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We study experimentally the influence of the intensity of the infrared (IR) probe field on attosecond pulse train (APT) phase measurements performed with the RABITT method (Reconstruction of Attosecond Beating by Interference in Two-Photon…

原子物理 · 物理学 2009-07-22 M. Swoboda , J. M. Dahlstrom , T. Ruchon , P. Johnsson , J. Mauritsson , K. J. Schafer , A. L'Huillier

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

化学物理 · 物理学 2017-05-18 David Ayuso

We illustrate how attosecond light pulses can be used to directly mapping out the time-dependence of the correlated motion of two excited atomic electrons, discuss how the two-electron correlations manifest themselves in realistic…

原子物理 · 物理学 2007-05-23 Toru Morishita , Shinichi Watanabe , C. D. Lin

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

原子物理 · 物理学 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

A theory for the many-electron multi-photon process is presented. It is shown that after single-electron excitation into some level in the continuum (ATI) an inelastic collision of the excited electron with the parent atomic particle can…

atom-ph · 物理学 2009-10-28 M. Yu. Kuchiev

We investigate the possibility to monitor the dynamics of autoionizing states in real time and control the yields of different ionization channels in helium by simulating XUV-pump IR-probe experiments focused on the N=2 threshold. The XUV…

原子物理 · 物理学 2015-05-18 Luca Argenti , Eva Lindroth

We report on the experimental observation of strong-field dressing of an autoionizing two-electron state in helium with intense extreme-ultraviolet laser pulses from a free-electron laser. The asymmetric Fano line shape of this transition…

In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time)…

原子物理 · 物理学 2019-09-04 Jan Troß , Georgios Kolliopoulos , Carlos A. Trallero-Herrero

A three-dimensional semiclassical model is used to study double ionization of Ar when driven by a near-infrared and near-single-cycle laser pulse for intensities ranging from 0.85$\times$10$^{14}$ W/cm$^{2}$ to 5$\times$10$^{14}$…

原子物理 · 物理学 2017-02-15 A. Chen , M. Kübel , B. Bergues , M. F. Kling , A. Emmanouilidou

Bright squeezed light from parametric down-conversion in the infrared (IR) frequency range has triggered the emergence of attosecond quantum optics -- a new research field at the interface of quantum optics, strong-field physics, and…

Nonsequential multiple ionization of atoms in intense laser fields is initiated by a recollision between an electron, freed by tunneling, and its parent ion. Following recollision, the initial electron shares its energy with several bound…

原子物理 · 物理学 2009-11-11 X. Liu , C. Figueira de Morisson Faria , W Becker , P. B. Corkum

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

仪器与探测器 · 物理学 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

We study the role of electron-electron correlation in the ground-state of Ne, as well as in photoionization dynamics induced by an attosecond XUV pulse. For a selection of central photon energies around 100 eV, we find that while the…

原子物理 · 物理学 2018-01-31 Juan J. Omiste , Lars Bojer Madsen

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We explore the influence of elliptical polarization on the (non)sequential two-photon double ionization of atomic helium with ultrashort extreme ultraviolet (XUV) light fields using time-dependent full ab-initio simulations. The energy and…

原子物理 · 物理学 2019-02-20 Stefan Donsa , Iva Brezinova , Hongcheng Ni , Johannes Feist , Joachim Burgdörfer

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Attosecond time-resolution experiments using noncollinear interferometers require precise and active control of the optical delay to prevent instabilities - including both slow drifts and rapid vibrations - that can obscure the time…

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

原子物理 · 物理学 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein