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An infrared study of the phonon spectra of ZrW2O8 as a function of temperature which includes the low energy (2-10 meV) region relevant to negative thermal expansion is reported and discussed in the context of specific heat and neutron…

材料科学 · 物理学 2010-07-28 Jason N. Hancock , Chandra Turpen , Zack Schlesinger , Glen Kowach , Art Ramirez

The electronic and optical parameters of {\gamma}-Al2O3 and {\theta}-Al2O3 have been studied by using the first principle within the framework of density function theory (DFT). The computational approach is based on full-potential…

材料科学 · 物理学 2019-03-21 Ahmed S. Jbara , Zulkafli Othaman , H. A. Rahnamaye Aliabad , M. A. Saeed

Negative thermal expansion in ZrW2O8 was investigated using a flexibility analysis of ab-initio phonons. It was shown that no previously proposed mechanism adequately describes the atomic-scale origin of negative thermal expansion in this…

材料科学 · 物理学 2016-02-17 Leila H. N. Rimmer , Martin T. Dove , Keith Refson

Zirconium hydride is an important material for storage of hydrogen isotopes. Here we report the structural, electronic, vibrational and thermodynamic properties of ZrH2, ZrD2 and ZrT2 using density functional theory (DFT). The structural…

材料科学 · 物理学 2013-05-28 D. Chattaraj , S. C. Parida , Smruti Dash , C. Majumder

This paper gives a short overview of the calculation of thermal properties of materials from first principles, using the Quasi-Harmonic Approximation (QHA). We first introduce some of the thermal properties of interest and describe how they…

材料科学 · 物理学 2011-12-22 Stefano Baroni , Paolo Giannozzi , Eyvaz Isaev

The hydration and ammonization of ZrW2O8 is known to lead to positive and negative thermal expansion behaviour respectively. We report ab-initio calculations to understand this anomalous behaviour. We identify the crucial low energy phonon…

材料科学 · 物理学 2018-12-12 M. K. Gupta , R. Mittal , Baltej Singh , S. L. Chaplot

The structural, electronic and optical properties of nearly ferromagnetic compound HfZn2 have been studied using ab-initio technique. We have carried out the plane-wave pseudopotential approach within the framework of the first-principles…

材料科学 · 物理学 2016-05-17 Md. Atikur Rahman , Md. Afjalur Rahman , Md. Zahidur Rahaman

The electronic structure and properties of PuO$_{2}$ and Pu$_{2}$O$_{3}$ have been studied from first principles by the all-electron projector-augmented-wave (PAW) method. The local density approximation (LDA)+$U$ and the generalized…

材料科学 · 物理学 2007-12-24 Bo Sun , Ping Zhang , Xian-Geng Zhao

We report a comprehensive temperature dependent Raman measurements on three different phases of monolayer WS2 from 4K to 330K in a wide spectral range. Our studies revels the anomalous nature of the first as well as the higher order…

材料科学 · 物理学 2020-01-08 Deepu Kumar , Birender Singh , Pawan Kumar , Viswanath Balakrishnan , Pradeep Kumar

Chalcogenide perovskites offer superior thermal and aqueous stability as well as a benign elemental composition compared to organic halide perovskites for optoelectronic applications. In this study, the structural, electrical, elastic,…

材料科学 · 物理学 2023-05-26 M. D. Kassa , N. G. Debelo , M. M. Woldemariam

The full-potential linearized augmented plane wave method with the generalized gradient approximation for the exchange-correlation potential (FLAPW-GGA) is used to predict the electronic and elastic properties of the newly discovered…

材料科学 · 物理学 2008-11-14 I. R. Shein , A. L. Ivanovskii

Structural, electronic, and optical properties for the cubic, tetragonal, and monoclinic crystalline phases of ZrO2, as derived from it ab initio full-relativistic calculations, are presented. The electronic structure calculations were…

Lattice parameter, electronic structure, mechanical and thermodynamic properties of ThN are systematically studied using the projector-augmented-wave method and the generalized gradient approximation based on the density functional theory.…

材料科学 · 物理学 2015-05-20 Yong Lu , Dafang Li , Bao-Tian Wang , Rong-Wu Li , Ping Zhang

The structural, dynamical, and thermodynamical properties of diamond, graphite and layered derivatives (graphene, rhombohedral graphite) are computed using a combination of density-functional theory (DFT) total-energy calculations and…

材料科学 · 物理学 2009-11-10 Nicolas Mounet , Nicola Marzari

The two-dimensional graphene-like carbon allotrope, graphyne, has been recently fabricated and exhibits many interesting electronic properties. In this work, we investigate the thermoelectric properties of {\gamma}-graphyne by performing…

介观与纳米尺度物理 · 物理学 2016-08-19 P. H. Jiang , H. J. Liu , L. Cheng , D. D. Fan , J. Zhang , J. Wei , J. H. Liang

The intermetallic compound ZrCo and its hydrides are important materials for their use in hydrogen isotope storage. The dynamical, thermodynamic and elastic properties of ZrCo and its hydrides ZrCoX3 (X= H, D and T) are reported. While the…

材料科学 · 物理学 2014-10-30 D. Chattaraj , S. C. Parida , Smruti Dash , C. Majumder

The elastic, thermodynamic, and electronic properties of fluorite RuO_2 under high pressure are investigated by plane-wave pseudopotential density functional theory. The optimized lattice parameters, elastic constants, bulk modulus, and…

材料科学 · 物理学 2017-08-23 Z. J. Yang , A. M. Guo , Y. D. Guo , J. Li , Z. Wang , Q. Liu , R. F. Linghu , X. D. Yang

Alloys of hexagonal $\delta$-phase UZr$_2$ have been synthesized and studied by means of heat capacity, magnetic susceptibility, magnetization, electrical resistivity, magnetoresistance, thermoelectric power, thermal conductivity…

In the realm of thermal expansion determination, the quasiharmonic approximation (QHA) stands as a widely embraced method for discerning minima of free energies across diverse temperatures such that the temperature dependence of lattice…

材料科学 · 物理学 2024-07-12 Samare Rostami , Xavier Gonze

The negative thermal expansion (NTE) compound ZrW2O8 has been well-studied because it remains cubic with a nearly constant, isotropic NTE coefficient over a broad temperature range. However, its elastic constants seem just as strange as its…

材料科学 · 物理学 2007-05-23 C. Pantea , A. Migliori , P. B. Littlewood , Y. Zhao , H. Ledbetter , T. Kimura , J. Van Duijn , G. R. Kowach
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