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We report magnetic and thermodynamic properties of single crystal $\alpha$-RuCl$_3$, in which the Ru$^{3+}$ ($4d^5$) ion is in its low spin state and forms a honeycomb lattice. Two features are observed in both magnetic susceptibility and…

强关联电子 · 物理学 2015-04-27 J. A. Sears , M. Songvilay , K. W. Plumb , J. P. Clancy , Y. Qiu , Y. Zhao , D. Parshall , Young-June Kim

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

材料科学 · 物理学 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

The layered transition metal trihalide $\alpha$-RuCl$_3$ has been studied extensively in recent years as a promising candidate for a proximate Kitaev quantum spin liquid state. In high quality samples, a complete structural transition from…

材料科学 · 物理学 2026-01-05 Paige Harford , Ezekiel Horsley , Subin Kim , Young-June Kim

$\alpha$-RuCl$_3$ is a candidate Kitaev material that exhibits zigzag antiferromagnetic ordering below 7 K. One contentious issue regarding this material is its bulk structure in the low-temperature phase. Recently, it has become generally…

材料科学 · 物理学 2026-01-27 Seung-Ju Hong , Tae Yun Kim , Cheol-Hwan Park

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

强关联电子 · 物理学 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

The layered honeycomb magnet alpha-RuCl3 has been proposed as a candidate to realize a Kitaev spin model with strongly frustrated, bond-dependent, anisotropic interactions between spin-orbit entangled jeff=1/2 Ru4+ magnetic moments. Here we…

We report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on two $\alpha$-RuCl$_{3}$ crystals with distinct magnetic transition temperatures: T$_{N}$=7.3K and 6.5K. We find that the sample with T$_{N}$=6.5K exhibits a…

强关联电子 · 物理学 2024-03-08 Subin Kim , Ezekiel Horsley , Christie Nelson , Jacob Ruff , Young-June Kim

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

$\alpha$-RuCl$_3$ has been proposed recently as an excellent playground for exploring Kitaev physics on a two-dimensional (2D) honeycomb lattice. However, structural clarification of the compound has not been completed, which is crucial in…

材料科学 · 物理学 2016-04-27 Heung-Sik Kim , Hae-Young Kee

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…

$\alpha$-RuCl$_3$, a well-known candidate material for Kitaev quantum spin liquid, is prone to stacking disorder due to the weak van der Waals bonding between the honeycomb layers. After a decade of intensive experimental and theoretical…

The layered honeycomb magnet $\alpha$-RuCl$_3$ has emerged as a promising candidate for realizing a Kitaev quantum spin liquid. Previous studies have reported oscillation-like anomalies in the longitudinal thermal conductivity and…

强关联电子 · 物理学 2025-04-01 Y. Xing , R. Namba , K. Imamura , K. Ishihara , S. Suetsugu , T. Asaba , K. Hashimoto , T. Shibauchi , Y. Matsuda , Y. Kasahara

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

强关联电子 · 物理学 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

Kitaev quantum spin liquids have attracted significant attention in condensed matter physics over the past decade. To understand their emergent quantum phenomena, high-quality single crystals of substantial size are essential. Here, we…

强关联电子 · 物理学 2025-02-18 Bowen Zhang , Xiangjun Li , Limin Yan , Wenbo Li , Nana Li , Jianfa Zhao , Xiaobing Liu , Shun-Li Yu , Zhiwei Hu , Wenge Yang , Runze Yu

The layered honeycomb magnet $\alpha$-RuCl$_3$ is the most promising candidate for a Kitaev quantum spin liquid (KQSL) that can host charge-neutral Majorana fermions. Recent studies have shown significant sample dependence of thermal…

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the…

Raman scattering has been employed to investigate lattice and magnetic excitations of the honeycomb Kitaev material $\alpha$-RuCl$_3$ and its Heisenberg counterpart CrCl$_3$. Our phonon Raman spectra give evidence for a first-order…

强关联电子 · 物理学 2017-06-07 A. Glamazda , P. Lemmens , S. -H. Do , Y. S. Kwon , K. -Y. Choi

Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

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