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We report inelastic neutron scattering measurements of the magnetic excitations in Ba2CuTeO6, proposed by ab initio calculations to magnetically realize weakly coupled antiferromagnetic two-leg spin-1/2 ladders. Isolated ladders are…

We report the magnetic susceptibility and the low-temperature specific heat of a double perovskite compound, Sr2CuTeO6, which is expected as the spin-1/2 square-lattice Heisenberg antiferromagnet with nearest-neighbor J1 and…

强关联电子 · 物理学 2015-06-23 Tomoyuki Koga , Nobuyuki Kurita , Hidekazu Tanaka

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

The manganese tellurate Li2MnTeO6 consists of trigonal spin lattices made up of Mn4+ (d3, S = 3/2) ions. The magnetic properties of this compound were characterized by several experimental techniques, which include magnetic susceptibility,…

The B-site ordered double perovskite Ba2CaOsO6 was studied by d.c. magnetic susceptibility, powder neutron diffraction and muon spin relaxation methods. The lattice parameter is a = 8.3619(6) A at 280K and cubic symmetry (Fm-3m) is retained…

We present single-crystal growth and magnetic property studies of tellurium-bridged copper spin-1/2 system Ba$_2$CuTeO$_6$. The spin-exchange interaction among copper spins via Cu-O-Te-O-Cu super-superexchange route leads to a novel two-leg…

We report on zero-field muon spin rotation, electron spin resonance and polarized Raman scattering measurements of the coupled quantum spin ladder Ba2CuTeO6. Zero-field muon spin rotation and electron spin resonance probes disclose a…

A new nanoscale ordered perovskite cobaltite, which consists of 90 degree ordered domains of the layered-112 LaBaCo2O6 has been evidenced by high resolution- transmission electron microscopy. This new form, like the disordered…

材料科学 · 物理学 2011-11-10 Asish K. Kundu , E. -L. Rautama , Ph. Boullay , V. Caignaert , V. Pralong , B. Raveau

A new series of cubic double perovskites Ba$_2R_{2/3}$TeO$_6$ ($R$ = Y, La, Pr, Nd, Sm-Lu) was synthesized via solid state reaction. The $R^{3+}$ and Te$^{6+}$ ions are ordered on alternating octahedral sites, with the rare earth sites 2/3…

材料科学 · 物理学 2019-03-14 Tai Kong , Robert J. Cava

The spin-1/2 Cu2+ ions in beta-Cu3V2O8 occupy the sites of a Kagome-staircase lattice, an anisotropic variant of the Kagome net: buckled layers and imbedded plaquettes of three edge-shared CuO4 squares break the ideal Kagome symmetry.…

凝聚态物理 · 物理学 2012-08-16 N. Rogado , M. K. Haas , G. Lawes , D. A. Huse , A. P. Ramirez , R. J. Cava

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

We report on the quasi-two-dimensional magnetism of the natural mineral diaboleite Pb2Cu(OH)4Cl2 with a tetragonal crystal structure, which is closely related to that of the frustrated spin-1/2 magnet PbVO3. Magnetic susceptibility of…

材料科学 · 物理学 2013-02-15 Alexander A. Tsirlin , Oleg Janson , Stefan Lebernegg , Helge Rosner

The magnetic properties of polycrystalline samples of Ba3Cu3In4O12 (In-334) and Ba3Cu3Sc4O12 (Sc-334) are reported. Both 334 phases have a structure derived from perovskite, with CuO4 squares interconnected to form half-twist ladders along…

强关联电子 · 物理学 2012-03-28 S. E. Dutton , M. Kumar , Z. G. Soos , C. L. Broholm , R. J. Cava

A comprehensive theoretical and experimental study is presented of the magnetic susceptibility versus temperature \chi(T) of spin S = 1/2 two- and three-leg Heisenberg ladders and ladder oxide compounds. Extensive quantum Monte Carlo…

We establish the double perovskite Ba$_2$CeIrO$_6$ as a nearly ideal model system for j=1/2 moments, with resonant inelastic x-ray scattering indicating a deviation of less than 1% from the ideally cubic j=1/2 state. The local j=1/2 moments…

\SCWO is a tetragonal ($I4/m$) double perovskite with diamagnetic W$^{6+}$ (5d$^0$) and (Jahn-Teller-active) Cu$^{2+}$ (3$d^9$) in a rocksalt-ordered arrangement on the B sites, modelling an anisotropic fcc-lattice antiferromagnet with…

We investigate magnetic, thermal, and dielectric properties of SrCuTe2O6, which is isostructural to PbCuTe2O6, a recently found, Cu-based 3D frustrated magnet with a corner sharing triangular spin network having dominant first and second…

The isostructural double perovskites Ba$_2$CuTeO$_6$ and Ba$_2$CuWO$_6$ are shown by theory and experiment to be frustrated square-lattice antiferromagnets with opposing dominant magnetic interactions. This is driven by differences in…

We construct and analyze a microscopic model for insulating rock salt ordered double perovskites, with the chemical formula A$_2$BB'O$_6$, where the B' atom has a 4d$^1$ or 5d$^1$ electronic configuration and forms a face centered cubic…

强关联电子 · 物理学 2018-10-08 Gang Chen , Rodrigo Pereira , Leon Balents
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