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We evaluate the electric quadrupole moments of the ${^1}\!S_0$ and ${^3}\!P_0$ clock states of $^{27}$Al$^+$ and $^{115}$In$^+$. To capture all dominant contributions, our analysis extends through third order of perturbation theory and…

原子物理 · 物理学 2017-04-11 K. Beloy , D. R. Leibrandt , W. M. Itano

We evaluate the feasibility of using magnetic-dipole (M1) transitions in highly-charged ions as a basis of an optical atomic clockwork of exceptional accuracy. We consider a range of possibilities, including M1 transitions between clock…

原子物理 · 物理学 2015-06-23 V. I. Yudin , A. V. Taichenachev , A. Derevianko

We consider hyperfine-mediated effects for clock transitions in $^{176}$Lu$^+$. Mixing of fine structure levels due to the hyperfine interaction bring about modifications to Land\'e $g$-factors and the quadrupole moment for a given state.…

原子物理 · 物理学 2020-09-08 Zhiqiang Zhang , K. J. Arnold , R. Kaewuam , M. S. Safronova , M. D. Barrett

Spherically-symmetric ground states of alkali-metal atoms do not posses electric quadrupole moments. However, the hyperfine interaction between nuclear moments and atomic electrons distorts the spherical symmetry of electronic clouds and…

原子物理 · 物理学 2016-01-13 Andrei Derevianko

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

原子物理 · 物理学 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

We use advanced computational techniques to study the electronic structure of the Hf$^{12+}$ ion, with the goal of assessing its potential for use in highly accurate atomic optical clocks and search for new physics. Such clocks should…

原子物理 · 物理学 2025-11-04 Saleh O. Allehabi , V. A. Dzuba , V. V. Flambaum

Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…

原子物理 · 物理学 2014-12-01 N. Huntemann , B. Lipphardt , Chr. Tamm , V. Gerginov , S. Weyers , E. Peik

Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider…

原子物理 · 物理学 2015-06-11 V. A. Dzuba , A. Derevianko , V. V. Flambaum

Divalent atoms and ions with a singlet $S$ ground state and triplet $P$ excited state form the basis of many high-precision optical atomic clocks. Along with the metastable $^{3}\mathrm{P}_{0}$ clock state, these atomic systems also have a…

Recent developments in frequency metrology and optical clocks have been based on electronic transitions in atoms and singly charged ions as references. These systems have enabled relative frequency uncertainties at a level of a few parts in…

原子物理 · 物理学 2018-12-06 M. G. Kozlov , M. S. Safronova , J. R. Crespo López-Urrutia , P. O. Schmidt

Permanent electric dipole moments (EDMs) of fundamental particles such as the electron are signatures of parity and time-reversal violation due to physics beyond the standard model. EDM measurements probe new physics at energy scales well…

原子物理 · 物理学 2020-10-09 Mohit Verma , Andrew M. Jayich , Amar C. Vutha

Searching for an accurate optical clock which can serve as a better time standard than the present day atomic clock is highly demanding from several areas of science and technology. Several attempts have been made to built more accurate…

原子物理 · 物理学 2007-09-17 Chiranjib Sur , Rajat K Chaudhuri

Demands from several areas of science and technology have lead to a worldwide search for accurate optical clocks with an uncertainty of 1 part in $10^{18}$, which is $10^{3}$ times more accurate than the present day cesium atomic clocks…

原子物理 · 物理学 2017-08-23 Chiranjib Sur , K. V. P. Latha , Rajat K. Chaudhuri , B. P. Das , D. Mukherjee

The influence of oscillating quadrupole fields on atomic energy levels is examined theoretically and general expressions for the quadrupole matrix elements are given. The results are relevant to any ion-based clock in which one of the clock…

量子物理 · 物理学 2019-03-06 Kyle J. Arnold , R. Kaewuan , T. R. Tan , M. D. Barrett

We have developed a broadly-applicable approach that drastically increases the ability to accurately predict properties of complex atoms. We applied it to the case of Ir$^{17+}$, which is of particular interest for the development of novel…

原子物理 · 物理学 2020-04-29 C. Cheung , M. S. Safronova , S. G. Porsev , M. G. Kozlov , I. I. Tupitsyn , A. I. Bondarev

We apply relativistic many-body methods to compute static differential polarizabilities for transitions inside the ground-state hyperfine manifolds of monovalent atoms and ions. Knowing this transition polarizability is required in a number…

原子物理 · 物理学 2011-07-13 V. A. Dzuba , V. V. Flambaum , K. Beloy , A. Derevianko

We report the coherent excitation of the highly forbidden $^2S_{1/2} \rightarrow {^2}F_{7/2}$ clock transition in the odd isotope $^{173}\mathrm{Yb}^+$ with nuclear spin $I = 5/2$, and reveal the hyperfine-state-dependent, nuclear spin…

Solid-state electronic spins are extensively studied in quantum information science, as their large magnetic moments offer fast operations for computing and communication, and high sensitivity for sensing. However, electronic spins are more…

Atomic clocks use atomic transitions as frequency references. The susceptibility of the atomic transition to external fields limits clock stability and introduces systematic frequency shifts. Here, we propose to realize an atomic clock that…

原子物理 · 物理学 2017-09-06 Nitzan Akerman , Roee Ozeri

Relativistic formulas for the electric quadrupole moment of a hydrogenlike atom, induced by the hyperfine interaction, are derived for $ns_{1/2}$ and $np_{1/2}$ states. Both the magnetic dipole and electric quadrupole hyperfine interactions…

原子物理 · 物理学 2009-11-11 Y. S. Kozhedub , V. M. Shabaev
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