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相关论文: Resonant second-harmonic-generation circular-dichr…

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Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…

Metasurfaces, the two-dimensional analogues of metamaterials, are ideal platforms for sensing molecular chirality at the nanoscale, e.g. of inclusions of natural optically active molecules, as they offer large accessible areas (they are…

应用物理 · 物理学 2020-08-19 Sotiris Droulias

In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar…

Photons with spin angular momentum possess intrinsic chirality which underpins many phenomena including nonlinear optics1, quantum optics2, topological photonics3 and chiroptics4. Intrinsic chirality is weak in natural materials, and recent…

We theoretically investigate light matter interactions for chiral molecules in the presence of non-chiral nanoantennas. Isotropic nanostructures supporting optical-frequency electric or magnetic dipoles are sufficient to locally enhance the…

介观与纳米尺度物理 · 物理学 2013-06-14 Aitzol Garcia-Etxarri , Jennifer A. Dionne

Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular…

Controlling optical chirality at the subwavelength scales is essential for many applications of nanophotonic structures in polarization optics, sensing, and nonlinear photonics. Achieving a strong chiroptical response in planar dielectric…

Chiral photonics aims to control and engineer light handedness for many applications in optical communications, biological and chemical sensing, and quantum technologies. While traditional approaches focus on engineering strong linear…

DNA and proteins are chiral: their three-dimensional structure cannot be superimposed with its mirror image. Circular dichroism spectroscopy is widely used to characterize chiral compounds, but data interpretation is difficult in the case…

生物大分子 · 定量生物学 2020-09-09 Steven Daly , Frederic Rosu , Valerie Gabelica

Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation (SHG) response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole (E1) and…

强关联电子 · 物理学 2019-12-11 S. W. Lovesey , G. van der Laan

We review the physics and some applications of photonic structures designed for the realisation of strong $\textit{nonlinear chiroptical response}$. We pay much attention to the recent strategy of utilizing different types of…

光学 · 物理学 2023-11-10 Kirill Koshelev , Pavel Tonkaev , Yuri Kivshar

Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a…

We study the resonant enhancement of linear and nonlinear chiroptical effects in asymmetric silicon metasurfaces supporting multipolar Mie resonances and quasi-bound states in the continuum (quasi-BICs). We demonstrate theoretically and…

光学 · 物理学 2023-01-10 Kirill Koshelev , Yutao Tang , Zixian Hu , Ivan Kravchenko , Guixin Li , Yuri Kivshar

Chirality refers to a geometric phenomenon in which objects are not superimposable on their mirror image. Structures made of nano-scale chiral elements can display chiroptical effects, such as dichroism for left- and right- handed…

光学 · 物理学 2020-02-25 Behrooz Semnani , Jeremy Flannery , Rubayet Al Maruf , Michal Bajcsy

We propose a system to visualize the chirality of the protein in brains, which would be helpful to diagnose early neurological degenerative diseases in vivo. These neurological degenerative diseases often occur along with some mark…

信号处理 · 电气工程与系统科学 2022-07-19 Wending Mai , Yifan Chen

Sometimes it appears, sometimes it does not. We present a theoretical study of circular dichroism in the second-harmonic signal of single dielectric nanostructures with different symmetries and noncentrosymmetric materials. We show that…

光学 · 物理学 2023-01-24 Anastasia Nikitina , Anna Nikolaeva , Kristina Frizyuk

Chirality is an intriguing property of certain molecules, materials or artificial nanostructures, which allows them to interact with the spin angular momentum of the impinging light field. Due to their chiral geometry, they can distinguish…

光学 · 物理学 2016-11-03 Peter Banzer , Pawel Wozniak , Uwe Mick , Israel De Leon , Robert W. Boyd

Dynamic control of circular dichroism in photonic structures is critically important for compact spectrometers, stereoscopic displays, and information processing exploiting multiple degrees of freedom. Metasurfaces can help miniaturize…

Chiral photonics opens new pathways to manipulate light-matter interactions and tailor the optical response of meta-surfaces and -materials by nanostructuring nontrivial patterns. Chirality of matter, such as that of molecules, and light,…

光学 · 物理学 2022-02-16 Oliver Mey , Arash Rahimi-Iman

Strong enhancement of molecular circular dichroism has the potential to enable efficient asymmetric photolysis, a method of chiral separation that has conventionally been impeded by insufficient yield and low enantiomeric excess. Here, we…

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