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相关论文: Thermal Recovery Mechanisms of UO2 Lattices

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Swelling of uranium dioxide with ingrowth of defects by irradiation is not fully understood. Experimental and theoretical groups have attempted to explain this phenomenon with various complex theories. In this study, experimental lattice…

材料科学 · 物理学 2016-05-03 S. D. Günay

The radiation damage in optical materials mostly manifests itself as the loss of optical transmittance. The optical materials recover from radiation damage to some extent when the radiation exposure is stopped. The recovery is at a faster…

To efficiently capture the energy of the nuclear bond, advanced nuclear reactor concepts seek solid fuels that must withstand unprecedented temperature and radiation extremes. In these advanced fuels, thermal energy transport under…

{\alpha}-particle irradiated single-crystal isostructural oxide lattices (CmO2, AmO2, CeO2, UO2, NpO2, PuO2, ThO2) were modeled by molecular dynamics simulation method. Lattice parameter changes with IFP cation defects displayed exponential…

材料科学 · 物理学 2023-02-17 S. D. Günay

Data available in the literature of lattice parameter changes in Ni, Cu and MgO single crystals irradiated in neutron reactors are tentatively reproduced using ad hoc ion irradiation experiments. The nature and energy of the ions were…

材料科学 · 物理学 2021-10-27 Xin Jin , Alexandre Boulle , Jérôme Bourcoit , Aurélien Debelle

In this article we investigated surface of nanocrystals (NC) of uranium dioxide (UO2) using molecular dynamics (MD) under isolated (non-periodic) boundary conditions with the approximation of pair potentials and rigid ions. It is shown that…

材料科学 · 物理学 2011-12-08 A. S. Boyarchenkov , S. I. Potashnikov , K. A. Nekrasov , A. Ya. Kupryazhkin

Melting of uranium dioxide (UO2) nanocrystals has been studied by molecular dynamics (MD) simulation. Ten recent and widely used sets of pair potentials were assessed in the rigid ion approximation. Both isolated (in vacuum) and periodic…

材料科学 · 物理学 2012-06-22 A. S. Boyarchenkov , S. I. Potashnikov , K. A. Nekrasov , A. Ya. Kupryazhkin

Uranium dioxide which is used as a fuel in light water nuclear reactors, is continually exposed to radiation damage originated from the collision of high-energy particles. Accumulation of the resulting defects gives rise to the evolution in…

材料科学 · 物理学 2025-04-14 Mahmoud Payami , Samira Sheykhi , Mohammad-Reza Basaadat

An atomistically informed mean field cluster dynamics model has been presented to investigate the nucleation and growth of defect loops in irradiated {\alpha}-U. TEM analysis of neutron irradiated {\alpha}-U shows the evolution of SIA and…

材料科学 · 物理学 2023-07-17 Sanjoy Kumar Mazumder , Tiankai Yao , Anter El-Azab

In the prevalent picture of ultrafast structural phase transitions, the atomic motion occurs in a slowly varying potential energy surface determined adiabatically by the fast electrons. However, this ignores non-conservative forces caused…

We study the mechanics of temperature-driven reconstructive martensitic transformations in crystalline materials, within the framework of nonlinear elasticity theory. We focus on the prototypical case of the square-hexagonal transition in…

材料科学 · 物理学 2025-05-23 Edoardo Arbib , Noemi Barrera , Paolo Biscari , Giovanni Zanzotto

Understanding the nature of irradiation damage often requires a multi-scale and multi-physics approach, i.e. it requires a significant amount of information from experiments, simulations and phenomenological models. This paper focuses on…

材料科学 · 物理学 2024-05-07 Bartosz Barzdajn , Christopher P Race

The structural and electronic recovery pathways of a photoexcited ultrathin VO2 film at nanosecond time scales have been studied using time-resolved x-ray diffraction and transient optical absorption techniques. The recovery pathways from…

Commercial nuclear power plants extensively rely on fission energy from uranium dioxide (UO2) fuel pellets that provide thermal energy; consequently, generating carbon-free power in current generation reactors. UO2 fuel incurs damage and…

Making use of the energetics and equations of state of defective uranium dioxide that calculated with first-principles method, we demonstrate a possibility of constraining the formation energy of point defects by measuring the transition…

材料科学 · 物理学 2013-05-30 Hua Y. Geng , Hong X. Song , Q. Wu

Lattice dynamics and molecular dynamics studies of the oxides UO2 and Li2O in their normal as well as superionic phase are reported. Lattice dynamics calculations have been carried out using a shell model in the quasiharmonic approximation.…

材料科学 · 物理学 2011-11-10 Prabhatasree Goel , N. Choudhury , S. L. Chaplot

X-ray absorption and resonant X-ray emission measurements at the O 1s edge of the uranium oxides UO2, U3O8 and UO3 are presented. The spectral shapes of the O K{\alpha} X-ray emission spectra of UO3 exhibit significant excitation energy…

强关联电子 · 物理学 2011-12-30 M. Magnuson , S. M. Butorin , L. Werme , J. Nordgren , K. Ivanov , J. -H. Guo , D. K. Shuh

Unraveling the adsorption mechanism and thermodynamics of O$_2$ and H$_2$O on uranium dioxide surfaces is critical for the nuclear fuel storage and uranium corrosion. Based on the first-principles DFT+U-D3 calculations, we carefully test…

材料科学 · 物理学 2025-02-13 Yang Huang , Le Zhang , Hefei Ji , Zhipeng Zhang , Qili Zhang , Bo Sun , Haifeng Liu , Haifeng Song

ODS steels based on yttrium oxide have been suggested as potential fusion reactor wall materials due to their observed radiation resistance properties. Presumably this radiation resistance can be related to the interaction of the particle…

材料科学 · 物理学 2015-06-17 J. Brodrick , D. J. Hepburn , G. J. Ackland

The economical lifetime of the divertor is a key concern for realizing nuclear fusion reactors that may solve the world's energy problem. A main risk is thermo-mechanical failure of the plasma-facing tungsten monoblocks, as a consequence of…

材料科学 · 物理学 2019-09-04 A. Mannheim , J. A. W. van Dommelen , M. G. D. Geers
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