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The resonant transfer of energy from the inversion sublevels in NH$_3$ to He atoms in triplet Rydberg states with principal quantum number $n=38$ has been controlled using electric fields below 15 V/cm in intrabeam collisions at…

化学物理 · 物理学 2020-01-24 K. Gawlas , S. D. Hogan

We demonstrate Rydberg blockade due to the charge-dipole interaction between a single Rb atom and a single RbCs molecule confined in optical tweezers. The molecule is formed by magnetoassociation of a Rb+Cs atom pair and subsequently…

Low-energy collisions of Rydberg atom-ion systems are investigated theoretically. We present the parameter space associated with suitable approaches for the dynamics of Rydberg atom-ion collisions, i.e. quantum-, Langevin and classical…

原子物理 · 物理学 2021-04-22 Henrik Hirzler , Jesús Pérez-Ríos

We have studied the behavior of cold Rydberg atoms embedded in an ultracold plasma. We demonstrate that even deeply bound Rydberg atoms are completely ionized in such an environment, due to electron collisions. Using a fast pulse extraction…

量子物理 · 物理学 2009-11-10 Nicolas Vanhaecke , Daniel Comparat , Duncan A. Tate , Pierre Pillet

The Rydberg excitation blockade has been at the heart of an impressive array of recent achievements; however, state-mixing interactions can compromise its efficiency. When ultracold atoms are excited to Rydberg states near F\"orster…

原子物理 · 物理学 2022-09-05 Milo Eder , Andrew Lesak , Abigail Plone , Tomohisa Yoda , Michael Highman , Aaron Reinhard

Assemblies of highly excited Rydberg atoms in an ultracold gas can be set into motion by a combination of van-der-Waals and resonant dipole-dipole interactions. Thereby, the collective electronic Rydberg state might change due to…

原子物理 · 物理学 2021-12-15 Ritesh Pant , Rajat Agrawal , Sebastian Wüster , Jan-Michael Rost

We present a theoretical analysis of the implementation of an entangling quantum gate between two trapped Ca$^+$ ions which is based on the dipolar interaction among ionic Rydberg states. In trapped ions the Rydberg excitation dynamics is…

量子物理 · 物理学 2014-08-06 Weibin Li , Igor Lesanovsky

We derive a quantum master equation for an atom coupled to a heat bath represented by a charged particle many-body environment. In Born-Markov approximation, the influence of the plasma environment on the reduced system is described by the…

原子物理 · 物理学 2016-05-04 Chengliang Lin , Christian Gocke , Gerd Röpke , Heidi Reinholz

Rydberg-atom ensembles are switched from a weakly- into a strongly-interacting regime via adiabatic transformation of the atoms from an approximately non-polar into a highly dipolar quantum state. The resultant electric dipole-dipole forces…

原子物理 · 物理学 2016-11-16 N. Thaicharoen , L. F. Gonçalves , G. Raithel

We present an overview of our recent investigations of long-range interactions in an ultracold Cs Rydberg gas. These interactions are studied by high-resolution photoassociation spectroscopy, using excitation close to one-photon transitions…

原子物理 · 物理学 2016-07-15 Heiner Saßmannshausen , Johannes Deiglmayr , Frédéric Merkt

We theoretically investigate the manipulation of the motional states of trapped ground-state atoms using Rydberg dressing via nonresonant laser fields. The forces resulting from Rydberg-state interaction between dressed neighboring atoms in…

量子物理 · 物理学 2017-01-10 L F Buchmann , K Mølmer , D Petrosyan

Rydberg dressing traditionally refers to a technique where interactions between cold atoms are imprinted through the far off-resonant continuous-wave excitation of high-lying Rydberg states. Dipolar interactions between these electronic…

原子物理 · 物理学 2025-05-07 Chris Nill , Sylvain de Léséleuc , Christian Groß , Igor Lesanovsky

Ultracold hybrid ion-atom traps offer the possibility of microscopic manipulation of quantum coherences in the gas using the ion as a probe. However, inelastic processes, particularly charge transfer can be a significant process of ion loss…

原子物理 · 物理学 2015-06-19 B. M. McLaughlin , H. D. L. Lamb , I. C. Lane , J. F. McCann

We propose a novel experimental method to extend the investigation of ion-atom collisions from the so far studied cold, essentially classical regime to the ultracold, quantum regime. Key aspect of this method is the use of Rydberg molecules…

原子物理 · 物理学 2018-04-18 T. Schmid , C. Veit , N. Zuber , R. Löw , T. Pfau , M. Tarana , M. Tomza

We present a method for generating cold neutral atoms via charge exchange reactions between trapped ions and Rydberg positronium. The high charge exchange reaction cross section leads to efficient neutralisation of the ions and since the…

原子物理 · 物理学 2017-06-07 W. A. Bertsche , M. Charlton , S. Eriksson

The charge transfer (ionization) of hydrogen Rydberg atoms (principal quantum number $n=25-34$) incident at a Cu(100) surface is investigated. Unlike fully metallic surfaces, where the Rydberg electron energy is degenerate with the…

化学物理 · 物理学 2016-06-22 J. A. Gibbard , M. Dethlefsen , M. Kohlhoff , C. J. Rennick , E. So , M. Ford , T. P. Softley

Resonant energy transfer (RET), between equal parity 1s65s$^3\mathrm{S}_1$ and 1s66s$^3\mathrm{S}_1$ Rydberg levels in helium has been observed in low-temperature ($\sim80$ mK) collisions with ammonia molecules which undergo inversion…

原子物理 · 物理学 2026-05-21 J. Zou , R. R. W. Wang , R. González-Férez , H. R. Sadeghpour , S. D. Hogan

When atoms are excited to high-lying Rydberg states they interact strongly with dipolar forces. The resulting state-dependent level shifts allow to study many-body systems displaying intriguing nonequilibrium phenomena, such as constrained…

量子物理 · 物理学 2024-09-04 Chris Nill , Kay Brandner , Beatriz Olmos , Federico Carollo , Igor Lesanovsky

We perform a comprehensive investigation of F\"orster resonant energy transfer in a room-temperature thermal mixture of ammonia molecules and rubidium Rydberg atoms. Fully state-resolved measurement of the Rydberg-atom populations is…

化学物理 · 物理学 2018-12-04 F. Jarisch , M. Zeppenfeld

The internal electric field of a Rydberg atom electron can bind a polar molecule to form a giant ultralong-range stable polyatomic molecule. Such molecules not only share their properties with Rydberg atoms, they possess huge permanent…

原子物理 · 物理学 2015-05-27 Seth T. Rittenhouse , M. Mayle , P. Schmelcher , H. R. Sadeghpour