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We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

强关联电子 · 物理学 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

We report structural, magnetic, transport and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 < x< 0.65). Ca2RuO4 is a structurally-driven Mott insulator with a metal-insulator transition at TMI = 357 K, which is well separated from…

强关联电子 · 物理学 2016-04-26 S. J. Yuan , J. Terzic , J. C. Wang , S. Aswartham , W. H. Song , F. Ye , G. Cao

We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin flop transition from…

The magnetic structure of RuO2 and the Ru atomic configuration are unknown. A magnetic structure is inferred by confronting measured and calculated Bragg diffraction patterns and adjusting the latter to achieve satisfactory agreement. An…

强关联电子 · 物理学 2023-06-22 S. W. Lovesey , D. D. Khalyavin , G. van der Laan

The structure of Nd$_{1-x}$Pb$_{x}$MnO$_{3}$ crystals is determined by single crystal X-ray diffraction. Substitution of Pb at the Nd site results in structural phase change from tetragonal (x = 0.25) to cubic (x = 0.37). These changes are…

强关联电子 · 物理学 2007-05-23 Nilotpal Ghosh , Suja Elizabeth , H. L. Bhat , G. Nalini , B. Muktha , T. N. Guru Row

The phase diagram of Ca$_{2-x}$Sr$_x$RuO$_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of…

超导电性 · 物理学 2009-10-31 O. Friedt , M. Braden , G. Andre , P. Adelmann , S. Nakatsuji , Y. Maeno

Crystal structure, electronic state of Ir$^{4+}$, and magnetic properties of the antifluorite compound K$_2$IrBr$_6$ are studied using high-resolution synchrotron x-ray diffraction, resonant inelastic x-ray scattering (RIXS), thermodynamic…

强关联电子 · 物理学 2021-04-02 Nazir Khan , Danil Prishchenko , Mary H. Upton , Vladimir G. Mazurenko , Alexander A. Tsirlin

We report on the spin structure of the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ that could be directly determined by means of powder neutron diffraction. Our magnetic structure refinement unravels a so-called all-in/all-out magnetic structure…

强关联电子 · 物理学 2016-10-14 H. Guo , C. Ritter , A. C. Komarek

Single crystal neutron diffraction reveals two distinct components to the magnetic ordering in geometrically frustrated SrEr$_2$O$_4$. One component is a long-range ordered ${\bf k}=0$ structure which appears below $T_N = 0.75$ K. Another…

强关联电子 · 物理学 2014-08-15 T. J. Hayes , G. Balakrishnan , P. P. Deen , P. Manuel , L. C. Chapon , O. A. Petrenko

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

强关联电子 · 物理学 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

Neutron single crystal diffraction and rotational anisotropy optical second harmonic generation data are presented resolving the nature of the structural distortion realized in electron-doped (Sr$_{1-x}$La$_x$)$_3$Ir$_2$O$_7$ with $x=0.035$…

强关联电子 · 物理学 2017-06-28 Tom Hogan , Xiaoping Wang , H. Chu , David Hsieh , Stephen D. Wilson

Layered ruthenates are prototype materials with strong structure-property correlations. We report the structural and physical properties of double-layered perovskite Sr3(Ru1-xMnx)2O7 single crystals with 0<=x<=0.7. Single crystal x-ray…

强关联电子 · 物理学 2012-05-01 Biao Hu , Gregory T. McCandless , V. O. Garlea , S. Stadler , Yimin Xiong , Julia Y. Chan , E. W. Plummer , R. Jin

Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J$_{eff}=1/2$ Mott insulating iridate Sr$_2$IrO$_4$. Comparisons are drawn between the correlated magnetism in this single…

Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the…

强关联电子 · 物理学 2024-10-08 Y. Nambu , M. Kawamata , X. Pang , H. Murakawa , M. Avdeev , H. Kimura , H. Masuda , N. Hanasaki , Y. Onose

RuO$_2$ was considered for a long time to be a paramagnetic metal with an ideal rutile-type structure down to low temperatures, but recent studies on single-crystals claimed evidence for antiferromagnetic order and some symmetry breaking in…

The crystal and magnetic structure of La_{1-x}Sr_{1+x}MnO_4 (0<x<0.7) has been studied by diffraction techniques and high resolution capacitance dilatometry. There is no evidence for a structural phase transition like those found in…

材料科学 · 物理学 2009-11-10 D. Senff , P. Reutler , M. Braden , O. Friedt , D. Bruns , A. Cousson , F. Bouree , M. Merz , B. Buechner , A. Revcolevschi

Samarium doped BiFeO3 compounds having nano-size crystallites were prepared by the ethylene glycol assisted sol-gel synthesis method. X-ray diffraction and SEM measurements as well as Raman spectroscopy and FTIR experiments were used to…

Magnetic structure of tetragonal UAu$_2$Si$_2$ was investigated by single-crystal neutron diffraction experiments. Below $T_{\rm N}$ = 20 K it orders antiferromagnetically with a propagation vector of $k = (2/3, 0, 0)$ and magnetic moments…

A complete structural solution of the bilayer iridate compound Sr3Ir2O7 presently remains outstanding. Previously reported structures for this compound vary and all fail to explain weak structural violations observed in neutron scattering…

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