds with flipping the spins…

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

We present an experimental study of the two-dimensional S=1/2 square-lattice antiferromagnet Cu(pz)$_2$(ClO$_4$)$_2$ (pz denotes pyrazine - $C_4H_4N_2$) using specific heat measurements, neutron diffraction and cold-neutron spectroscopy.…

We study the quantum transition from a strongly correlated metal, with heavy fermionic quasiparticles, to a metal with commensurate charge or spin density wave order. To this end, we introduce and numerically analyze a large dimensionality…

We examine the nature of the transition to the antiferromagnetically ordered state in the half-filled three-dimensional Hubbard model using the dual-fermion multiscale approach. Consistent with analytics, in the weak-coupling regime we find…

Magnetic properties in the quasi-one-dimensional organic salt (TMTTF)2SbF6 are investigated by 13C NMR under pressures. Antiferromagnetic phase transition at ambient pressure (AFI) is confirmed. Charge-ordering is suppressed by pressure and…

We successfully synthesize single crystals of the verdazyl radical $\alpha$-2,3,5-Cl$_3$-V. $Ab$ $initio$ molecular orbital calculations indicate that the two dominant antiferromagnetic interactions, $J_{\rm{1}}$ and $J_{\rm{2}}$ ($\alpha…