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Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

介观与纳米尺度物理 · 物理学 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

Developments in optoelectronics and spin-optronics based on transition metal dichalcogenide monolayers (MLs) need materials with efficient optical emission and well-defined transition energies. In as-exfoliated MoS2 MLs the…

Optically dark excitonic states play a critical role in the valleytronic, electronic, and optical properties of monolayer semiconducting transition metal dichalcogenides. Here, we investigate how electrostatic doping affects the in-plane…

Strong Coulomb interactions in single-layer transition metal dichalcogenides (TMDs) result in the emergence of strongly bound excitons, trions and biexcitons. These excitonic complexes possess the valley degree of freedom, which can be…

Transition metal dichalcogenides (TMDs) are layered materials that have a semiconducting phase with many advantageous optoelectronic properties, including tightly bound excitons and spin-valley locking. In Tungsten-based TMDs, spin and…

介观与纳米尺度物理 · 物理学 2022-04-27 Saroj B. Chand , John M. Woods , Enrique Mejia , Takashi Taniguchi , Kenji Watanabe , Gabriele Grosso

We perform photoluminescence experiments at 4K on two different transition metal diselenide monolayers, namely MoSe2 and WSe2 in magnetic fields $B_z$ up to 9T applied perpendicular to the sample plane. In MoSe2 monolayers the valley…

材料科学 · 物理学 2015-06-12 G. Wang , L. Bouet , M. M. Glazov , T. Amand , E. L. Ivchenko , E. Palleau , X. Marie , B. Urbaszek

Embedding a WS$_2$ monolayer in flakes of hexagonal boron nitride allowed us to resolve and study the photoluminescence response due to both singlet and triplet states of negatively charged excitons (trions) in this atomically thin…

介观与纳米尺度物理 · 物理学 2018-06-08 D. Vaclavkova , J. Wyzula , K. Nogajewski , M. Bartos , A. O. Slobodeniuk , C. Faugeras , M. Potemski , M. R. Molas

Photoluminescence (PL) of transition metal dichalcogenide (TMD) monolayers is strongly influenced by the dielectric environment. The defect states present in the substrate induces uncontrollable doping in the TMD monolayer and thereby…

We investigate the transport of excitons and trions in monolayer semiconductor WS$_2$ subjected to controlled non-uniform mechanical strain. We actively control and tune the strain profiles with an AFM-based setup in which the monolayer is…

介观与纳米尺度物理 · 物理学 2020-05-20 Moshe G. Harats , Jan N. Kirchhof , Mengxiong Qiao , Kyrylo Greben , Kirill I. Bolotin

Excitons are composite bosons that can feature spin singlet and triplet states. In usual semiconductors, without an additional spin-flip mechanism, triplet excitons are extremely inefficient optical emitters. Large spin-orbit coupling in…

Monolayer transition metal dichalcogenide (TMDC) crystals, as direct-gap materials with unusually strong light-matter interaction, have attracted much recent attention. In contrast to the initial understanding, the minima of the conduction…

The effect of an external in-plane electric field on neutral and charged exciton states in two-dimensional (2D) materials is theoretically investigated. These states are argued to be strongly bound, so that electron-hole dissociation is not…

材料科学 · 物理学 2021-03-31 L. S. R. Cavalcante , D. R. da Costa , G. A. Farias , D. R. Reichman , A. Chaves

Structural, electronic, and chemical nanoscale modifications of transition metal dichalcogenide monolayers alter their optical properties, including the generation of single photon emitters. A key missing element for complete control is a…

The origin of the variation of photoluminescence (PL) spectra of monolayer tungsten disulfide (WS2) is investigated systematically. Dependence of the PL spectrum on the excitation power show that the relatively sharp component corresponds…

介观与纳米尺度物理 · 物理学 2018-06-01 Yongjae Kwon , Kangwon Kim , Wontaek Kim , Sunmin Ryu , Hyeonsik Cheong

The optically dark states play an important role in the electronic and optical properties of monolayers (MLs) of semiconducting transition metal dichalcogenides. The effect of temperature on the in-plane-field activation of the neutral and…

Two-dimensional semiconductors exhibit pronounced many-body effects and intense optical responses due to strong coulombic interactions. Consequently, subtle differences in photoexcitation conditions can strongly influence how the material…

The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

The possibility of electrical manipulation and detection of charged exciton (trion) before its radiative recombination makes it promising for excitonic devices. Using a few-layer graphene/monolayer WS$_{2}$/monolayer graphene vertical…

介观与纳米尺度物理 · 物理学 2019-04-04 Sangeeth Kallatt , Sarthak Das , Suman Chatterjee , Kausik Majumdar

Strong Coulomb interaction in monolayer transition metal dichalcogenides can facilitate nontrivial many-body effects among excitonic complexes. Many-body effects like exciton-exciton annihilation (EEA) have been widely explored in this…

介观与纳米尺度物理 · 物理学 2022-04-05 Suman Chatterjee , Garima Gupta , Sarthak Das , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

Monolayer phosphorene provides a unique two-dimensional (2D) platform to investigate the fundamental dynamics of excitons and trions (charged excitons) in reduced dimensions. However, owing to its high instability, unambiguous…

材料科学 · 物理学 2015-04-30 Jiong Yang , Renjing Xu , Jiajie Pei , Ye Win Myint , Fan Wang , Zhu Wang , Shuang Zhang , Zongfu Yu , Yuerui Lu