相关论文: A Chemical Kinetics Network for Lightning and Life…
Determining the habitability and interpreting atmospheric spectra of exoplanets requires understanding their atmospheric physics and chemistry. We use a 3-D Coupled Climate-Chemistry Model, the Met Office Unified Model with the UK Chemistry…
The potential of prebiotic chemistry to propagate on an exoplanet fundamentally depends on whether the atmospheric conditions can facilitate the production of prebiotic feedstock molecules. Photochemical simulations of exoplanet atmospheres…
We aimed to build a new and updated C0-C2 chemical network to study the CHON disequilibrium chemistry of warm and hot exoplanet atmospheres that relies on extensively validated and recent state-of-the-art combustion networks. The…
We present an open-source and validated chemical kinetics code for studying hot exoplanetary atmospheres, which we name VULCAN. It is constructed for gaseous chemistry from 500 to 2500 K using a reduced C-H-O chemical network with about 300…
Our purpose is to release a chemical network, and the associated rate coefficients, developed for the temperature and pressure range relevant to hot Jupiters atmospheres. Using this network, we study the vertical atmospheric composition of…
With the advent of JWST and spectroscopic characterization of exoplanet atmospheres with unprecedented detail, there is a demand for a more complete picture of chemical and photochemical reactions and their impact on atmospheric…
The near-term capability to characterize terrestrial exoplanet atmospheres may bring us closer to discovering alien life through atmospheric data. However, remotely detectable candidate biosignature gases are subject to false positive…
The detection of the amino acid glycine and its amine precursor methylamine on the comet 67P/Churyumov-Gerasimenko by the Rosetta mission provides strong evidence for a cosmic origin of prebiotics on Earth. How and when such complex organic…
Lightning has been suggested to play a role in triggering the occurrence of bio-ready chemical species. Future missions (PLATO, ARIEL, HWO, LIFE) and ground-based ELTs will investigate the atmospheres of potentially habitable exoplanets. We…
Chemical compositions of exoplanets can provide key insights into their physical processes, and formation and evolutionary histories. Atmospheric spectroscopy provides a direct avenue to probe exoplanetary compositions. However, whether…
Growing evidence has indicated that the global composition distribution plays an indisputable role in interpreting observational data. 3D general circulation models (GCMs) with a reliable treatment of chemistry and clouds are particularly…
Chemical kinetics is becoming an increasingly vital component of hot Jupiter general circulation models (GCMs). Here we simulate the hot Jupiter WASP-96b using two chemical networks, a reduced chemical network frequently used in the GCM…
We present a comprehensive photochemistry model for exploration of the chemical composition of terrestrial exoplanet atmospheres. The photochemistry model is designed from the ground up to have the capacity to treat all types of terrestrial…
We present a model for lightning shock induced chemistry that can be applied to atmospheres of arbitrary H/C/N/O chemistry, hence for extrasolar planets and brown dwarfs. The model couples hydrodynamics and the STAND2015 kinetic gas-phase…
Hydrogen cyanide (HCN) is a critical reactive source of nitrogen for building key biomolecules relevant for the origin of life. Still, many HCN reactions remain uncharacterized by experiments and theory, and the complete picture of HCN…
Almost all planetary atmospheres are affected by disequilibrium chemical processes. In this paper we introduce our recently developed Chemical Kinetic Model (\texttt{ChemKM}). We show that the results of our HD189733b model are in good…
Saturnian moon Titan presents a compelling testbed for probing prebiotic chemistry beyond early Earth. Impact-generated melt pools provide transient aqueous habitats in an otherwise cryogenic environment. We use Cantera equilibrium models…
Hydrogen cyanide (HCN) is a key feedstock molecule for the production of life's building blocks. The formation of HCN in an N$_2$-rich atmospheres requires first that the triple bond between N$\equiv$N be severed, and then that the atomic…
A recent observation of the exoplanet K2-18b sparked interest among scientists - large amounts of carbon dioxide and methane were detected in an H2-rich background atmosphere. If the planet is a hycean world (liquid water ocean +…
The search for habitable exoplanets in the Universe is actively ongoing in the field of astronomy. The biggest future milestone is to determine whether life exists on such habitable exoplanets. In that context, oxygen in the atmosphere has…