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We construct a model for interacting electrons with strong spin orbit coupling in the pyrochlore iridates. We establish the importance of the direct hopping process between the Ir atoms and use the relative strength of the direct and…

强关联电子 · 物理学 2012-02-02 William Witczak-Krempa , Yong Baek Kim

Recently, there have been contrary claims of Kitaev spin-liquid behaviour and ordered behavior in the honeycomb compound Ag$_3$LiIr$_2$O$_6$ based on various experimental signatures. Our investigations on this system reveal a…

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

强关联电子 · 物理学 2013-05-30 Jean-Michel Carter , Hae-Young Kee

The effect of compression on the magnetic ground state of Sr$_2$IrO$_4$ is studied with x-ray resonant techniques in the diamond anvil cell. The weak interlayer exchange coupling between square-planar 2D IrO$_2$ layers is readily modified…

We report Resonant Inelastic X-ray Scattering (RIXS) study of the magnetic excitation spectrum in a highly insulating Eu$_{2}$Ir$_{2}$O$_{7}$ single crystal that exhibits a metal-insulator transition at $T_{MI}$ = 111(7) K. A propagating…

The family of magnetic rare-earth pyrochlore oxides R2M2O7 plays host to a diverse array of exotic phenomena, driven by the interplay between geometrical frustration and spin-orbit interaction, which leads to anisotropy in both magnetic…

强关联电子 · 物理学 2017-03-21 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

强关联电子 · 物理学 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

The magnetic excitation spectrum in the bilayer iridate Sr$_3$Ir$_2$O$_7$ has been investigated using high-resolution resonant inelastic x-ray scattering (RIXS) performed at the iridium L$_3$ edge and theoretical techniques. A study of the…

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

统计力学 · 物理学 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

The pyrochlore iridates have become ideal platforms to unravel fascinating correlated and topolog?ical phenomena that stem from the intricate interplay among strong spin-orbit coupling, electronic correlations, lattice with geometric…

Dirac matters provide a platform for exploring the interplay of their carriers with other quantum phenomena. Sr$_{1-x}$Mn$_{1-y}$Sb$_2$ has been proposed to be a magnetic Weyl semimetal and provides an excellent platform to study the…

Quasiperiodic structures possess long range positional order, but are freed of constraints imposed by translational invariance. For spins interacting via Heisenberg couplings, one may expect therefore to find novel magnetic configurations…

强关联电子 · 物理学 2008-10-15 Anuradha Jagannathan , Attila Szallas

We study the ground state properties of an anisotropic, quasi-2D version of the quantum (S=1/2) pyrochlore antiferromagnet. In the presence of Dzyaloshinsky-Moriya interactions, in addition to the Heisenberg exchanges, it is shown that two…

强关联电子 · 物理学 2008-10-08 Valeri N. Kotov

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

We discuss the ground state properties of a spin 1/2 magnetic ion with threefold $t_{2g}$ orbital degeneracy on a highly frustrated pyrochlore lattice, like Ti$^{3+}$ ion in B-spinel MgTi$_2$O$_4$. We formulate an effective spin-orbital…

强关联电子 · 物理学 2007-05-23 S. Di Matteo , G. Jackeli , N. B. Perkins

We discuss the ground state of a pyrochlore lattice of threefold-orbitally-degenerate $S=1/2$ magnetic ions. We derive an effective spin-orbital Hamiltonian and show that the orbital degrees of freedom can modulate the spin exchange,…

强关联电子 · 物理学 2007-05-23 S. Di Matteo , G. Jackeli , C. Lacroix , N. B. Perkins

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

We performed resonant x-ray diffraction experiments at the $L$ absorption edges for the post-perovskite-type compound CaIrO$_{3}$ with $(t_{2g})^5$ electronic configuration. By observing the magnetic signals, we could clearly see that the…

We study the electronic state of an inverse spinel compound MnMg$_{2}$O$_{4}$ based on first-principles calculations. The high-spin state is realized in Mn ions on the diamond lattice, resulting in that this material is found to be a…

材料科学 · 物理学 2022-03-22 Satoshi Tomita , DaPeng Yao , Hiroki Tsuchiura , Kentaro Nomura

Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…