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Through analysis of variable temperature neutron powder diffraction data, we present solutions for the magnetic structures of SrMn$_7$O$_{12}$, CdMn$_7$O$_{12}$, and PbMn$_7$O$_{12}$ in all long-range ordered phases. The three compounds…

强关联电子 · 物理学 2017-09-06 R. D. Johnson , D. D. Khalyavin , P. Manuel , P. G. Radaelli , I. S. Glazkova , N. Terada , A. A. Belik

Orbitally ordered states evolving coincidentally with structural distortions and magnetic ordering provide a novel route to controlling electronic and magnetic properties of materials through external fields. We report an unprecedented…

强关联电子 · 物理学 2012-08-06 N. J. Perks , R. D. Johnson , C. Martin , L. C. Chapon , P. G. Radaelli

The magnetic structure of the novel Hg$_{0.7}$Na$_{0.3}$Mn$_3$Mn$_4$O$_{12}$, a quadruple manganite perovskite that exhibits a unique $G$-type charge and orbital ordered state distinct to other $A^{2+}$Mn$_3$Mn$_4$O$_{12}$ equivalents ($A$…

强关联电子 · 物理学 2025-12-17 Ben R. M. Tragheim , Fabio Orlandi , En-Pei Liu , Wei-Tin Chen , Mark S. Senn

Magnetic structures and the relationship between spin and charge-orbital orderings of an A-site ordered double-perovskite manganite SmBaMn2O6, an anticipated multiferroic material, were investigated by means of neutron diffraction. The spin…

We report a neutron powder diffraction study of $R$Mn$_7$O$_{12}$ quadruple perovskite manganites with $R$ = La, Ce, Nd, Sm, and Eu. We show that in all measured compounds concomitant magnetic ordering of the $A$ and $B$ manganese…

强关联电子 · 物理学 2018-08-29 R. D. Johnson , D. D. Khalyavin , P. Manuel , L. Zhang , K. Yamaura , A. A. Belik

We have investigated the spin fluctuations in the langasite compound Ba3NbFe3Si2O14 in both the ordered state and as a function of temperature. The low temperature magnetic structure is defined by a spiral phase characterized by magnetic…

强关联电子 · 物理学 2015-05-19 C. Stock , L. C. Chapon , A. Schneidewind , Y. Su , P. G. Radaelli , D. F. McMorrow , A. Bombardi , N. Lee , S. -W. Cheong

The crystallographic and magnetic phase diagram of the n=2 layered manganite La2-2xSr1+2xMn2O7 in the region x=>0.5 has been studied using temperature dependent neutron powder diffraction. The magnetic phase diagram reveals a progression of…

材料科学 · 物理学 2009-10-31 C. D. Ling , J. E. Millburn , J. F. Mitchell , D. N. Argyriou J. Linton , H. N. Bordallo

Spin density waves, based on modulated local moments, are usually associated with metallic materials, but have recently been reported in insulators which display coupled magnetic and structural order parameters. We discuss one such example,…

材料科学 · 物理学 2020-07-30 N. Giles-Donovan , N. Qureshi , R. D. Johnson , L. Y. Zhang , S. -W. Cheong , S. Cochran , C. Stock

The layered compound La2-2xSr1+2xMn2O7 (x=0.3) consists of bilayers of metallic MnO2 sheets separated by insulating material. The compound exhibits markedly anisotropic magnetoresistance at temperatures well below the three-dimensional…

强关联电子 · 物理学 2009-10-31 T. G. Perring , G. Aeppli , T. Kimura , Y. Tokura , M. A. Adams

Structural behaviour of PbMn$_{7}$O$_{12}$ has been studied by high resolution synchrotron X-ray powder diffraction. This material belongs to a family of quadruple perovskite manganites that exhibit an incommensurate structural modulation…

强关联电子 · 物理学 2021-05-05 R. D. Johnson , D. D. Khalyavin , P. Manuel , A. A. Belik

We have performed muon spin rotation/relaxation (muSR) measurements on single crystals of the chiral helimagnet Cr1/3NbS2 at zero to low magnetic field. The transition from the paramagnetic to helical magnetically ordered phase at zero…

材料科学 · 物理学 2015-06-23 D. Braam , C. Gomez , S. Tezok , E. V. L. de Mello , L. Li , D. Mandrus , Hae-Young Kee , J. E. Sonier

The magnetic response of CaK(Fe$_{0.949}$Ni$_{0.051}$)$_4$As$_4$ was investigated by means of the muon-spin rotation/relaxation. The long-range commensurate magnetic order sets in below the N\'{e}el temperature $T_{\rm N}= 50.0(5)$~K. The…

Quantum-disordered magnetic ground states are challenging to identify in three-dimensional (3D) oxides, where strong exchange pathways typically favour long-range magnetic order or spin freezing. The quadruple perovskite…

We study theoretically the phase diagram of the double-layered perovskite manganites taking into account the orbital degeneracy, the strong Coulombic repulsion, and the coupling with the lattice deformation. Observed spin structural changes…

强关联电子 · 物理学 2009-10-31 Ryo Maezono , Naoto Nagaosa

Marcasite-type compounds have been proposed as promising hosts of exotic magnetic quantum states, yet experimental realizations in stoichiometric, disorder-free systems remain limited. Here, we report the high-pressure stabilization and…

Structure with orbital degeneracy is unstable toward spontaneous distortion. Such orbital correlation usually has a much higher energy scale than spins, and therefore, magnetic transition takes place at a much lower temperature, almost…

强关联电子 · 物理学 2018-10-11 Huiyuan Man , Mario Halim , Hiroshi Sawa , Masayuki Hagiwara , Yusuke Wakabayashi , Satoru Nakatsuji

The monoclinic double-perovskite Sr2YRuO6 has recently gained a renewed interest in order to get a deeper insight into the exotic magnetic ground states associated with geometric frustration. Striking discrepancies between the spin order…

材料科学 · 物理学 2016-04-19 P. L. Bernardo , L. Ghivelder , H. S. Amorim , J. J. Neumeier , S. Garcia

We present the discovery and refinement by neutron powder diffraction of a new magnetic phase in the Na1-xCaxMn7O12 quadruple perovskite phase diagram, which is the incommensurate analogue of the well-known pseudo-CE phase of the simple…

强关联电子 · 物理学 2018-08-01 R. D. Johnson , F. Mezzadri , P. Manuel , D. D. Khalyavin , E. Gilioli , P. G. Radaelli

The manganese tellurate Li2MnTeO6 consists of trigonal spin lattices made up of Mn4+ (d3, S = 3/2) ions. The magnetic properties of this compound were characterized by several experimental techniques, which include magnetic susceptibility,…

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

强关联电子 · 物理学 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel
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