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Graphene is a nonlinear material which can be used as a saturable absorber, frequency mixer and frequency multiplier. We investigate the third harmonic generation from graphene lying on different substrates, consisting of a dielectric…

介观与纳米尺度物理 · 物理学 2017-02-09 N. A. Savostianova , S. A. Mikhailov

Optical harmonic generation occurs when high intensity light ($>10^{10}$W/m$^{2}$) interacts with a nonlinear material. Electrical control of the nonlinear optical response enables applications such as gate-tunable switches and frequency…

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear…

It is shown that the massless energy spectrum of electrons and holes in graphene leads to the strongly non-linear electromagnetic response of this system. We predict that the graphene layer, irradiated by electromagnetic waves, emits…

介观与纳米尺度物理 · 物理学 2007-07-24 S. A. Mikhailov

The linear energy dispersion of graphene electrons leads to a strongly nonlinear electromagnetic response of this material. We develop a general quantum theory of the third-order nonlinear local dynamic conductivity of graphene…

介观与纳米尺度物理 · 物理学 2016-02-04 S. A. Mikhailov

We observe optical third harmonic generation from graphene and few-layer graphite flakes produced by exfoliation. The emission scales with the cube of the intensity of the incident near-infrared femtosecond pulses and has a wavelength that…

介观与纳米尺度物理 · 物理学 2013-03-20 Nardeep Kumar , Jatinder Kumar , Chris Gerstenkorn , Rui Wang , Hsin-Ying Chiu , Arthur L. Smirl , Hui Zhao

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching…

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

介观与纳米尺度物理 · 物理学 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

Materials with massless Dirac fermions can possess exceptionally strong and widely tunable optical nonlinearities. Experiments on graphene monolayer have indeed found very large third-order nonlinear responses, but the reported variation of…

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

强关联电子 · 物理学 2017-10-20 K. V. Germash , D. V. Fil

Graphene is a recently discovered carbon based material with unique physical properties. This is a monolayer of graphite, and the two-dimensional electrons and holes in it are described by the effective Dirac equation with a vanishing…

介观与纳米尺度物理 · 物理学 2009-11-13 S. A. Mikhailov , K. Ziegler

The linear electrodynamic properties of graphene -- the frequency-dependent conductivity, the transmission spectra and collective excitations -- are briefly outlined. The non-linear frequency multiplication effects in graphene are studied,…

介观与纳米尺度物理 · 物理学 2009-05-27 S. A. Mikhailov

The nonlinear responses of different materials provide useful mechanisms for optical switching, low noise amplification, and harmonic frequency generation. However, the nonlinear processes usually have an extremely weak nature and require…

光学 · 物理学 2017-08-24 Boyuan Jin , Tianjing Guo , Christos Argyropoulos

We develop a density matrix formalism in the length gauge to calculate the nonlinear response of intrinsic monolayer graphene at terahertz frequencies. Employing a tight-binding model, we find that the interplay of the interband and…

光学 · 物理学 2014-12-17 Ibraheem Al-Naib , J. E. Sipe , Marc M. Dignam

A quantum theory of the third-harmonic generation in graphene is presented. An analytical formula for the nonlinear conductivity tensor $\sigma^{(3)}_{\alpha\beta\gamma\delta}(\omega,\omega,\omega)$ is derived. Resonant maxima of the third…

介观与纳米尺度物理 · 物理学 2015-06-02 S. A. Mikhailov

Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of…

应用物理 · 物理学 2018-01-31 Parvin Navaeipour , Ibraheem Al-Naib , Marc M. Dignam

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

材料科学 · 物理学 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

The optical nonlinear effects can provide different advanced electromagnetic functionalities, such as wave mixing and phase conjugation, which can be applied in a variety of new applications. However, these effects usually suffer from…

光学 · 物理学 2020-06-29 Boyuan Jin , Christos Argyropoulos

If we stack up two layers of graphene while changing their respective orientation by some twisting angle, we end up with a system that has striking differences when compared to single-layer graphene. For a very specific value of this twist…

介观与纳米尺度物理 · 物理学 2024-09-18 Eduardo B. Molinero , Anushree Datta , María J. Calderón , Elena Bascones , Rui E. F. Silva

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The…

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