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Coherent and squeezed phonon oscillations can be excited in solids impulsively by a single femtosecond pulse whose duration is shorter that a phonon period. By applying the second ultrafast pump pulse these oscillations can be…

介观与纳米尺度物理 · 物理学 2013-04-30 O. V Misochko

We report the observation of dynamic fringe patterns in the diffuse scattering of extreme ultraviolet light from surfaces, following femtosecond optical excitation. At each point on the detector, the diffuse scattering intensity exhibits…

We study squeezed states of phonons, which allow a reduction in the quantum fluctuations of the atomic displacements to below the zero-point quantum noise level of coherent phonon states. We investigate the generation of squeezed phonon…

凝聚态物理 · 物理学 2009-10-30 X. Hu , Franco Nori

We study squeezed quantum states of phonons, which allow the possibility of modulating the quantum fluctuations of atomic displacements below the zero-point quantum noise level of coherent phonon states. We calculate the corresponding…

凝聚态物理 · 物理学 2009-10-28 X. Hu , Franco Nori

In this paper we investigate coherent and squeezed quantum states of phonons. The latter allow the possibility of modulating the quantum fluctuations of atomic displacements below the zero-point quantum noise level of coherent states. The…

凝聚态物理 · 物理学 2009-10-28 X. Hu , Franco Nori

Radio-frequency compressed ultrafast electron diffraction has been used to probe the coherent and incoherent coupling of impulsive electronic excitation at 1.55 eV (800 nm) to optical and acoustic phonon modes directly from the perspective…

Recent experiments demonstrating storage of optical pulses in acoustic phonons based on stimulated Brillouin scattering raise a number of questions about the spectral and temporal capacities of such protocols and the limitations of the…

We observe anharmonic decay of the photoexcited coherent A1g phonon in bismuth to points in the Brillouin zone where conservation of momentum and energy are satisfied for three-phonon scattering. The decay of a coherent phonon can be…

We discuss the mechanism of coherent phonon generation by Stimulated Ionic Raman Scattering, a process different from conventional excitation with near visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling between…

超导电性 · 物理学 2015-05-25 R. Mankowsky , M. Först , T. Loew , J. Porras , B. Keimer , A. Cavalleri

For over a century, x-ray scattering has been the most powerful tool for determining the equilibrium structure of crystalline materials. Deviations from perfect periodicity, for example due to thermal motion of the atoms, reduces the…

材料科学 · 物理学 2013-05-29 M. Trigo , Y. M Sheu , J. Chen , V. H. Vishwanath , T. Graber , R. Henning , D. A. Reis

The study of the fundamental properties of phonons is crucial to understand their role in applica- tions in quantum information science, where the active use of phonons is currently highly debated. A genuine quantum phenomenon associated…

介观与纳米尺度物理 · 物理学 2018-09-27 Daniel Wigger , Helge Gehring , V. Martin Axt , Doris E. Reiter , Tilmann Kuhn

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

We study theoretically the fluctuation properties of acoustic phonons created in a semiconductor quantum dot after ultrafast optical excitation. An excitation with a single ultrafast pulse creates an exciton confined to the quantum dot,…

介观与纳米尺度物理 · 物理学 2015-06-12 D. Wigger , D. E. Reiter , V. M. Axt , T. Kuhn

This article discusses quantum fluctuation properties of a crystal lattice, and in particular, phonon squeezed states. Squeezed states of phonons allow a reduction in the quantum fluctuations of the atomic displacements to below the…

介观与纳米尺度物理 · 物理学 2009-11-07 Xuedong Hu , Franco Nori

We report on the impulsive generation of coherent optical phonons in CdTe0.68Se0.32 nanocrystallites embedded in a glass matrix. Pump probe experiments using femtosecond laser pulses were performed by tuning the laser central energy to…

介观与纳米尺度物理 · 物理学 2009-11-10 A. V. Bragas , C. Aku-Leh , S. Costantino , Alka Ingale , J. Zhao , R. Merlin

Squeezed, nonclassical states are an integral tool of quantum metrology due to their ability to push the sensitivity of a measurement apparatus beyond the limits of classical states. While their creation in light has become a standard…

量子气体 · 物理学 2021-01-15 Paul Juschitz

We investigate from first-principles theory and experiment the generation of phonons on picosecond timescales and the relaxation of carriers in multiple conduction band valleys of photo-excited Ge by inter-valley electron-phonon scattering.…

介观与纳米尺度物理 · 物理学 2025-02-03 F. Murphy-Armando , É. D. Murray , I. Savić , M. Trigo , D. Reis , S. Fahy

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…

We directly measure by femtosecond time-resolved x-ray diffraction the E$_g$ symmetry coherent phonon excited in bismuth by strong optical excitation. The magnitude of the E$_g$ mode observed is 0.2 pm peak-to-peak, compared against the 2.7…

材料科学 · 物理学 2015-06-12 S. L. Johnson , P. Beaud , E. Möhr-Vorobeva , A. Caviezel , G. Ingold , C. J. Milne

We consider Brillouin scattering on short-lived phonon modes, such that the relative Brillouin shift between propagating and scattered waves is smaller than the relative width of phonon modes. In this case one phonon mode facilitates…

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