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The breathing pyrochlore lattice material Ba$_3$Yb$_2$Zn$_5$O$_{11}$ exists in the nearly decoupled limit, in contrast to most other well-studied breathing pyrochlore compounds. As a result, it constitutes a useful platform to benchmark…

Ba3Yb2Zn5O11 is unique among breathing pyrochlore compounds for being in the nearly decoupled limit where inter-tetrahedron interactions are weak, hosting isolated clusters or "molecular magnet" like tetrahedra of magnetic ytterbium (Yb3+)…

Paramagnetic correlations in the magnetic material Yb2Ti2O7 have been investigated via neutron scattering, revealing a [111] rod of scattering intensity. Assuming interactions between the Yb^{3+} ions composed of all symmetry-allowed…

We report inelastic neutron scattering measurements from our newly synthesized single crystals of the structurally metastable antiferromagnetic pyrochlore Yb$_{2}$Ge$_{2}$O$_{7}$. We determine the four symmetry-allowed nearest-neighbor…

Recently a new class of quantum magnets, the so-called breathing pyrochlore spin systems, have attracted much attention due to their potential to host exotic emergent phenomena. Here, we present magnetometry, heat capacity, thermal…

We consider the structure of anisotropic exchange interactions in ytterbium-based insulating rare-earth magnets built from edge-sharing octahedra. We argue the features of trivalent ytterbium and this structural configuration allow for a…

强关联电子 · 物理学 2018-08-14 Jeffrey G. Rau , Michel J. P. Gingras

Inelastic neutron scattering measurement is performed on a breathing pyrochlore antiferromagnet Ba3Yb2Zn5O11. The observed dispersionless excitations are explained by a crystalline electric field (CEF) Hamiltonian of Kramers ion Yb3+ of…

材料科学 · 物理学 2016-03-03 T. Haku , M. Soda , M. Sera , K. Kimura , S. Itoh , T. Yokoo , T. Masuda

In the Heisenberg antiferromagnet $Gd_2Ti_2O_7$, the exchange interactions are geometrically frustrated by the pyrochlore lattice structure. This ESR study reveals a strong temperature dependent anisotropy with respect to a [111] body…

强关联电子 · 物理学 2016-08-16 A. K. Hassan , L. P. Lévy , C. Darie , P. Strobel

By the single crystal inelastic neutron scattering the orthoferrite HoFeO3 was studied. We show that the spin dynamics of the Fe subsystem does not change through the spin-reorientation transitions. The observed spectrum of magnetic…

材料科学 · 物理学 2020-04-09 A. K. Ovsyanikov , I. A. Zobkalo , W. Schmidt , S. N. Barilo , S. A. Guretskii , V. Hutanu

Thermomagnetic and inelastic neutron scattering measurements on Na2PrO3 are reported. This material is an antiferromagnetic honeycomb magnet based on the tetravalent lanthanide Pr4+ and has been proposed to host dominant antiferromagnetic…

Fe3-xGeTe2 is an itinerant ferromagnet composed of two-dimensional layers weakly connected by van der Waals bonding that shows a variety of intriguing phenomena. Inelastic neutron scattering measurements on bulk single crystals of…

强关联电子 · 物理学 2019-03-27 S. Calder , A. I. Kolesnikov , A. F. May

We study low energy excitations in the quantum breathing pyrochlore antiferromagnet Ba$_3$Yb$_2$Zn$_5$O$_{11}$ by combination of inelastic neutron scattering (INS) and thermodynamical properties measurements. The INS spectra are…

We report an extensive study on the zero field ground state of a powder sample of the pyrochlore $\mathrm{Yb_2Ti_2O_7}$. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK.…

The magnetic excitation spectrum of the unconventional ferromagnet CeRh$_{3}$B$_{2}$ was measured by inelastic neutron scattering on single crystal sample in the magnetically ordered and paramagnetic phases. The spin-wave excitation…

强关联电子 · 物理学 2012-02-29 S. Raymond , J. Panarin , F. Givord , A. P. Murani , J. X. Boucherle , P. Lejay

We have studied the low energy spin dynamics between 4.6K and 0.07K in a Tb2Ti2O7 single crystal sample, by means of inelastic neutron scattering experiments. The spectra consist in a dual response, with a static and an inelastic…

强关联电子 · 物理学 2015-06-11 Sylvain Petit , Pierre Bonville , Julien Robert , Claudia Decorse , Isabelle Mirebeau

The synthesis and characterization of a new Yb-based material Ba3Yb2Zn5O11 are reported. This material is identified as the first model system of a pseudospin-1/2 quantum antiferromagnet on "breathing" pyrochlore lattice characterized by an…

强关联电子 · 物理学 2014-09-02 K. Kimura , S. Nakatsuji , T. Kimura

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

强关联电子 · 物理学 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras

We present a comprehensive ellipsometric study of an untwinned, nearly stoichiometric LaMnO_3 crystal in the spectral range 1.2-6.0 eV at temperatures 20 K < T < 300 K. The complex dielectric response along the b and c axes of the Pbnm…

强关联电子 · 物理学 2015-05-13 N. N. Kovaleva , Andrzej M. Oles , A. M. Balbashov , A. Maljuk , D. N. Argyriou , G. Khaliullin , B. Keimer

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

无序系统与神经网络 · 物理学 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic $\text{Cu}_2\text{OSeO}_3$. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic…

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